Critical behavior and the Kibble-Zurek mechanism in a musical phase transition.

We investigate the critical phenomena emerging from a statistical mechanics model of musical harmony on a three-dimensional (3D) lattice, and the resulting structure of the ordered phase. In this model, each lattice site represents a tone, with nearest neighbors interacting via the perception of dissonance between them. With dissonance assumed to be an octave-wise periodic function of pitch difference, this model is a 3D XY system with the same symmetry and dimensionality as superfluid helium and models of the cosmological axion field. We use numerical simulation to observe a phase transition from disordered sound to ordered arrangements of musical pitches as a parameter analogous to the temperature is quenched towards zero. We observe the divergence of correlation length and relaxation time at the phase boundary, consistent with the critical exponents in similar systems. Furthermore, the quenched low-temperature phase of these systems displays topological defects in the form of vortex strings that thread throughout the system volume. We observe the formation of these vortex strings in accordance with the Kibble-Zurek mechanism, and discuss the structure of these vortex strings in the context of the theory of musical harmony, finding both similarities to established music theory, and uncovering new avenues to explore.

Three-dimensional frequency- and phase-multiplexed magneto-optical microscopy.

We describe a new approach to scanning magneto-optical Kerr effect (MOKE) microscopy in which two opto-mechanical choppers modulate the spatial profile of a probe laser beam to separately encode all three magnetization components at different frequencies and phases in one signal. We demonstrate this multiplexed technique in two representative regimes: the equilibrium and non-equilibrium response of a magnetic vortex to a changing magnetic field. We observe the translation of the vortex state in equilibrium and the spiraling gyrotropic trajectory of the vortex position out of equilibrium. We compare the results to a traditional MOKE measurement and to micromagnetic simulations. We find that the multiplexed method presented here provides better agreement with simulation than previous methods and equal or better signal-to-noise ratio.

Cooperative Energy Transfer Controls the Spontaneous Emission Rate Beyond Field Enhancement Limits.

Quantum emitters located in proximity to a metal nanostructure individually transfer their energy via near-field excitation of surface plasmons. The energy transfer process increases the spontaneous emission (SE) rate due to plasmon-enhanced local field. Here, we demonstrate a significant acceleration of the quantum emitter SE rate in a plasmonic nanocavity due to cooperative energy transfer (CET) from plasmon-correlated emitters. Using an integrated plasmonic nanocavity, we realize up to sixfold enhancement in the emission rate of emitters coupled to the same nanocavity on top of the plasmonic enhancement of the local density of states. The radiated power spectrum retains the plasmon resonance central frequency and line shape, with the peak amplitude proportional to the number of excited emitters indicating that the observed cooperative SE is distinct from superradiance. Plasmon-assisted CET offers unprecedented control over the SE rate and allows us to dynamically control the spontaneous emission rate at room temperature which can enable SE rate based optical modulators.

The structure of musical harmony as an ordered phase of sound: A statistical mechanics approach to music theory.

Music, while allowing nearly unlimited creative expression, almost always conforms to a set of rigid rules at a fundamental level. The description and study of these rules, and the ordered structures that arise from them, is the basis of the field of music theory. Here, I present a theoretical formalism that aims to explain why basic ordered patterns emerge in music, using the same statistical mechanics framework that describes emergent order across phase transitions in physical systems. I first apply the mean field approximation to demonstrate that phase transitions occur in this model from disordered sound to discrete sets of pitches, including the 12-fold octave division used in Western music. Beyond the mean field model, I use numerical simulation to uncover emergent structures of musical harmony. These results provide a new lens through which to view the fundamental structures of music and to discover new musical ideas to explore.

Coaxial atomic force microscope probes for imaging with dielectrophoresis.

We demonstrate atomic force microscope (AFM) imaging using dielectrophoresis (DEP) with coaxial probes. DEP provides force contrast allowing coaxial probes to image with enhanced spatial resolution. We model a coaxial probe as an electric dipole to provide analytic formulas for DEP between a dipole, dielectric spheres, and a dielectric substrate. AFM images taken of dielectric spheres with and without an applied electric field show the disappearance of artifacts when imaging with DEP. Quantitative agreement between our model and experiment shows that we are imaging with DEP.

Imaging universal conductance fluctuations in graphene.

We study conductance fluctuations (CF) and the sensitivity of the conductance to the motion of a single scatterer in two-dimensional massless Dirac systems. Our extensive numerical study finds limits to the predicted universal value of CF. We find that CF are suppressed for ballistic systems near the Dirac point and approach the universal value at sufficiently strong disorder. The conductance of massless Dirac fermions is sensitive to the motion of a single scatterer. CF of order e(2)/h result from the motion of a single impurity by a distance comparable to the Fermi wavelength. This result applies to graphene systems with a broad range of impurity strength and concentration while the dependence on the Fermi wavelength can be explored via gate voltages. Our prediction can be tested by comparing graphene samples with varying amounts of disorder and can be used to understand interference effects in mesoscopic graphene devices.

Scaling of transverse nuclear magnetic relaxation due to magnetic nanoparticle aggregation.

The aggregation of superparamagnetic iron oxide (SPIO) nanoparticles decreases the transverse nuclear magnetic resonance (NMR) relaxation time T2CP of adjacent water molecules measured by a Carr-Purcell-Meiboom-Gill (CPMG) pulse-echo sequence. This effect is commonly used to measure the concentrations of a variety of small molecules. We perform extensive Monte Carlo simulations of water diffusing around SPIO nanoparticle aggregates to determine the relationship between T2CP and details of the aggregate. We find that in the motional averaging regime T2CP scales as a power law with the number N of nanoparticles in an aggregate. The specific scaling is dependent on the fractal dimension d of the aggregates. We find T2CP∝N-0.44 for aggregates with d = 2.2, a value typical of diffusion limited aggregation. We also find that in two-nanoparticle systems, T2CP is strongly dependent on the orientation of the two nanoparticles relative to the external magnetic field, which implies that it may be possible to sense the orientation of a two-nanoparticle aggregate. To optimize the sensitivity of SPIO nanoparticle sensors, we propose that it is best to have aggregates with few nanoparticles, close together, measured with long pulse-echo times.

Imaging coherent transport in graphene. Part II: probing weak localization.

Graphene has opened new avenues of research in quantum transport, with potential applications for coherent electronics. Coherent transport depends sensitively on scattering from microscopic disorder present in graphene samples: electron waves traveling along different paths interfere, changing the total conductance. Weak localization is produced by the coherent backscattering of waves, while universal conductance fluctuations are created by summing over all paths. In this work, we obtain conductance images of weak localization with a liquid-He-cooled scanning probe microscope, by using the tip to create a movable scatterer in a graphene device. This technique allows us to investigate coherent transport with a probe of size comparable to the electron wavelength. Images of magnetoconductance versus tip position map the effects of disorder by moving a single scatterer, revealing how electron interference is modified by the tip perturbation. The weak localization dip in conductivity at B = 0 is obtained by averaging magnetoconductance traces at different positions of the tip-created scatterer. The width Delta B(WL) of the dip yields an estimate of the electron coherence length L(phi) at fixed charge density. This 'scanning scatterer' method provides a new way of investigating coherent transport in graphene by directly perturbing the disorder configuration that creates these interferometric effects.