A quantum ruler for orbital magnetism in moiré quantum matter.

For almost a century, magnetic oscillations have been a powerful "quantum ruler" for measuring Fermi surface topology. In this study, we used Landau-level spectroscopy to unravel the energy-resolved valley-contrasting orbital magnetism and large orbital magnetic susceptibility that contribute to the energies of Landau levels of twisted double-bilayer graphene. These orbital magnetism effects led to substantial deviations from the standard Onsager relation, which manifested as a breakdown in scaling of Landau-level orbits. These substantial magnetic responses emerged from the nontrivial quantum geometry of the electronic structure and the large length scale of the moiré lattice potential. Going beyond traditional measurements, Landau-level spectroscopy performed with a scanning tunneling microscope offers a complete quantum ruler that resolves the full energy dependence of orbital magnetic properties in moiré quantum matter.

Robust zero-energy modes in an electronic higher-order topological insulator.

Quantum simulators are essential tools for understanding complex quantum materials. Platforms based on ultracold atoms in optical lattices and photonic devices have led the field so far, but the basis for electronic quantum simulators is now being developed. Here, we experimentally realize an electronic higher-order topological insulator (HOTI). We create a breathing kagome lattice by manipulating carbon monoxide molecules on a Cu(111) surface using a scanning tunnelling microscope. We engineer alternating weak and strong bonds to show that a topological state emerges at the corner of the non-trivial configuration, but is absent in the trivial one. Different from conventional topological insulators, the topological state has two dimensions less than the bulk, denoting a HOTI. The corner mode is protected by a generalized chiral symmetry, which leads to a particular robustness against perturbations. Our versatile approach to designing artificial lattices holds promise for revealing unexpected quantum phases of matter.

Design and characterization of electrons in a fractal geometry.

The dimensionality of an electronic quantum system is decisive for its properties. In one dimension electrons form a Luttinger liquid and in two dimensions they exhibit the quantum Hall effect. However, very little is known about the behavior of electrons in non-integer, or fractional dimensions1. Here, we show how arrays of artificial atoms can be defined by controlled positioning of CO molecules on a Cu (111) surface2-4, and how these sites couple to form electronic Sierpinski fractals. We characterize the electron wave functions at different energies with scanning tunneling microscopy and spectroscopy and show that they inherit the fractional dimension. Wave functions delocalized over the Sierpinski structure decompose into self-similar parts at higher energy, and this scale invariance can also be retrieved in reciprocal space. Our results show that electronic quantum fractals can be artificially created by atomic manipulation in a scanning tunneling microscope. The same methodology will allow future study to address fundamental questions about the effects of spin-orbit interaction and a magnetic field on electrons in non-integer dimensions. Moreover, the rational concept of artificial atoms can readily be transferred to planar semiconductor electronics, allowing for the exploration of electrons in a well-defined fractal geometry, including interactions and external fields.