Quantum-well states at the surface of a heavy-fermion superconductor.

Two-dimensional electronic states at surfaces are often observed in simple wide-band metals such as Cu or Ag (refs. 1-4). Confinement by closed geometries at the nanometre scale, such as surface terraces, leads to quantized energy levels formed from the surface band, in stark contrast to the continuous energy dependence of bulk electron bands2,5-10. Their energy-level separation is typically hundreds of meV (refs. 3,6,11). In a distinct class of materials, strong electronic correlations lead to so-called heavy fermions with a strongly reduced bandwidth and exotic bulk ground states12,13. Quantum-well states in two-dimensional heavy fermions (2DHFs) remain, however, notoriously difficult to observe because of their tiny energy separation. Here we use millikelvin scanning tunnelling microscopy (STM) to study atomically flat terraces on U-terminated surfaces of the heavy-fermion superconductor URu2Si2, which exhibits a mysterious hidden-order (HO) state below 17.5 K (ref. 14). We observe 2DHFs made of 5f electrons with an effective mass 17 times the free electron mass. The 2DHFs form quantized states separated by a fraction of a meV and their level width is set by the interaction with correlated bulk states. Edge states on steps between terraces appear along one of the two in-plane directions, suggesting electronic symmetry breaking at the surface. Our results propose a new route to realize quantum-well states in strongly correlated quantum materials and to explore how these connect to the electronic environment.

Interior and Edge Magnetization in Thin Exfoliated CrGeTe3 Films.

CrGeTe3 (CGT) is a semiconducting vdW ferromagnet shown to possess magnetism down to a two-layer thick sample. Although CGT is one of the leading candidates for spintronics devices, a comprehensive analysis of CGT thickness dependent magnetization is currently lacking. In this work, we employ scanning SQUID-on-tip (SOT) microscopy to resolve the magnetic properties of exfoliated CGT flakes at 4.2 K. Combining transport measurements of CGT/NbSe2 samples with SOT images, we present the magnetic texture and hysteretic magnetism of CGT, thereby matching the global behavior of CGT to the domain structure extracted from local SOT magnetic imaging. Using this method, we provide a thickness dependent magnetization state diagram of bare CGT films. No zero-field magnetic memory was found for films thicker than 10 nm, and hard ferromagnetism was found below that critical thickness. Using scanning SOT microscopy, we identify a unique edge magnetism, contrasting the results attained in the CGT interior.

Simplified feedback control system for scanning tunneling microscopy.

A Scanning Tunneling Microscope (STM) is one of the most important scanning probe tools available to study and manipulate matter at the nanoscale. In a STM, a tip is scanned on top of a surface with a separation of a few Å. Often, the tunneling current between the tip and the sample is maintained constant by modifying the distance between the tip apex and the surface through a feedback mechanism acting on a piezoelectric transducer. This produces very detailed images of the electronic properties of the surface. The feedback mechanism is nearly always made using a digital processing circuit separate from the user computer. Here, we discuss another approach using a computer and data acquisition through the universal serial bus port. We find that it allows successful ultralow noise studies of surfaces at cryogenic temperatures. We show results on different compounds including a type II Weyl semimetal (WTe2), a quasi-two-dimensional dichalcogenide superconductor (2H-NbSe2), a magnetic Weyl semimetal (Co3Sn2S2), and an iron pnictide superconductor (FeSe).

Coherent coupling between vortex bound states and magnetic impurities in 2D layered superconductors.

Bound states in superconductors are expected to exhibit a spatially resolved electron-hole asymmetry which is the hallmark of their quantum nature. This asymmetry manifests as oscillations at the Fermi wavelength, which is usually tiny and thus washed out by thermal broadening or by scattering at defects. Here we demonstrate theoretically and confirm experimentally that, when coupled to magnetic impurities, bound states in a vortex core exhibit an emergent axial electron-hole asymmetry on a much longer scale, set by the coherence length. We study vortices in 2H-NbSe2 and in 2H-NbSe1.8S0.2 with magnetic impurities, characterizing these with detailed Hubbard-corrected density functional calculations. We find that the induced electron-hole imbalance depends on the band character of the superconducting material. Our results show that coupling between quantum bound states in superconductors is remarkably robust and has a strong influence in tunneling measurements.

Large magnetoresistance in the iron-free pnictide superconductor LaRu2P2.

The magnetoresistance (MR) of iron pnictide superconductors is often dominated by electron-electron correlations and deviates from theH2or saturating behaviors expected for uncorrelated metals. Contrary to similar Fe-based pnictide systems, the superconductor LaRu2P2(Tc= 4 K) shows no enhancement of electron-electron correlations. Here we report a non-saturating MR deviating from theH2or saturating behaviors in LaRu2P2. We present results in single crystals of LaRu2P2, where we observe a MR followingH1.3up to 22 T. We discuss our result by comparing the bandstructure of LaRu2P2with that of Fe based pnictide superconductors. The different orbital structures of Fe and Ru leads to a 3D Fermi surface with negligible bandwidth renormalization in LaRu2P2, that contains a large open sheet over the whole Brillouin zone. We show that the large MR in LaRu2P2is unrelated to the one obtained in materials with strong electron-electron correlations and that it is compatible instead with conduction due to open orbits on the rather complex Fermi surface structure of LaRu2P2.