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1.
Adv Sci (Weinh) ; 11(32): e2402263, 2024 Aug.
Article in English | MEDLINE | ID: mdl-38924658

ABSTRACT

This work describes light-driven assembly of dynamic formations and functional particle swarms controlled by appropriately programmed light patterns. The system capitalizes on the use of a fluidic bed whose low thermal conductivity assures that light-generated heat remains "localized" and sets strong convective flows in the immediate vicinity of the particles being irradiated. In this way, even low-power laser light or light from a desktop slide projector can be used to organize dynamic formations of objects spanning four orders of magnitude in size (from microns to centimeters) and over nine orders of magnitude in terms of mass. These dynamic assemblies include open-lattice structures with individual particles performing intricate translational and/or rotational motions, density-gradient particle arrays, nested architectures of mechanical components (e.g., planetary gears), or swarms of light-actuated microbots controlling assembly of other objects.

2.
Soft Matter ; 17(38): 8595-8604, 2021 Oct 06.
Article in English | MEDLINE | ID: mdl-34528041

ABSTRACT

This work describes granular crystals held together by unusual, multipolar interactions and, under the application of an external bias, undergoing reversible structural transitions between closed and open forms. The system comprises two types of polymeric beads agitated on one or between two conductive plates and gradually acquiring charges by contact electrification. The charges thus developed induce a series of electrostatic images in the conductive supports and, in effect, the beads interact via dipolar or multipolar interactions, enabling the stabilization of non-electroneutral crystals. Furthermore, under an applied bias, the beads become polarized and their complex interactions (due to the series of image charges as well as series of image dipoles) result in open-pore crystals which return to compact forms upon bias removal. These effects are rationalized by analytical calculations, and the crystal structures observed in the experiments are reproduced by molecular dynamics simulations.

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