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Reconciling divergent estimates of oil and gas methane emissions.
Zavala-Araiza, Daniel; Lyon, David R; Alvarez, Ramón A; Davis, Kenneth J; Harriss, Robert; Herndon, Scott C; Karion, Anna; Kort, Eric Adam; Lamb, Brian K; Lan, Xin; Marchese, Anthony J; Pacala, Stephen W; Robinson, Allen L; Shepson, Paul B; Sweeney, Colm; Talbot, Robert; Townsend-Small, Amy; Yacovitch, Tara I; Zimmerle, Daniel J; Hamburg, Steven P.
Afiliação
  • Zavala-Araiza D; Environmental Defense Fund, Austin, TX 78701;
  • Lyon DR; Environmental Defense Fund, Austin, TX 78701;
  • Alvarez RA; Environmental Defense Fund, Austin, TX 78701;
  • Davis KJ; Carbon Now Cast, LLC, State College, PA 16802;
  • Harriss R; Environmental Defense Fund, Austin, TX 78701;
  • Herndon SC; Aerodyne Research, Inc., Billerica, MA 01821;
  • Karion A; Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309; Earth System Research Laboratory, National Oceanic and Atmospheric Administration, Boulder, CO 80305;
  • Kort EA; Department of Climate and Space Sciences and Engineering, University of Michigan, Ann Arbor, MI 48109;
  • Lamb BK; Department of Civil and Environmental Engineering, Washington State University, Pullman, WA 99163;
  • Lan X; Department of Earth and Atmospheric Sciences, University of Houston, Houston, TX 77004;
  • Marchese AJ; Department of Mechanical Engineering, Colorado State University, Fort Collins, CO 80523;
  • Pacala SW; Department of Ecology and Evolutionary Biology, Princeton University, Princeton, NJ 08544; pacala@princeton.edu shamburg@edf.org.
  • Robinson AL; Department of Mechanical Engineering, Carnegie Mellon University, Pittsburgh, PA 15213;
  • Shepson PB; Department of Chemistry, Purdue University, West Lafayette, IN 47907;
  • Sweeney C; Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309; Earth System Research Laboratory, National Oceanic and Atmospheric Administration, Boulder, CO 80305;
  • Talbot R; Department of Earth and Atmospheric Sciences, University of Houston, Houston, TX 77004;
  • Townsend-Small A; Department of Geology, University of Cincinnati, Cincinnati, OH 45221.
  • Yacovitch TI; Aerodyne Research, Inc., Billerica, MA 01821;
  • Zimmerle DJ; Department of Mechanical Engineering, Colorado State University, Fort Collins, CO 80523;
  • Hamburg SP; Environmental Defense Fund, Austin, TX 78701; pacala@princeton.edu shamburg@edf.org.
Proc Natl Acad Sci U S A ; 112(51): 15597-602, 2015 Dec 22.
Article em En | MEDLINE | ID: mdl-26644584
Published estimates of methane emissions from atmospheric data (top-down approaches) exceed those from source-based inventories (bottom-up approaches), leading to conflicting claims about the climate implications of fuel switching from coal or petroleum to natural gas. Based on data from a coordinated campaign in the Barnett Shale oil and gas-producing region of Texas, we find that top-down and bottom-up estimates of both total and fossil methane emissions agree within statistical confidence intervals (relative differences are 10% for fossil methane and 0.1% for total methane). We reduced uncertainty in top-down estimates by using repeated mass balance measurements, as well as ethane as a fingerprint for source attribution. Similarly, our bottom-up estimate incorporates a more complete count of facilities than past inventories, which omitted a significant number of major sources, and more effectively accounts for the influence of large emission sources using a statistical estimator that integrates observations from multiple ground-based measurement datasets. Two percent of oil and gas facilities in the Barnett accounts for half of methane emissions at any given time, and high-emitting facilities appear to be spatiotemporally variable. Measured oil and gas methane emissions are 90% larger than estimates based on the US Environmental Protection Agency's Greenhouse Gas Inventory and correspond to 1.5% of natural gas production. This rate of methane loss increases the 20-y climate impacts of natural gas consumed in the region by roughly 50%.
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Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Revista: Proc Natl Acad Sci U S A Ano de publicação: 2015 Tipo de documento: Article

Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Revista: Proc Natl Acad Sci U S A Ano de publicação: 2015 Tipo de documento: Article