Quantum Plasmonic Nonreciprocity in Parity-Violating Magnets.

The optical responses of metals are often dominated by plasmonic resonances, that is, the collective oscillations of interacting electron liquids. Here we unveil a new class of plasmons─quantum metric plasmons (QMPs)─that arise in a wide range of parity-violating magnetic metals. In these materials, a dipolar distribution of the quantum metric (a fundamental characteristic of Bloch wave functions) produces intrinsic nonreciprocal bulk plasmons. Strikingly, QMP nonreciprocity manifests even when the single-particle dispersion is symmetric: QMPs are sensitive to time-reversal and parity violations hidden in the Bloch wave function. In materials with asymmetric single-particle dispersions, quantum metric dipole induced nonreciprocity can continue to dominate at large frequencies. We anticipate that QMPs can be realized in a wide range of parity-violating magnets, including twisted bilayer graphene heterostructures, where quantum geometric quantities can achieve large values.

Vibronic Exciton-Phonon States in Stack-Engineered van der Waals Heterojunction Photodiodes.

Stack engineering, an atomic-scale metamaterial strategy, enables the design of optical and electronic properties in van der Waals heterostructure devices. Here we reveal the optoelectronic effects of stacking-induced strong coupling between atomic motion and interlayer excitons in WSe2/MoSe2 heterojunction photodiodes. To do so, we introduce the photocurrent spectroscopy of a stack-engineered photodiode as a sensitive technique for probing interlayer excitons, enabling access to vibronic states typically found only in molecule-like systems. The vibronic states in our stack are manifest as a palisade of pronounced periodic sidebands in the photocurrent spectrum in frequency windows close to the interlayer exciton resonances and can be shifted "on demand" through the application of a perpendicular electric field via a source-drain bias voltage. The observation of multiple well-resolved sidebands as well as their ability to be shifted by applied voltages vividly demonstrates the emergence of interlayer exciton vibronic structure in a stack-engineered optoelectronic device.

Electronic Floquet gyro-liquid crystal.

Floquet engineering uses coherent time-periodic drives to realize designer band structures on-demand, thus yielding a versatile approach for inducing a wide range of exotic quantum many-body phenomena. Here we show how this approach can be used to induce non-equilibrium correlated states with spontaneously broken symmetry in lightly doped semiconductors. In the presence of a resonant driving field, the system spontaneously develops quantum liquid crystalline order featuring strong anisotropy whose directionality rotates as a function of time. The phase transition occurs in the steady state of the system achieved due to the interplay between the coherent external drive, electron-electron interactions, and dissipative processes arising from the coupling to phonons and the electromagnetic environment. We obtain the phase diagram of the system using numerical calculations that match predictions obtained from a phenomenological treatment and discuss the conditions on the system and the external drive under which spontaneous symmetry breaking occurs. Our results demonstrate that coherent driving can be used to induce non-equilibrium quantum phases of matter with dynamical broken symmetry.

Floquet metal-to-insulator phase transitions in semiconductor nanowires.

We study steady states of semiconductor nanowires subjected to strong resonant time-periodic drives. The steady states arise from the balance between electron-phonon scattering, electron-hole recombination via photoemission, and Auger scattering processes. We show that tuning the strength of the driving field drives a transition between an electron-hole metal (EHM) phase and a Floquet insulator (FI) phase. We study the critical point controlling this transition. The EHM-to-FI transition can be observed by monitoring the presence of peaks in the density-density response function, which are associated with the Fermi momentum of the EHM phase and are absent in the FI phase. Our results may help guide future studies toward inducing exotic nonequilibrium phases of matter by periodic driving.

Current-Induced Gap Opening in Interacting Topological Insulator Surfaces.

Two-dimensional topological insulators (TIs) host gapless helical edge states that are predicted to support a quantized two-terminal conductance. Quantization is protected by time-reversal symmetry, which forbids elastic backscattering. Paradoxically, the current-carrying state itself breaks the time-reversal symmetry that protects it. Here we show that the combination of electron-electron interactions and momentum-dependent spin polarization in helical edge states gives rise to feedback through which an applied current opens a gap in the edge state dispersion, thereby breaking the protection against elastic backscattering. Current-induced gap opening is manifested via a nonlinear contribution to the system's I-V characteristic, which persists down to zero temperature. We discuss prospects for realizations in recently discovered large bulk band gap TIs, and an analogous current-induced gap opening mechanism for the surface states of three-dimensional TIs.

Fractional Quantum Hall Effect at ν=2+6/13: The Parton Paradigm for the Second Landau Level.

The unexpected appearance of a fractional quantum Hall effect (FQHE) plateau at ν=2+6/13 [A. Kumar et al., Phys. Rev. Lett. 105, 246808 (2010)PRLTAO0031-900710.1103/PhysRevLett.105.246808] offers a clue into the physical mechanism of the FQHE in the second Landau level (SLL). Here we propose a "3[over ¯]2[over ¯]111" parton wave function, which is topologically distinct from the 6/13 state in the lowest Landau level. We demonstrate the 3[over ¯]2[over ¯]111 state to be a good candidate for the ν=2+6/13 FQHE, and make predictions for experimentally measurable properties that can reveal the nature of this state. Furthermore, we propose that the "n[over ¯]2[over ¯]111" family of parton states naturally describes many observed SLL FQHE plateaus.

Many-Body Dynamics and Gap Opening in Interacting Periodically Driven Systems.

We study transient dynamics in a two-dimensional system of interacting Dirac fermions subject to a quenched drive with circularly polarized light. In the absence of interactions, the drive opens a gap at the Dirac point in the quasienergy spectrum, inducing nontrivial band topology. We investigate the dynamics of this gap opening process, taking into account the essential role of electron-electron interactions. Crucially, scattering due to interactions (1) induces dephasing, which erases memory of the system's prequench state and yields the intrinsic timescale for gap emergence, and (2) provides a mechanism for the system to absorb energy of the drive, leading to heating which must be mitigated to ensure the success of Floquet band engineering. We characterize the gap opening process via the system's generalized spectral function and correlators probed by photoemission experiments, and we identify a parameter regime at moderate driving frequencies where a hierarchy of timescales allows a well-defined Floquet gap to be produced and studied before the deleterious effects of heating set in.

Quantized Magnetization Density in Periodically Driven Systems.

We study micromotion in two-dimensional periodically driven systems in which all bulk Floquet eigenstates are localized by disorder. We show that this micromotion gives rise to a quantized time-averaged orbital magnetization density in any region completely filled with fermions. The quantization of magnetization density has a topological origin, and reveals the physical nature of the new phase identified in P. Titum, E. Berg, M. S. Rudner, G. Refael, and N. H. Lindner [Phys. Rev. X 6, 021013 (2016)PRXHAE2160-330810.1103/PhysRevX.6.021013]. We thus establish that the topological index of this phase can be accessed directly in bulk measurements, and propose an experimental protocol to do so using interferometry in cold-atom-based realizations.

Spectrum of the Nuclear Environment for GaAs Spin Qubits.

Using a singlet-triplet spin qubit as a sensitive spectrometer of the GaAs nuclear spin bath, we demonstrate that the spectrum of Overhauser noise agrees with a classical spin diffusion model over 6 orders of magnitude in frequency, from 1 mHz to 1 kHz, is flat below 10 mHz, and falls as 1/f^{2} for frequency f≳1 Hz. Increasing the applied magnetic field from 0.1 to 0.75 T suppresses electron-mediated spin diffusion, which decreases the spectral content in the 1/f^{2} region and lowers the saturation frequency, each by an order of magnitude, consistent with a numerical model. Spectral content at megahertz frequencies is accessed using dynamical decoupling, which shows a crossover from the few-pulse regime (≲16π pulses), where transverse Overhauser fluctuations dominate dephasing, to the many-pulse regime (≳32 π pulses), where longitudinal Overhauser fluctuations with a 1/f spectrum dominate.

Notch filtering the nuclear environment of a spin qubit.

Electron spins in gate-defined quantum dots provide a promising platform for quantum computation. In particular, spin-based quantum computing in gallium arsenide takes advantage of the high quality of semiconducting materials, reliability in fabricating arrays of quantum dots and accurate qubit operations. However, the effective magnetic noise arising from the hyperfine interaction with uncontrolled nuclear spins in the host lattice constitutes a major source of decoherence. Low-frequency nuclear noise, responsible for fast (10 ns) inhomogeneous dephasing, can be removed by echo techniques. High-frequency nuclear noise, recently studied via echo revivals, occurs in narrow-frequency bands related to differences in Larmor precession of the three isotopes 69Ga, 71Ga and 75As (refs 15,16,17). Here, we show that both low- and high-frequency nuclear noise can be filtered by appropriate dynamical decoupling sequences, resulting in a substantial enhancement of spin qubit coherence times. Using nuclear notch filtering, we demonstrate a spin coherence time (T2) of 0.87 ms, five orders of magnitude longer than typical exchange gate times, and exceeding the longest coherence times reported to date in Si/SiGe gate-defined quantum dots.

Composite Topological Excitations in Ferromagnet-Superconductor Heterostructures.

We investigate the formation of a new type of composite topological excitation-the Skyrmion-vortex pair (SVP)-in hybrid systems consisting of coupled ferromagnetic and superconducting layers. Spin-orbit interaction in the superconductor mediates a magnetoelectric coupling between the vortex and the Skyrmion, with a sign (attractive or repulsive) that depends on the topological indices of the constituents. We determine the conditions under which a bound SVP is formed and characterize the range and depth of the effective binding potential through analytical estimates and numerical simulations. Furthermore, we develop a semiclassical description of the coupled Skyrmion-vortex dynamics and discuss how SVPs can be controlled by applied spin currents.

Chiral plasmons without magnetic field.

Plasmons, the collective oscillations of interacting electrons, possess emergent properties that dramatically alter the optical response of metals. We predict the existence of a new class of plasmons-chiral Berry plasmons (CBPs)-for a wide range of 2D metallic systems including gapped Dirac materials. As we show, in these materials the interplay between Berry curvature and electron-electron interactions yields chiral plasmonic modes at zero magnetic field. The CBP modes are confined to system boundaries, even in the absence of topological edge states, with chirality manifested in split energy dispersions for oppositely directed plasmon waves. We unveil a rich CBP phenomenology and propose setups for realizing them, including in anomalous Hall metals and optically pumped 2D Dirac materials. Realization of CBPs will offer a powerful paradigm for magnetic field-free, subwavelength optical nonreciprocity, in the mid-IR to terahertz range, with tunable splittings as large as tens of THz, as well as sensitive all-optical diagnostics of topological bands.

Nonlocal Polarization Feedback in a Fractional Quantum Hall Ferromagnet.

In a quantum Hall ferromagnet, the spin polarization of the two-dimensional electron system can be dynamically transferred to nuclear spins in its vicinity through the hyperfine interaction. The resulting nuclear field typically acts back locally, modifying the local electronic Zeeman energy. Here we report a nonlocal effect arising from the interplay between nuclear polarization and the spatial structure of electronic domains in a ν=2/3 fractional quantum Hall state. In our experiments, we use a quantum point contact to locally control and probe the domain structure of different spin configurations emerging at the spin phase transition. Feedback between nuclear and electronic degrees of freedom gives rise to memristive behavior, where electronic transport through the quantum point contact depends on the history of current flow. We propose a model for this effect which suggests a novel route to studying edge states in fractional quantum Hall systems and may account for so-far unexplained oscillatory electronic-transport features observed in previous studies.

Observation of a Topological Transition in the Bulk of a Non-Hermitian System.

We present the first experimental observation of a topological transition in a non-Hermitian system. In contrast to standard methods for examining topological properties, which involve probing edge (or surface) states, we monitor the topological transition by employing bulk dynamics only. The system is composed of a lattice of evanescently coupled optical waveguides, and non-Hermitian behavior is engineered by inducing bending loss by spatially "wiggling" every second waveguide.

Spin-Lattice Order in One-Dimensional Conductors: Beyond the RKKY Effect.

We investigate magnetic order in a lattice of classical spins coupled to an isotropic gas of one-dimensional conduction electrons via local exchange interactions. The frequently discussed Ruderman-Kittel-Kasuya-Yosida effective exchange model for this system predicts that spiral order is always preferred. Here we consider the problem nonperturbatively, and find that such order vanishes above a critical value of the exchange coupling that depends strongly on the lattice spacing. The critical coupling tends to zero as the lattice spacing becomes commensurate with the Fermi wave vector, signaling the breakdown of the perturbative Ruderman-Kittel-Kasuya-Yosida picture, and spiral order, even at weak coupling. We provide the exact phase diagram for arbitrary exchange coupling and lattice spacing, and discuss its stability. Our results shed new light on the problem of utilizing a spiral spin-lattice state to drive a one-dimensional superconductor into a topological phase.

Multilevel interference resonances in strongly driven three-level systems.

We study multiphoton resonances in a strongly driven three-level quantum system, where one level is periodically swept through a pair of levels with constant energy separation E. Near the multiphoton resonance condition nℏω=E, where n is an integer, we find qualitatively different behavior for n even or odd. We explain this phenomenon in terms of families of interfering trajectories of the multilevel system. Remarkably, the behavior is insensitive to fluctuations of the energy of the driven level, and survives deep into the strong dephasing regime. The setup can be relevant for a variety of solid state and atomic or molecular systems. In particular, it provides a clear mechanism to explain recent puzzling experimental observations in strongly driven double quantum dots.

Observation of topologically protected bound states in photonic quantum walks.

Topological phases exhibit some of the most striking phenomena in modern physics. Much of the rich behaviour of quantum Hall systems, topological insulators, and topological superconductors can be traced to the existence of robust bound states at interfaces between different topological phases. This robustness has applications in metrology and holds promise for future uses in quantum computing. Engineered quantum systems--notably in photonics, where wavefunctions can be observed directly--provide versatile platforms for creating and probing a variety of topological phases. Here we use photonic quantum walks to observe bound states between systems with different bulk topological properties and demonstrate their robustness to perturbations--a signature of topological protection. Although such bound states are usually discussed for static (time-independent) systems, here we demonstrate their existence in an explicitly time-dependent situation. Moreover, we discover a new phenomenon: a topologically protected pair of bound states unique to periodically driven systems.

Hot carrier transport and photocurrent response in graphene.

Strong electron-electron interactions in graphene are expected to result in multiple-excitation generation by the absorption of a single photon. We show that the impact of carrier multiplication on photocurrent response is enhanced by very inefficient electron cooling, resulting in an abundance of hot carriers. The hot-carrier-mediated energy transport dominates the photoresponse and manifests itself in quantum efficiencies that can exceed unity, as well as in a characteristic dependence of the photocurrent on gate voltages. The pattern of multiple photocurrent sign changes as a function of gate voltage provides a fingerprint of hot-carrier-dominated transport and carrier multiplication.

Gate-activated photoresponse in a graphene p-n junction.

We study photodetection in graphene near a local electrostatic gate, which enables active control of the potential landscape and carrier polarity. We find that a strong photoresponse only appears when and where a p-n junction is formed, allowing on-off control of photodetection. Photocurrents generated near p-n junctions do not require biasing and can be realized using submicrometer gates. Locally modulated photoresponse enables a new range of applications for graphene-based photodetectors including, for example, pixilated infrared imaging with control of response on subwavelength dimensions.

Klein backscattering and Fabry-Pérot interference in graphene heterojunctions.

We present a theory of quantum-coherent transport through a lateral p-n-p structure in graphene, which fully accounts for the interference of forward and backward scattering on the p-n interfaces. The backreflection amplitude changes sign at zero incidence angle because of the Klein phenomenon, adding a phase pi to the interference fringes. The contributions of the two p-n interfaces to the phase of the interference cancel with each other at zero magnetic field, but become imbalanced at a finite field. The resulting half-period shift in the Fabry-Pérot fringe pattern, induced by a relatively weak magnetic field, can provide a clear signature of Klein scattering in graphene. This effect is shown to be robust in the presence of spatially inhomogeneous potential of moderate strength.