Modeling the space-time correlation of pulsed twin beams.

Entangled twin-beams generated by parametric down-conversion are among the favorite sources for imaging-oriented applications, due their multimodal nature in space and time. However, a satisfactory theoretical description is still lacking. In this work we propose a semi-analytic model which aims to bridge the gap between time-consuming numerical simulations and the unrealistic plane-wave pump theory. The model is used to study the quantum correlation and the coherence in the angle-frequency domain of the parametric emission, and demonstrates a [Formula: see text] growth of their size as the gain g increases, with a corresponding contraction of the space-time distribution. These predictions are systematically compared with the results of stochastic numerical simulations, performed in the Wigner representation, of the full model equations: an excellent agreement is shown even for parameters well outside the expected limit of validity of the model.

Study of Through-Hole Micro-Drilling in Sapphire by Means of Pulsed Bessel Beams.

Ultrashort Bessel beams have been used in this work to study the response of a 430-µm-thick monocrystalline sapphire sample to laser-matter interaction when injecting the beam orthogonally through the whole sample thickness. We show that with a 12° Bessel beam cone angle, we are able to internally modify the material and generate tailorable elongated microstructures while preventing the formation of surface cracks, even in the picosecond regime, contrary to what was previously reported in the literature. On the other hand, by means of Bessel beam machining combined with a trepanning technique where very high energy pulses are needed, we were able to generate 100 µm diameter through-holes, eventually with negligible cracks and very low taper angles thanks to an optimization achieved by using a 60-µm-thick layer of Kapton Polyimide removable tape.

Micro-Hole Generation by High-Energy Pulsed Bessel Beams in Different Transparent Materials.

Micro-drilling transparent dielectric materials by using non-diffracting beams impinging orthogonally to the sample can be performed without scanning the beam position along the sample thickness. In this work, the laser micromachining process, based on the combination of picosecond pulsed Bessel beams with the trepanning technique, is applied to different transparent materials. We show the possibility to create through-apertures with diameter on the order of tens of micrometers, on dielectric samples with different thermal and mechanical characteristics as well as different thicknesses ranging from two hundred to five hundred micrometers. Advantages and drawbacks of the application of this technique to different materials such as glass, polymer, or diamond are highlighted by analyzing the features, the morphology, and the aspect-ratio of the through-holes generated. Alternative Bessel beam drilling configurations, and the possibility of optimization of the quality of the aperture at the output sample/air interface is also discussed in the case of glass.

Hot-spots and gain enhancement in a doubly pumped parametric down-conversion process.

We experimentally investigate the parametric down-conversion process in a nonlinear bulk crystal, driven by two non-collinear pump modes. The experiment shows the emergence of bright hot-spots in modes shared by the two pumps, similar to the phenomenology recently observed in 2D nonlinear photonic crystals. By exploiting the spatial walk-off between the two extraordinary pump modes, we have been able to recreate a peculiar resonance condition, reported by a local enhancement of the parametric gain, which corresponds to a transition from a three-mode to a four-mode coupling. From a quantum point of view, this opens the way to the generation of multimode entangled states of light, such as tripartite or quadripartite states, in simple bulk nonlinear sources.

Laser surface structuring of diamond with ultrashort Bessel beams.

We investigate the effect of ultrafast laser surface machining on a monocrystalline synthetic diamond sample by means of pulsed Bessel beams. We discuss the differences of the trench-like microstructures generated in various experimental conditions, by varying the beam cone angle, the energy and pulse duration, and we present a brief comparison of the results with those obtained with the same technique on a sapphire sample. In diamond, we obtain V-shaped trenches whose surface width varies with the cone angle, and which are featured by micrometer sized channels having depths in the range of 10-20 µm. By laser writing crossed trenches we are also able to create and tailor on the diamond surface pillar-like or tip-like microstructures potentially interesting for large surface functionalization, cells capturing and biosensing.

Golden Ratio Gain Enhancement in Coherently Coupled Parametric Processes.

Nonlinear optical processes are an essential tool in modern optics, with a broad spectrum of applications, including signal processing, frequency conversion, spectroscopy and quantum optics. Ordinary parametric devices nevertheless still suffer from relatively low gains and wide spectral emission. Here we demonstrate a unique configuration for phase-matching multiple nonlinear processes in a monolithic 2D nonlinear photonic crystal, resulting in the coherent parametric emission of four signal and idler modes, featuring an exponential gain enhancement equal to the Golden Ratio. The results indicate a new route towards compact high-brightness and coherent sources for multi-photon generation, manipulation and entanglement, overcoming limitations of conventional parametric devices.

Broadband and efficient adiabatic three-wave-mixing in a temperature-controlled bulk crystal.

Nonlinear interactions are commonly used to access to wavelengths not covered by standard laser systems. In particular, optical parametric amplification (OPA) is a powerful technique to produce broadly tunable light. However, common implementations of OPA suffer from a well-known trade-off, either achieving high efficiency for narrow spectra or inefficient conversion over a broad bandwidth. This shortcoming can be addressed using adiabatic processes. Here, we demonstrate a novel technique towards this direction, based on a temperature-controlled phase mismatch between the interacting waves. Using this approach, we demonstrate, by tailoring the temperature profile, an increase in conversion efficiency by 21%, reaching a maximum of 57%, while simultaneously expanding the bandwidth to over 300 nm. Our technique can readily enhance the performances of current OPA systems.

Diamond photonics platform enabled by femtosecond laser writing.

Diamond is a promising platform for sensing and quantum processing owing to the remarkable properties of the nitrogen-vacancy (NV) impurity. The electrons of the NV center, largely localized at the vacancy site, combine to form a spin triplet, which can be polarized with 532 nm laser light, even at room temperature. The NV's states are isolated from environmental perturbations making their spin coherence comparable to trapped ions. An important breakthrough would be in connecting, using waveguides, multiple diamond NVs together optically. However, still lacking is an efficient photonic fabrication method for diamond akin to the photolithographic methods that have revolutionized silicon photonics. Here, we report the first demonstration of three dimensional buried optical waveguides in diamond, inscribed by focused femtosecond high repetition rate laser pulses. Within the waveguides, high quality NV properties are observed, making them promising for integrated magnetometer or quantum information systems on a diamond chip.

High visibility pump reconstruction via ultra broadband sum frequency mixing of intense phase-conjugated twin beams.

In this paper we show how after the generation of parametric down-conversion radiation (PDC) in the very high gain pulsed regime, we are able to reconstruct the pump via up-conversion of the twin beams originated from that PDC process. The peculiarity of the experiment is the ultra-broad spectral and angular bandwidth sent into the process of sum frequency mixing thanks to an achromatic imaging technique from the exit face of the PDC crystal using off-axis parabolic mirrors. The recorded spectra presented illustrate the high visibility recombination of the intense phase-conjugated signal and idler beams and pave the way for the investigation of both the spatial and temporal properties of the near field biphoton amplitude.

Colored conical emission by means of second-harmonic generation.

We predict that the combination of space and time modulational instabilities that occur by means of parametric wave mixing in quadratic media leads to colored conical emission. This phenomenon should be observed under conditions usually employed in second-harmonic experiments.