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1.
Langmuir ; 40(18): 9669-9675, 2024 May 07.
Artículo en Inglés | MEDLINE | ID: mdl-38648519

RESUMEN

With the fast development of the smart lifestyle in recent years, simple and flexible body condition monitoring has become more and more important. However, currently, commercially available motion-sensing devices always lack flexibility or at a high cost. This article has fully explored the merits of a commercial and easily available material of carbon fiber powder (CFP) and prepared CFP-based screen printing inks. This conductive ink can be directly and quickly printed onto a variety of different flexible common substrates, such as paper, cotton fabrics, etc., to prepare flexible sensors. At the same time, as a result of the good photothermal performance and conductivity of CFP, the printed flexible sensors have fast and stable performance on thermal and human motion detection. The use of CFP as the smart element to construct a wearable device will offer a choice for the intelligent industry.

2.
Chem Asian J ; 18(18): e202300483, 2023 Sep 15.
Artículo en Inglés | MEDLINE | ID: mdl-37553785

RESUMEN

Flexible sensors show great application potential in wearable electronics, human-computer interaction, medical health, bionic electronic skin and other fields. Compared with rigid sensors, hydrogel-based devices are more flexible and biocompatible and can easily fit the skin or be implanted into the body, making them more advantageous in the field of flexible electronics. In all designs, polyvinyl alcohol (PVA) series hydrogels exhibit high mechanical strength, excellent sensitivity and fatigue resistance, which make them promising candidates for flexible electronic sensing devices. This paper has reviewed the latest progress of PVA/plant-based biomass hydrogels in the construction of flexible sensor applications. We first briefly introduced representative plant biomass materials, including sodium alginate, phytic acid, starch, cellulose and lignin, and summarized their unique physical and chemical properties. After that, the design principles and performance indicators of hydrogel sensors are highlighted, and representative examples of PVA/plant-based biomass hydrogel applications in wearable electronics are illustrated. Finally, the future research is briefly prospected. We hope it can promote the research of novel green flexible sensors based on PVA/biomass hydrogel.

3.
ACS Appl Mater Interfaces ; 14(46): 52402-52410, 2022 Nov 23.
Artículo en Inglés | MEDLINE | ID: mdl-36256442

RESUMEN

Artificial intelligence (AI) has become increasingly popular along with the development of the bionic neural system. Ionic conductors play an important role in the AI system due to the ability of bionic sensing and signal transporting. Traditional low-polarity elastomers possess outstanding mechanical strength and stability, such as polyurethane, which is difficult to be directly endowed with ionic conductivity without impairing its properties. Herein, we have first put forward a new approach to synthesize a liquid-free ionic conductive polyurethane (CPU) through one-step copolymerization between a green deep eutectic solvent (DES) and a prepolymer of polyurethane. The as-prepared CPU can retain the native properties of the traditional polyurethane (PU) such as the homogeneous phase, ease of molding, high transparency (about 93.3%), and excellent mechanical properties. By introducing the DES as the covalent cross-linking agent and ionic conductor at the same time, the CPU also has fine ionic conductivity (3.78 × 10-5 S cm-1), environmental resistance like anti-freezing (-20 °C), and solvent resistance. Based on the excellent conductivity and mechanical strength, the flexible CPU can be applied as a sensing element in pressure sensors. The CPU-based sensor has presented long-term stability, high sensitivity, and wide-ranging response (0.17-3.28 MPa) to the applied pressure, which will be suitable for the industrial demands for practical applications.

4.
ACS Appl Mater Interfaces ; 12(33): 37637-37646, 2020 Aug 19.
Artículo en Inglés | MEDLINE | ID: mdl-32705862

RESUMEN

Photothermal conversion behavior has a vital application to disease therapy, water purification, or uncontacted heaters. The fabrication of high-performance photothermal conversion materials especially for near-infrared (NIR) light and microstructures has attracted a great deal of attention. Among numerous substances, MXene as a new type of 2D material with semi-metallic and unique electromagnetic properties presents a broader absorption of light and even a typical plasmonic absorption near the NIR-I area (808 nm), which has made it suitable for photothermal conversion. Here, we propose a facile approach for preparing a Ti3C2Tx/ionic liquid ink with a high photothermal conversion efficiency. The as-prepared ink has showed good wettability of various substrates as well as the high sensitivity of 808 nm NIR light irradiation and a wide range of thermal variation. After packing the ink into a gel pen refill, the flexible thermal chips could be easily obtained just by pen writing on the soft surface with the designed size, which also have become an optimal candidate for the thermal alarm system.

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