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1.
Nanoscale Horiz ; 9(6): 968-975, 2024 May 29.
Artículo en Inglés | MEDLINE | ID: mdl-38647350

RESUMEN

A single nanotube synthesized from a transition metal dichalcogenide (TMDC) exhibits strong exciton resonances and, in addition, can support optical whispering gallery modes. This combination is promising for observing exciton-polaritons without an external cavity. However, traditional energy-momentum-resolved detection methods are unsuitable for this tiny object. Instead, we propose to use split optical modes in a twisted nanotube with the flattened cross-section, where a gradually decreasing gap between the opposite walls leads to a change in mode energy, similar to the effect of the barrier width on the eigenenergies in the double-well potential. Using micro-reflectance spectroscopy, we investigated the rich pattern of polariton branches in single MoS2 tubes with both variable and constant gaps. Observed Rabi splitting in the 40-60 meV range is comparable to that for a MoS2 monolayer in a microcavity. Our results, based on the polariton dispersion measurements and polariton dynamics analysis, present a single TMDC nanotube as a perfect polaritonic structure for nanophotonics.

2.
J Phys Condens Matter ; 31(10): 105002, 2019 Mar 13.
Artículo en Inglés | MEDLINE | ID: mdl-30583291

RESUMEN

We report on experimental studies of the surface plasmon-phonon polariton excitations in heavily doped GaAs epitaxial layers. Reflection and emission of radiation in the frequency range of 2-19 THz were investigated for samples with surface-relief grating, as well as for samples with planar surface. The reflectivity spectrum for p-polarized radiation measured for the sample with the surface-relief grating demonstrates a set of resonances attributed to excitations of different surface plasmon-phonon polariton modes. The observed resonances lie beyond the limits of the Reststrahlen band. Terahertz radiation emission from the samples was studied in nonequilibrium conditions under the pulsed electric field excitation. Two contributions to the spectral density of the terahertz radiation have been revealed, the first being due to bulk plasmon-phonon polaritons (PPhPs), while the second originating from the surface PPhPs. A field dependence of the effective temperature of the bulk PPhPs has been established. Polarization dependence of the terahertz radiation related to surface PPhPs has been experimentally examined for the first time.

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