A simple approach to generate high-energy few-cycle optical vortices with minimized topological charge dispersion is introduced. By means of numerical simulations, it is shown that, by leveraging the intrinsic properties of optical parametric chirped pulse amplification (OPCPA), clean transfer of topological charge from a high-energy narrowband pump pulse to a broadband idler is feasible under certain particular conditions, enabling the generation of high-energy few-cycle vortex pulses with extremely low topological charge dispersion.
Since its first demonstration in 2016, the multi-pass spectral broadening technique has covered impressive ranges of pulse energy (3 µJ - 100 mJ) and peak power (4 MW - 100 GW). Energy scaling of this technique into the joule-level is currently limited by phenomena such as optical damage, gas ionization and spatio-spectral beam inhomogeneity. These limitations can be overcome by the novel multi-pass convex-concave arrangement, which exhibits crucial properties such as large mode size and compactness. In a proof-of-principle experiment, 260 fs, 15 µJ and 200 µJ pulses are broadened and subsequently compressed to approximately 50 fs with 90% efficiency and excellent spatio-spectral homogeneity across the beam profile. We simulate the proposed concept for spectral broadening of 40 mJ and 1.3 ps input pulses and discuss the possibility of further scaling.
Few-cycle pulses present an essential tool to track ultrafast dynamics in matter and drive strong field effects. To address photon-hungry applications, high average power lasers are used which, however, cannot directly provide sub-100-fs pulse durations. Post-compression of laser pulses by spectral broadening and dispersion compensation is the most efficient method to overcome this limitation. We present a notably compact setup which turns a 0.1-GW peak power, picosecond burst-mode laser into a 2.9-GW peak power, 8.2-fs source. The 120-fold pulse duration shortening is accomplished in a two-stage hybrid multi-pass, multi-plate compression setup. To our knowledge, neither shorter pulses nor higher peak powers have been reported to-date from bulk multi-pass cells alone, manifesting the power of the hybrid approach. It puts, for instance, compact, cost-efficient, and high repetition rate attosecond sources within reach.
The output of a 200kHz, 34W, 300fs ytterbium amplifier is compressed to 31fs with >88% efficiency to reach a peak power of 2.5GW, which to date is a record for a single-stage bulk multi-pass cell. Despite operation 80 times above the critical power for self-focusing in bulk material, the setup demonstrates excellent preservation of the input beam quality. Extensive beam and pulse characterizations are performed to show that the compressed pulses are promising drivers for high harmonic generation and nonlinear optics in gases or solids.
Spectroscopy in the wavelength range from 2 to 11 µm (900 to 5000 cm-1) implies a multitude of applications in fundamental physics, chemistry, as well as environmental and life sciences. The related vibrational transitions, which all infrared-active small molecules, the most common functional groups, as well as biomolecules like proteins, lipids, nucleic acids, and carbohydrates exhibit, reveal information about molecular structure and composition. However, light sources and detectors in the mid-infrared have been inferior to those in the visible or near-infrared, in terms of power, bandwidth, and sensitivity, severely limiting the performance of infrared experimental techniques. This article demonstrates the generation of femtosecond radiation with up to 5 W at 4.1 µm and 1.3 W at 8.5 µm, corresponding to an order-of-magnitude average power increase for ultrafast light sources operating at wavelengths longer than 5 µm. The presented concept is based on power-scalable near-infrared lasers emitting at a wavelength near 1 µm, which pump optical parametric amplifiers. In addition, both wavelength tunability and supercontinuum generation are reported, resulting in spectral coverage from 1.6 to 10.2 µm with power densities exceeding state-of-the-art synchrotron sources over the entire range. The flexible frequency conversion scheme is highly attractive for both up-conversion and frequency comb spectroscopy, as well as for a variety of time-domain applications.
Noncollinear optical parametric amplifiers (NOPAs) have become the leading technique for the amplification of carrier-envelope phase (CEP)-stable, few-cycle pulses at high repetition rate and high average power. In this Letter, a NOPA operating at a repetition rate of 100 kHz delivering more than 24 W of average power before compression is reported. The amplified bandwidth supports sub-7 fs pulse durations and pulse compression close to the transform limit is realized. CEP stability after amplification is demonstrated. The system paves the way to attosecond pump-probe spectroscopy with electron-ion coincidence detection.
Peak and average power scalability is the key feature of advancing femtosecond laser technology. Today, near-infrared light sources are capable of providing hundreds of Watts of average power. These sources, however, scarcely deliver pulses shorter than 100 fs which are, for instance, highly beneficial for frequency conversion to the extreme ultraviolet or to the mid- infrared. Therefore, the development of power scalable pulse compression schemes is still an ongoing quest. This article presents the compression of 90 W average power, 190 fs pulses to 70 W, 30 fs. An increase in peak power from 18 MW to 60 MW is achieved. The compression scheme is based on cascaded phase-mismatched quadratic nonlinearities in BBO crystals. In addition to the experimental results, simulations are presented which compare spatially resolved spectra of pulses spectrally broadened in self-focusing and self-defocusing media, respectively. It is demonstrated that balancing self- defocusing and Gaussian beam convergence results in an efficient, power-scalable spectral broadening mechanism in bulk material.
During amplification in a noncollinear optical parametric amplifier the spatial and temporal coordinates of the amplified field are inherently coupled. These couplings or distortions can limit the peak intensity, among other things. In this work, a numerical study of the spatiotemporal distortions in BBO-based noncollinear optical parametric chirped-pulse amplifiers (NOPCPAs) is presented for a wide range of parameters and for different amplification conditions. It is shown that for Gaussian pump beams, gain saturation introduces strong distortions and high conversion efficiency always comes at the price of strong spatiotemporal couplings which drastically reduce the peak intensity even when pulse fronts of the pump and the signal are matched. However, high conversion efficiencies with minimum spatiotemporal distortions can still be achieved with flat-top pump beam profiles.
We report on the generation of a multi-octave, phase-stable continuum from the output of a Yb:YAG regenerative amplifier delivering 1-ps pulses with randomly varying carrier-envelope phase (CEP). The intrinsically CEP-stable spectral continuum spans from 450 nm to beyond 2500 nm, covering a spectral range of about 0.6 PHz. The generated coherent broadband light carries an energy of 4 µJ, which can be scaled to higher values if required. The system has been designed and is ideally suited for seeding broadband parametric amplifiers and multichannel synthesizers pumped by picosecond Yb:YAG amplifiers, obviating the need for active timing synchronization required in previous approaches. The presented concept paves the way to cost-effective, reliable all-Yb:YAG single-cycle sources with terawatt peak-power and tens-of-Watts average power.
Spectral broadening in bulk material is a simple, robust and low-cost method to extend the bandwidth of a laser source. Consequently, it enables ultrashort pulse compression. Experiments with a 38 MHz repetition rate, 50 W average power Kerr-lens mode-locked thin-disk oscillator were performed. The initially 1.2 µJ, 250 fs pulses are compressed to 43 fs by means of self-phase modulation in a single 15 mm thick quartz crystal and subsequent chirped-mirror compression. The losses due to spatial nonlinear effects are only about 40 %. A second broadening stage reduced the Fourier transform limit to 15 fs. It is shown that the intensity noise of the oscillator is preserved independent of the broadening factor. Simulations manifest the peak power scalability of the concept and show that it is applicable to a wide range of input pulse durations and energies.
We report a 100 W, 20 mJ, 1-ps, all-Yb:YAG thin-disk regenerative amplifier seeded by a microjoule-level Yb:YAG thin-disk Kerr-lens mode-locked oscillator. The regenerative amplifier is implemented in a chirped pulse amplification system and operates at an ambient temperature in air, delivering ultrastable output pulses at a 5 kHz repetition rate and with a root mean square power noise value of less than 0.5%. Second harmonic generation of the amplifier's output in a 1.5 mm-thick BBO crystal results in more than 70 W at 515 nm, making the system an attractive source for pumping optical parametric chirped pulse amplifiers in the visible and near-infrared spectral ranges.
Absorption at the idler wavelength in an optical parametric oscillator (OPO) is often considered detrimental. We show through simulations that pulsed OPOs with significant idler absorption can perform better than OPOs with low idler absorption both in terms of conversion efficiency and beam quality. The main reason for this is reduced back conversion. We also show how the beam quality depends on the beam width and pump pulse length, and present scaling relations to use the example simulations for other pulsed nanosecond OPOs.
Amplifiers, Electronic , Computer-Aided Design , Lasers, Solid-State , Models, Theoretical , Oscillometry/instrumentation , Energy Transfer , Equipment Design , Equipment Failure Analysis
A mid-infrared synchronously pumped optical parametric oscillator pumped by a femtosecond erbium-doped fiber laser is demonstrated and characterised. The idler is tunable from 3.7-4.7 µm, with a maximum average power of 37 mW and a pulse length of â¼ 480 fs at 4 µm. We compare the experimental results with numerical results based on an extensive simulation model.
We report on a ZnGeP(2)-based optical parametric oscillator (OPO) with 22 W of output power in the 3-5 µm range and a beam quality factor M(2) ≈1.4. The OPO uses a novel V-shaped 3-mirror ring resonator that allows two passes of the beams through the same nonlinear crystal. The pump is a 39 W hybrid Tm:fiber laser/Ho:YAG laser.
Amplifiers, Electronic , Lasers, Solid-State , Lenses , Oscillometry/instrumentation , Transducers , Computer-Aided Design , Equipment Design , Equipment Failure Analysis , Infrared Rays
We present three-dimensional simulations of optical-parametric chirped-pulse amplification stages for a few-cycle petawatt-class laser. The simulations take into account the effects of depletion, diffraction, walk-off, quantum noise, and the nonlinear refractive index (n(2)). In the absence of n(2) effects, we show these stages can generate 3.67J pulses supporting 4fs transform-limited pulse durations. Adding the nonlinear refractive index to the simulation, the energy output is reduced by ~11% and the bandwidth narrows by ~129nm, increasing the Fourier limit by ~17.5%.
We demonstrate with simulations and experiments that an optical parametric oscillator using two different crystals with orthogonal walk-off planes can generate a symmetric, high-quality beam even if the resonator has a high Fresnel number. In the experiments we used KTA and BBO crystals to convert 5 ns pulses at 1.06 microm to 1.7 microm pulses with more than 10 mJ energy and beam quality M(2) approximately 2.
A high power, efficient, and tunable laser source in the 8-10 microm range, based on a ZnGeP(2) optical parametric oscillator (OPO) pumped by a hybrid 2.1 microm laser is demonstrated. The hybrid laser consists of a Q-switched Ho:YAG laser pumped by a 15 W CW thulium fiber laser. With 8.9 W of 2.1 microm pump power we obtained 0.95 W at 8 microm with an M(2)-value of 2.7 from an OPO with two walk-off compensating crystals.
Amplifiers, Electronic , Germanium/chemistry , Lasers, Solid-State , Oscillometry/instrumentation , Phosphorus/chemistry , Zinc/chemistry , Equipment Design , Equipment Failure Analysis , Infrared Rays
Nonlinear optical conversion of 1.064 microm pulses from a Q-switched Nd:YAG laser to the mid-infrared is demonstrated. The experimental setup is based on a two-stage master-oscillator/power-amplifier (MOPA) design with a KTiOPO(4) based MOPA in the first stage and a KTiOAsO(4)/ZnGeP(2) based MOPA in the second stage. The setup can be tuned to provide output at 8 microm or in the 3-5 microm wavelength region. We obtain more than 8 mJ at 8 microm, and up to 33 mJ at 3-5 microm. The measured beam quality factors are in the range M(2) =2-4 for both wavelength regions.
Amplifiers, Electronic , Computer-Aided Design , Germanium/chemistry , Lasers , Phosphorus/chemistry , Zinc/chemistry , Computer Simulation , Equipment Design , Equipment Failure Analysis , Infrared Rays , Models, Theoretical
Group velocity mismatch (GVM) is a major concern in the design of optical parametric amplifiers (OPAs) and generators (OPGs) for pulses shorter than a few picoseconds. By simplifying the coupled propagation equations and exploiting their scaling properties, the number of free parameters for a collinear OPA is reduced to a level where the parameter space can be studied systematically by simulations. The resulting set of figures show the combinations of material parameters and pulse lengths for which high performance can be achieved, and they can serve as a basis for a design.
A simple scheme for generation of high power in the midinfrared is demonstrated. By using a 15 W thulium-doped fiber laser emitting at 1907 nm to pump a Q-switched Ho:YAG laser, we obtained 9.8 W at 2096 nm at a 20 kHz pulse repetition rate with excellent beam quality. The output of this laser was used to pump a doubly resonant zinc germanium phosphide based optical parametric oscillator, and we obtained 5.1 W average power in the 3-5 microm range with M2 approximately = 1.8.
