Fractal dynamics in a single crystal of a relaxor ferroelectric.

We report the high-resolution and broadband light-scattering spectroscopy of a single crystal of a prototypical relaxor ferroelectric, Pb(Mg(1/3)Nb(2/3))O(3). A self-similar broad central peak, whose intensity is expressed as I(ω) [Symbol: see text] ω(α) has been observed, indicating the presence of a fractal in the crystal. A strong correspondence exists between the temperature dependence of the exponent α and that of the reported behaviors of polar nanoregions. The estimated fractal dimension (d(f) ≈ 2.6) at low temperatures clearly indicates a percolation transition of the polar nanoregions at around 240 K.

Note: Higher resolution Brillouin spectroscopy by offset stabilization of a tandem Fabry-Pérot interferometer.

A simple modification to a Sandercock-type tandem Fabry-Pérot interferometer is demonstrated. By adding an independent reference laser with temperature tunability, narrow Brillouin lines that are tens GHz shifted from the Rayleigh line can be recorded with much higher frequency resolution than in the original system.

Second sound in SrTiO3.

We study collective phonon excitations in SrTiO3 by low-frequency light scattering. We employ extended thermodynamics for phonon gas to construct a theoretical spectral function that is applicable regardless of local thermal equilibrium. Our analysis reveals the temperature dependence of tauN, the relaxation time for the momentum-conserving phonon collisions (normal processes), in SrTiO3. These results indicate that the previously reported anomalous soundlike spectrum originates from second sound, which is a wavelike propagation of heat.

Measurement of polarization dependence of nonlinear susceptibility responsible for Rayleigh-wing and Brillouin scattering.

By using a simple optical geometry based on backward light scattering and employing a Sandercock-type tandem Fabry-Perot interferometer, we measure both the linear and the circular polarization dependences of Rayleigh-wing and Brillouin scattering in a sample of liquid-crystal 4-n-pentyl-4'-cyanobiphenyl. Observed polarization dependences are consistent with the third-order nonlinear susceptibilities, taking into account the traceless symmetric scattering tensor for Rayleigh-wing scattering and the isotropic scattering tensor for Brillouin scattering.