Spectral splitting in phase mismatched harmonics.

Spectral splitting of high harmonic radiation is observed when a gas target is irradiated with a high-energy laser pulse, having an extreme amount of frequency chirp. The phenomenon, which may be observed only by using a multi-TW laser system, originates from the temporal evolution of the phase-matching conditions. We illustrate how these conditions are mapped to the spectral domain, and present experimental evidence which is validated by our model.

Simple algorithm for the design of accelerating Bessel-like beams with adjustable features along their propagation.

We present an extremely simple method for designing self-accelerating non-diffracting beams having arbitrary trajectories while their intensity, width and orbital angular momentum are modulated in a prescribed way along their propagation. Different beams constructed with this method are demonstrated experimentally in the paraxial regime and numerically in the non-paraxial regime.

Multiscale dynamical symmetries and selection rules in nonlinear optics.

Symmetries and their associated selection rules are extremely useful in many fields of science. For systems of electromagnetic (EM) fields interacting with matter, the symmetries of matter and the EM fields' time-dependent polarization determine the properties of the nonlinear responses, and they can be facilitated for controlling light emission and enabling ultrafast symmetry breaking spectroscopy of various properties. Here, we formulate a general theory that describes the macroscopic and microscopic dynamical symmetries (including quasicrystal-like symmetries) of EM vector fields, revealing many previously unidentified symmetries and selection rules in light-matter interactions. We demonstrate an example of multiscale selection rules experimentally in the framework of high harmonic generation. This work paves the way for novel spectroscopic techniques in multiscale systems and for imprinting complex structures in extreme ultraviolet-x-ray beams, attosecond pulses, or the interacting medium itself.

Toward multimode-fiber shape sensing.

We demonstrate machine-learning assisted dynamic tracking of the shape of a multimode fiber whose spatial configuration is manipulated by the movement of three linear stages. The data source used for the analysis is the coherent speckle pattern of light that has made a round trip in the fiber.

Visual data detection through side-scattering in a multimode optical fiber.

Light propagation in optical fibers is accompanied by random omnidirectional scattering. The small fraction of coherent guided light that escapes outside the cladding of the fiber forms a speckle pattern. Here, visual information imaged into the input facet of a multimode fiber with a transparent buffer is retrieved, using a convolutional neural network, from the side-scattered light at several locations along the fiber. This demonstration can promote the development of distributed optical imaging systems and optical links interfaced via the sides of the fiber.

Light beams with volume superoscillations.

Using a superposition of shifted Bessel beams with different longitudinal wave vectors and orbital angular momenta, we realize an optical beam having simultaneous axial, angular, and radial focusing narrower than the Fourier limit. Our findings can be useful for optical particle manipulation and high-resolution microscopy.

Beam profiler network (BPNet): a deep learning approach to mode demultiplexing of Laguerre-Gaussian optical beams.

The transverse field profile of light has been recognized as a resource for classical and quantum communications for which reliable methods of sorting or demultiplexing spatial optical modes are required. Here we experimentally demonstrate state-of-the-art mode demultiplexing of Laguerre-Gaussian beams according to both their orbital angular momentum and radial topological numbers using a flow of two concatenated deep neural networks. The first network serves as a transfer function from experimentally generated to ideal numerically generated data, while using a unique "histogram weighted loss" function that solves the problem of images with limited significant information. The second network acts as a spatial-modes classifier. Our method uses only the intensity profile of modes or their superposition, making the phase information redundant.

On-the-Fly Control of High-Harmonic Generation Using a Structured Pump Beam.

We demonstrate experimentally a relatively simple yet powerful all-optical enhancement and control technique for high harmonic generation. This is achieved by using as a pump beam two different spatial optical modes interfering together to realize tunable periodic quasi-phase matching of the interaction. With this technique, we demonstrate on-the-fly quasi-phase matching of harmonic orders 29-41 at ambient gas pressure levels of 50 and 100 Torr, where an up to 100-fold enhancement of the emission is observed. The technique is scalable to different harmonic orders and ambient pressure conditions.

Experimental realization of structured super-oscillatory pulses.

We demonstrate experimentally a generic method for the synthesis of optical femtosecond pulses based on Gaussian, Airy and Hermite-Gauss functions, which are transformed to exhibit fringes with tunable width. The width of the fringes is set in some cases to be much narrower than the inverse of the spectral bandwidth. Such pulses might be useful for ultrafast spectroscopy, coherent control and nonlinear optics.

Axial sub-Fourier focusing of an optical beam.

We demonstrate experimentally the generation of an optical beam having an axial focusing that is narrower than the Fourier limit. The beam is constructed from a superposition of Bessel beams with different longitudinal wave vectors, realizing a super-oscillatory axial intensity distribution. Such beams can be useful for microscopy and for optical particle manipulation.

Breaking the Temporal Resolution Limit by Superoscillating Optical Beats.

Band-limited functions can oscillate locally at an arbitrarily fast rate through an interference phenomenon known as superoscillations. Using an optical pulse with a superoscillatory envelope we experimentally break the temporal Fourier-transform focusing limit with a temporal feature that is approximately three times shorter than the duration of a transform-limited Gaussian pulse having a comparable bandwidth while maintaining 30% visibility. We experimentally demonstrate the ability of such signals to achieve temporal superresolution and show numerically in which cases such pulses can outperform transform-limited pulses.

Double Fano resonance in a plasmonic double grating structure.

It is shown theoretically and numerically that a simple gratings-based plasmonic structure can support a nearly-degenerate double Fano resonance which can lead to a relatively narrow spectral line shape. The double-resonance spectral location and line-shape are controllable by either adjusting the periodicity and unit-cell of the gratings or by adjusting the angle of incidence of the incoming radiation.

Periodic density modulation for quasi-phase-matching of optical frequency conversion is inefficient under shallow focusing and constant ambient pressure.

The two main mechanisms of a periodic density modulation relevant to nonlinear optical conversion in a gas medium are spatial modulations of the index of refraction and of the number of emitters. For a one-dimensional model neglecting focusing and using a constant ambient pressure, it is shown theoretically and demonstrated numerically that the effects of these two mechanisms during frequency conversion cancel each other exactly. Under the considered conditions, this makes density modulation inefficient for quasi-phase-matching an optical frequency conversion process. This result is particularly relevant for high-order harmonic generation.

Breathing solitary-pulse pairs in a linearly coupled system.

It is shown that pairs of solitary pulses (SPs) in a linearly coupled system with opposite group velocity dispersions form robust breathing bound states. The system can be realized by temporal-modulation coupling of SPs with different carrier frequencies propagating in the same medium, or by coupling of SPs in a dual-core waveguide. Broad SP pairs are produced in a virtually exact form by means of the variational approximation. Strong nonlinearity tends to destroy the periodic evolution of the SP pairs.

Super-transmission: the delivery of superoscillations through the absorbing resonance of a dielectric medium.

The delivery of a super-oscillatory optical signal through a medium with an absorbing resonance at the super-oscillation frequency is considered theoretically and through simulations. While a regular signal oscillating at the absorption resonance frequency would be completely absorbed after a few absorption lengths, it is found that the superoscillation undergoes quasi-periodic revivals over optically thick distances. In particular revivals of extreme UV local oscillations propagating through Silica Glass over distances which are three orders of magnitude longer than the associated absorbing length are numerically demonstrated.

Macroscopic manipulation of high-order-harmonic generation through bound-state coherent control.

We propose a paradigm for macroscopic control of high-order harmonic generation by modulating the bound-state population of the medium atoms. A unique result of this scheme is that apart from regular spatial quasi-phase-matching (QPM), also purely temporal QPM of the emitted radiation can be established. Our simulations demonstrate temporal QPM by inducing homogenous Rabi oscillations in the medium and also spatial QPM by creating a grating of population inversion using the process of rapid adiabatic passage. In the simulations a scaled version of high-order harmonic generation is used: a far off-resonance 2.6 µm source generates UV-visible high-order harmonics from alkali-metal-atom vapor, while a resonant near IR source is used to coherently control the medium.

Sawtooth grating-assisted phase-matching.

We show that a sawtooth phase-modulation is the optimal profile for grating assisted phase matching (GAPM). Perfect (sharp) sawtooth modulation fully corrects the phase-mismatch, exhibiting conversion equal to conventional phase matching, while smoothened, approximate sawtooth structures are more efficient than sinusoidal or square GAPM modulations that were previously studied. As an example, we demonstrate numerically optically-induced sawtooth GAPM for high harmonic generation. Sawtooth GAPM is the most efficient method for increasing the conversion efficiency of high harmonic generation through quasi-phase-matching, with an ultimate efficiency that closely matches the ideal phase-matching case.

Quasi-phase-matched concurrent nonlinearities in periodically poled KTiOPO(4) for quantum computing over the optical frequency comb.

We report the successful design and experimental implementation of three coincident nonlinear interactions, namely ZZZ (type 0), ZYY (type I), and YYZ/YZY (type II) second-harmonic generation of 780 nm light from a 1560 nm pump beam in a single, multigrating, periodically poled KTiOPO(4) crystal. The resulting nonlinear medium is the key component for making a scalable quantum computer over the optical frequency comb of a single optical parametric oscillator.

Phase matching of high harmonic generation in the soft and hard X-ray regions of the spectrum.

We show how bright, tabletop, fully coherent hard X-ray beams can be generated through nonlinear upconversion of femtosecond laser light. By driving the high-order harmonic generation process using longer-wavelength midinfrared light, we show that, in theory, fully phase-matched frequency upconversion can extend into the hard X-ray region of the spectrum. We verify our scaling predictions experimentally by demonstrating phase matching in the soft X-ray region of the spectrum around 330 eV, using ultrafast driving laser pulses at 1.3-microm wavelength, in an extended, high-pressure, weakly ionized gas medium. We also show through calculations that scaling of the overall conversion efficiency is surprisingly favorable as the wavelength of the driving laser is increased, making tabletop, fully coherent, multi-keV X-ray sources feasible. The rapidly decreasing microscopic single-atom yield, predicted for harmonics driven by longer-wavelength lasers, is compensated macroscopically by an increased optimal pressure for phase matching and a rapidly decreasing reabsorption of the generated X-rays.

Quasi-phase-matching and dispersion characterization of harmonic generation in the perturbative regime using counterpropagating beams.

It is shown theoretically that second harmonic generation can be quasi-phase-matched by using a pump beam consisting of a forward propagating field and a counterpropagating pulse train. The counterpropagating setup can also be used for direct measurement of the coherence length of the nonlinear process which can determine the dispersion properties of the medium.