Demonstration of a combined differential absorption and high spectral resolution lidar for profiling atmospheric temperature.

This work presents the first demonstration of atmospheric temperature measurement using the differential absorption lidar (DIAL) technique. While DIAL is routinely used to measure atmospheric gases such as ozone and water vapor, almost no success has been found in using DIAL to measure atmospheric temperature. Attempts to measure temperature using a well-mixed gas like oxygen (O2) have largely failed based on a need for quantitative ancillary measurements of water vapor and atmospheric aerosols. Here, a lidar is described and demonstrated that simultaneously measures O2 absorption, water vapor number density, and aerosol backscatter ratio. This combination of measurements allows for the first measurements of atmospheric temperature with useful accuracy. DIAL temperature measurements are presented to an altitude of 4 km with 225 m and 30 min resolution with accuracy better than 3 K. DIAL temperature data is compared to a co-located Raman lidar system and radiosondes to evaluate the system's performance. Finally, an analysis of current performance characteristics is presented, which highlights pathways for future improvement of this proof-of-concept instrument.

Modeling the performance of a diode laser-based (DLB) micro-pulse differential absorption lidar (MPD) for temperature profiling in the lower troposphere.

Ground-based, network-deployable remote sensing instruments for thermodynamic profiling in the lower troposphere are needed by the atmospheric science research community. The recent development of a low-cost diode-laser-based (DLB) micro-pulse differential absorption lidar (DIAL) has begun to address the need for ground-based remote sensing instruments for water vapor profiling in the lower troposphere. Now, taking advantage of the broad spectral coverage of the DLB architecture, an enhancement to the water vapor micro-pulse DIAL (MPD) instrument is proposed to enable atmospheric temperature profiling. The new instrument is based on measuring a temperature-dependent oxygen (O2) absorption coefficient and using this to retrieve the range-resolved temperature profile. In this paper, a retrieval method is proposed based on the recently developed perturbative solution to the DIAL equation that takes into account the Doppler broadening of the molecularly backscattered signal. This perturbative solution relies on an ancillary high spectral resolution lidar (HSRL) measurement of the backscatter ratio. Data from an operational water vapor MPD combined with a DLB-HSRL were used to create an atmosphere model, from which return signals for the O2-MPD were generated. The perturbative retrieval was then applied to these data and a comparison of the retrieved temperature and the model temperature profile allowed the efficacy of retrieval to be evaluated. The results indicate that the temperature profile may be retrieved from a theoretical O2-MPD instrument with a ±1 K accuracy up to 2.5 km and ±3 K accuracy up to 4.5 km with a 150 m range resolution and 30-minute averaging time. Using data from a recently developed O2-MPD in combination with a WV-MPD, and a DLB-HSRL, an initial temperature retrieval is demonstrated. The results of this initial demonstration are consistent with the performance modeling.

Perturbative solution to the two-component atmosphere DIAL equation for improving the accuracy of the retrieved absorption coefficient.

Thermodynamic profiling using ground-based remote sensing instruments such as differential absorption lidar (DIAL) has the potential to fill observational needs for climate and weather-related research and improve weather forecasting. The DIAL technique uses the return signal resulting from atmospherically scattered light at two closely spaced wavelengths to determine the range-resolved absorption coefficient for a molecule of interest. Temperature profiles can be retrieved using a temperature-sensitive absorption feature of a molecule with a known mixing ratio such as oxygen. In order to obtain accuracies of less than 1 K, the narrowband DIAL equation must be expanded to account for Doppler broadening of molecular backscatter, and its relative contribution to the total signal, the backscatter ratio, must be known. While newly developed low-cost high spectral resolution lidar (HSRL) can measure backscatter ratio with sufficient accuracy, the frequency-resolved DIAL equation, even with this information, remains transcendental, and solving it for temperature can be computationally expensive. In this paper, we present a perturbative solution to the frequency-resolved DIAL equation when we have an HSRL providing the required ancillary measurements. This technique leverages perturbative techniques commonly employed in quantum mechanics and has the ability to obtain accurate temperature profiles (better than 1 K) with low computational cost. The perturbative solution is applied to a modeled atmosphere as an initial demonstration of this retrieval technique. An initial estimate of the error in the temperature retrieval for a diode-laser-based O2 DIAL is presented, indicating that temperature retrievals with an error of less than ±1 K can be achieved in the lower troposphere. While this paper focuses on temperature measurements, the perturbative solution to the DIAL equation can also be used to improve the accuracy of retrieved number density profiles.

Hyperspectral detection of a subsurface CO2 leak in the presence of water stressed vegetation.

Remote sensing of vegetation stress has been posed as a possible large area monitoring tool for surface CO2 leakage from geologic carbon sequestration (GCS) sites since vegetation is adversely affected by elevated CO2 levels in soil. However, the extent to which remote sensing could be used for CO2 leak detection depends on the spectral separability of the plant stress signal caused by various factors, including elevated soil CO2 and water stress. This distinction is crucial to determining the seasonality and appropriateness of remote GCS site monitoring. A greenhouse experiment tested the degree to which plants stressed by elevated soil CO2 could be distinguished from plants that were water stressed. A randomized block design assigned Alfalfa plants (Medicago sativa) to one of four possible treatment groups: 1) a CO2 injection group; 2) a water stress group; 3) an interaction group that was subjected to both water stress and CO2 injection; or 4) a group that received adequate water and no CO2 injection. Single date classification trees were developed to identify individual spectral bands that were significant in distinguishing between CO2 and water stress agents, in addition to a random forest classifier that was used to further understand and validate predictive accuracies. Overall peak classification accuracy was 90% (Kappa of 0.87) for the classification tree analysis and 83% (Kappa of 0.77) for the random forest classifier, demonstrating that vegetation stressed from an underground CO2 leak could be accurately discerned from healthy vegetation and areas of co-occurring water stressed vegetation at certain times. Plants appear to hit a stress threshold, however, that would render detection of a CO2 leak unlikely during severe drought conditions. Our findings suggest that early detection of a CO2 leak with an aerial or ground-based hyperspectral imaging system is possible and could be an important GCS monitoring tool.

Micropulse differential absorption lidar for identification of carbon sequestration site leakage.

A scanning differential absorption lidar (DIAL) instrument for identification of carbon dioxide leaks at carbon sequestration sites has been developed and initial data has been collected at Montana State University. The laser transmitter uses two tunable discrete mode laser diodes operating in the continuous-wave mode with one locked to the online absorption wavelength and the other operating at the offline wavelength. Two in-line fiber optic switches are used to switch between online and offline operation. After the fiber optic switch, an acousto-optic modulator is used to generate a pulse train used to injection seed an erbium-doped fiber amplifier to produce eye-safe laser pulses with maximum pulse energies of 66 µJ, a pulse repetition frequency of 15 kHz, and an operating wavelength of 1.571 µm. The DIAL receiver uses a 28 cm diameter Schmidt-Cassegrain telescope to collect that backscattered light, which is then monitored using a photomultiplier tube module operating in the photon counting mode. The DIAL has measured carbon dioxide profiles from 1 to 2.5 km with 60 min temporal averaging. Comparisons of DIAL measurements with a Licor LI-820 gas analyzer point sensor have been made.

Micropulse water vapor differential absorption lidar: transmitter design and performance.

An all diode-laser-based micropulse differential absorption lidar (DIAL) laser transmitter for tropospheric water vapor and aerosol profiling is presented. The micropulse DIAL (MPD) transmitter utilizes two continuous wave (cw) external cavity diode lasers (ECDL) to seed an actively pulsed, overdriven tapered semiconductor optical amplifier (TSOA). The MPD laser produces up to 7 watts of peak power over a 1 µs pulse duration (7 µJ) and a 10 kHz pulse repetition frequency. Spectral switching between the online and offline seed lasers is achieved on a 1Hz basis using a fiber optic switch to allow for more accurate sampling of the atmospheric volume between the online and offline laser shots. The high laser spectral purity of greater than 0.9996 coupled with the broad tunability of the laser transmitter will allow for accurate measurements of tropospheric water vapor in a wide range of geographic locations under varying atmospheric conditions. This paper describes the design and performance characteristics of a third generation MPD laser transmitter with enhanced laser performance over the previous generation DIAL system.

Development of a high spectral resolution lidar based on confocal Fabry-Perot spectral filters.

The high spectral resolution lidar (HSRL) instrument described in this paper utilizes the fundamental and second-harmonic output from an injection seeded Nd:YAG laser as the laser transmitter. The light scattered in the atmosphere is collected using a commercial Schmidt-Cassegrain telescope with the optical receiver train first splitting the fundamental and second-harmonic return signal with the fundament light monitored using an avalanche photodiode. The second-harmonic return signal is mode matched into a tunable confocal Fabry-Perot (CFP) interferometer with a free spectral range of 7.5 GHz and a finesse of 50.7 (312) at 532 nm (1064 nm) placed in the optical receiver for spectrally filtering the molecular and aerosol return signals. The light transmitted through the CFP is used to monitor the aerosol return signal while the light reflected from the CFP is used to monitor the molecular return signal. Data collected with the HSRL are presented and inversion results are compared to a co-located solar radiometer, demonstrating the successful operation of the instrument. The CFP-based filtering technique successfully employed by this HSRL instrument is easily portable to other arbitrary wavelengths, thus allowing for the future development of multiwavelength HSRL instruments.

Field demonstration of a scanning lidar and detection algorithm for spatially mapping honeybees for biological detection of land mines.

A biological detection scheme based on the natural foraging behavior of conditioned honeybees for detecting chemical vapor plumes associated with unexploded ordnance devices utilizes a scanning lidar instrument to provide spatial mapping of honeybee densities. The scanning light detection and ranging (lidar) instrument uses a frequency doubled Nd:YAG microchip laser to send out a series of pulses at a pulse repetition rate of 6.853 kHz. The scattered light is monitored to produce a discrete time series for each range. This discrete time series is then processed using an efficient algorithm that is able to isolate and identify the return signal from a honeybee in a cluttered environment, producing spatially mapped honeybee densities. Two field experiments were performed with the scanning lidar instrument that demonstrate good correlation between the honeybee density maps and the target locations.

Testing carbon sequestration site monitor instruments using a controlled carbon dioxide release facility.

Two laser-based instruments for carbon sequestration site monitoring have been developed and tested at a controlled carbon dioxide (CO(2)) release facility. The first instrument uses a temperature tunable distributed feedback (DFB) diode laser capable of accessing the 2.0027-2.0042 microm spectral region that contains three CO(2) absorption lines and is used for aboveground atmospheric CO(2) concentration measurements. The second instrument also uses a temperature tunable DFB diode laser capable of accessing the 2.0032-2.0055 mum spectral region that contains five CO(2) absorption lines for underground CO(2) soil gas concentration measurements. The performance of these instruments for carbon sequestration site monitoring was studied using a newly developed controlled CO(2) release facility. A 0.3 ton CO(2)/day injection experiment was performed from 3-10 August 2007. The aboveground differential absorption instrument measured an average atmospheric CO(2) concentration of 618 parts per million (ppm) over the CO(2) injection site compared with an average background atmospheric CO(2) concentration of 448 ppm demonstrating this instrument's capability for carbon sequestration site monitoring. The underground differential absorption instrument measured a CO(2) soil gas concentration of 100,000 ppm during the CO(2) injection, a factor of 25 greater than the measured background CO(2) soil gas concentration of 4000 ppm demonstrating this instrument's capability for carbon sequestration site monitoring.

Range-resolved optical detection of honeybees by use of wing-beat modulation of scattered light for locating land mines.

An imaging lidar instrument with the capability of measuring the frequency response of a backscattered return signal up to 3.6 kHz is demonstrated. The instrument uses a commercial microchip frequency-doubled pulsed Nd:YAG laser with a 7.2 kHz pulse repetition rate, a pulse duration of less than 1 ns, and a pulse energy of greater than 10 microJ. A 15.2 cm commercial telescope is used to collect the backscattered signal, and a photomultiplier tube is used to monitor the scattered light. This instrument is designed for range- and angle-resolved optical detection of honeybees for explosives and land-mine detection. The instrument is capable of distinguishing between the scattered light from honeybees and other sources through the frequency content of the return signal caused by the wing-beat modulation of the backscattered light. Detection of honeybees near a bee hive and spatial mapping of honeybee densities near feeders are demonstrated.

Extending the continuous tuning range of an external-cavity diode laser.

The continuous tuning range of an external-cavity diode laser can be extended by making small corrections to the external-cavity length through an electronic feedback loop so that the cavity resonance condition is maintained as the laser wavelength is tuned. By maintaining the cavity resonance condition as the laser is tuned, the mode hops that typically limit the continuous tuning range of the external-cavity diode laser are eliminated. We present the design of a simple external-cavity diode laser based on the Littman-Metcalf external-cavity configuration that has a measured continuous tuning range of 1 GHz without an electronic feedback loop. To include the electronic feedback loop, a small sinusoidal signal is added to the drive current of the laser diode creating a small oscillation of the laser power. By comparing the phase of the modulated optical power with the phase of the sinusoidal drive signal using a lock-in amplifier, an error signal is created and used in an electronic feedback loop to control the external-cavity length. With electronic feedback, we find that the continuous tuning range can be extended to over 65 GHz. This occurs because the electronic feedback maintains the cavity resonance condition as the laser is tuned. An experimental demonstration of this extended tuning range is presented in which the external-cavity diode laser is tuned through an absorption feature of diatomic oxygen near 760 nm.

Optical detection of honeybees by use of wing-beat modulation of scattered laser light for locating explosives and land mines.

An instrument is demonstrated that can be used for optical detection of honeybees in a cluttered environment. The instrument uses a continuous-wave diode laser with a center wavelength of 808 nm and an output power of 28 mW as the laser transmitter source. Light scattered from moving honeybee wings will produce an intensity-modulated signal at a characteristic wing-beat frequency (170-270 Hz) that can be used to detect the honeybees against a cluttered background. The optical detection of honeybees has application in the biological detection of land mines and explosives, as was recently demonstrated.

Normalized differential detection by use of smart pixels with smart illumination.

Smart pixels permit rapid signal processing through the use of integrated photodetectors and processing electronics on a single semiconductor chip. Smart pixels with smart illumination can increase the dynamic range and functionality of smart pixels by employing optoelectronic feedback to control the illumination of a scene. This combination of smart pixels and optoelectronic feedback leads to many potential sensor applications, including normalized differential detection, which is modeled and demonstrated here.