Variability of ambient black carbon concentration in the Central Himalaya and its assessment over the Hindu Kush Himalayan region.

During 2015-2018, eight black carbon (BC) monitoring sites were established in Nepal and Bhutan to fill a significant data gap regarding BC measurement in Central Himalaya. This manuscript analyzes and presents data from these eight stations and one additional station on the Tibetan plateau (TP). Complex topography, varied emission sources, and atmospheric transport pathways significantly impacted the BC concentrations across these stations, with annual mean concentrations varying from 36 ng m-3 to 45,737 ng m-3. Higher annual mean concentrations (5609 ± 4515 ng m-3) were recorded at low-altitude sites than in other locations, with seasonal concentrations highest in the winter (7316 ± 2541 ng m-3). In contrast, the annual mean concentrations were lowest at high-altitude sites (376 ± 448 ng m-3); the BC concentrations at these sites peaked during the pre-monsoon season (930 ± 685 ng m-3). Potential source contributions to the total observed BC were analyzed using the absorption angstrom exponent (AAE). AAE analysis showed the dominance of biomass burning sources (>50 %), except in Kathmandu. By combining our data with previously published literature, we put our measurements in perspective by presenting a comprehensive assessment of BC concentrations and their variability over the Hindu Kush Himalayan (HKH) region. The BC levels in all three geographic regions, high, mid, and low altitude significantly influenced by the persistent seasonal meteorology. However, the mid-altitude stations were substantially affected by valley dynamics and urbanization. The low-altitude stations experienced high BC concentrations during the winter and post-monsoon seasons. Concentration weighted trajectory (CWT) and frequency analyses revealed the dominance of long-range transported pollution during winter over HKH, from west to east. South Asian sources remained significant during the monsoon season. During pre- and post-monsoon, the local, regional, and long-distance pollution varied depending on the location of the receptor site.

Asian aerosols: current and year 2030 distributions and implications to human health and regional climate change.

Aerosol distributions in Asia calculated over a 4-year period and constrained by satellite observations of aerosol optical depth (AOD) are presented. Vast regions in Asia that include > 80% of the population have PM2.5 concentrations that exceed on an annual basis the WHO guideline of 10 microg/m3, often by factors of 2 to 4. These high aerosol loadings also have important radiative effects, causing a significant dimming at the surface, and mask approximately 45% of the warming by greenhouse gases. Black carbon (BC) concentrations are high throughout Asia, representing 5-10% of the total AOD, and contributing significantly to atmospheric warming (its warming potential is approximately 55% of that due to CO2). PM levels and AODs in year 2030, estimated based on simulations that consider future changes in emissions, are used to explore opportunities for win-win strategies built upon addressing air quality and climate change together. It is found that in 2030 the PM2.5 levels in significant parts of Asia will increase and exacerbate health impacts; but the aerosols will have a larger masking effect on radiative forcing, due to a decrease in BC and an increase in SO2 emissions.