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1.
J Geophys Res Atmos ; 121(12): 7254-7283, 2016 Jun 27.
Article in English | MEDLINE | ID: mdl-32818126

ABSTRACT

The ability of 11 models in simulating the aerosol vertical distribution from regional to global scales, as part of the second phase of the AeroCom model intercomparison initiative (AeroCom II), is assessed and compared to results of the first phase. The evaluation is performed using a global monthly gridded data set of aerosol extinction profiles built for this purpose from the CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) Layer Product 3.01. Results over 12 subcontinental regions show that five models improved, whereas three degraded in reproducing the interregional variability in Z α0-6 km, the mean extinction height diagnostic, as computed from the CALIOP aerosol profiles over the 0-6 km altitude range for each studied region and season. While the models' performance remains highly variable, the simulation of the timing of the Z α0-6 km peak season has also improved for all but two models from AeroCom Phase I to Phase II. The biases in Z α0-6 km are smaller in all regions except Central Atlantic, East Asia, and North and South Africa. Most of the models now underestimate Z α0-6 km over land, notably in the dust and biomass burning regions in Asia and Africa. At global scale, the AeroCom II models better reproduce the Z α0-6 km latitudinal variability over ocean than over land. Hypotheses for the performance and evolution of the individual models and for the intermodel diversity are discussed. We also provide an analysis of the CALIOP limitations and uncertainties contributing to the differences between the simulations and observations.

2.
Environ Sci Technol ; 48(24): 14445-54, 2014 Dec 16.
Article in English | MEDLINE | ID: mdl-25405926

ABSTRACT

Biofuels are proposed to play an important role in several mitigation strategies to meet future CO2 emission targets for the transport sector but remain controversial due to significant uncertainties in net impacts on environment, society, and climate. A switch to biofuels can also affect short-lived climate forcers (SLCFs), which provide significant contributions to the net climate impact of transportation. We quantify the radiative forcing (RF) and global-mean temperature response over time to EU on-road fossil diesel SLCFs and the impact of 20% (B20) and 100% (B100) replacement of fossil diesel by biodiesel. SLCFs are compared to impacts of on-road CO2 using different approaches from existing literature to account for biodiesel CO2. Given the best estimates for changes in emissions when replacing fossil diesel with biodiesel, the net positive RF from EU on-road fossil diesel SLCFs of 3.4 mW/m(2) is reduced by 15% and 80% in B20 and B100, respectively. Over time the warming of SLCFs is likely small compared to biodiesel CO2 impacts. However, SLCFs may be relatively more important for the total warming than in the fossil fuel case if biodiesel from feedstock with very short rotation periods and low land-use-change impacts replaces a high fraction of fossil diesel.


Subject(s)
Biofuels , Gasoline , Air Pollutants/analysis , Carbon Dioxide/analysis , Climate , Temperature
3.
Environ Sci Technol ; 48(22): 13273-9, 2014 Nov 18.
Article in English | MEDLINE | ID: mdl-25347302

ABSTRACT

The changing climate in the Arctic opens new shipping routes. A shift to shorter Arctic transit will, however, incur a climate penalty over the first one and a half centuries. We investigate the net climate effect of diverting a segment of Europe-Asia container traffic from the Suez to an Arctic transit route. We find an initial net warming for the first one-and-a-half centuries, which gradually declines and transitions to net cooling as the effects of CO2 reductions become dominant, resulting in climate mitigation only in the long term. Thus, the possibilities for shifting shipping to the Arctic confront policymakers with the question of how to weigh a century-scale warming with large uncertainties versus a long-term climate benefit from CO2 reductions.


Subject(s)
Climate , Ships , Transportation , Arctic Regions , Asia , Europe , Internationality , Temperature , Uncertainty
4.
Environ Sci Technol ; 47(14): 7608-14, 2013 Jul 16.
Article in English | MEDLINE | ID: mdl-23763307

ABSTRACT

The climate impact from a long-distance trip can easily vary by a factor of 10 per passenger depending on mode choice, vehicle efficiency, and occupancy. In this paper we compare the specific climate impact of long-distance car travel with coach, train, or air trips. We account for both, CO2 emissions and short-lived climate forcers. This particularly affects the ranking of aircraft's climate impact relative to other modes. We calculate the specific impact for the Global Warming Potential and the Global Temperature Change Potential, considering time horizons between 20 and 100 years, and compare with results accounting only for CO2 emissions. The car's fuel efficiency and occupancy are central whether the impact from a trip is as high as from air travel or as low as from train travel. These results can be used for carbon-offsetting schemes, mode choice and transportation planning for climate mitigation.


Subject(s)
Climate , Travel , Motor Vehicles
5.
Environ Sci Technol ; 46(9): 5205-13, 2012 May 01.
Article in English | MEDLINE | ID: mdl-22436085

ABSTRACT

Passenger transport affects climate through various mechanisms involving both long-lived and short-lived climate forcers. Because diesel cars generally emit less CO(2) than gasoline cars, CO(2) emission taxes for vehicle registrations and fuels enhance the consumer preference for diesel cars over gasoline cars. However, with the non-CO(2) components, which have been changed and will be changed under the previous and upcoming vehicle emission standards, what does the shift from gasoline to diesel cars mean for the climate mitigation? By using a simple climate model, we demonstrate that, under the earlier emissions standards (EURO 3 and 4), a diesel car causes a larger warming up to a decade after the emissions than a similar gasoline car due to the higher emissions of black carbon and NO(X) (enhancing the O(3) production). Beyond a decade, the warming caused by a diesel car becomes, however, weaker because of the lower CO(2) emissions. As the latter emissions standards (EURO 5 and 6) are phased in, the short-term warming due to a diesel car becomes smaller primarily due to the lower black carbon emissions. Thus, although results are subject to restrictive assumptions and uncertainties, the switch from gasoline to diesel cars encouraged by CO(2) taxes does not contradict with the climate mitigation focusing on long-term consequences.


Subject(s)
Climate , Gasoline , Motor Vehicles/standards , Vehicle Emissions , Uncertainty
6.
Environ Sci Technol ; 44(15): 5700-6, 2010 Aug 01.
Article in English | MEDLINE | ID: mdl-20666553

ABSTRACT

Emissions of short-lived species contribute significantly to the climate impact of transportation. The magnitude of the effects varies over time for each transport mode. This paper compares first the absolute climate impacts of current passenger and freight transportation. Second, the impacts are normalized with the transport work performed and modes are compared. Calculations are performed for the integrated radiative forcing and mean temperature change, for different time horizons and various measures of transport work. An unambiguous ranking of the specific climate impact can be established for freight transportation, with shipping and rail having lowest and light trucks and air transport having highest specific impact for all cases calculated. Passenger travel with rail, coach or two- and three-wheelers has on average the lowest specific climate impact also on short time horizons. Air travel has the highest specific impact on short-term warming, while on long-term warming car travel has an equal or higher impact per passenger-kilometer.


Subject(s)
Air Pollution/statistics & numerical data , Climate Change , Environment , Transportation/statistics & numerical data , Vehicle Emissions/analysis , Air Pollution/analysis , Environmental Monitoring
8.
Proc Natl Acad Sci U S A ; 105(49): 19154-9, 2008 Dec 09.
Article in English | MEDLINE | ID: mdl-19047640

ABSTRACT

Transport affects climate directly and indirectly through mechanisms that cause both warming and cooling of climate, and the effects operate on very different timescales. We calculate climate responses in terms of global mean temperature and find large differences between the transport sectors with respect to the size and mix of short- and long-lived effects, and even the sign of the temperature response. For year 2000 emissions, road transport has the largest effect on global mean temperature. After 20 and 100 years the response in net temperature is 7 and 6 times higher, respectively, than for aviation. Aviation and shipping have strong but quite uncertain short-lived warming and cooling effects, respectively, that dominate during the first decades after the emissions. For shipping the net cooling during the first 4 decades is due to emissions of SO(2) and NOx. On a longer timescale, the current emissions from shipping cause net warming due to the persistence of the CO(2) perturbation. If emissions stay constant at 2000 levels, the warming effect from road transport will continue to increase and will be almost 4 times larger than that of aviation by the end of the century.


Subject(s)
Aviation , Greenhouse Effect , Ships , Temperature , Aerosols/chemistry , Atmosphere , Carbon Dioxide/chemistry , Environment , Models, Theoretical , Nitrogen Oxides/chemistry , Sulfur Dioxide/chemistry
9.
Proc Natl Acad Sci U S A ; 105(2): 454-8, 2008 Jan 15.
Article in English | MEDLINE | ID: mdl-18180450

ABSTRACT

Although the transport sector is responsible for a large and growing share of global emissions affecting climate, its overall contribution has not been quantified. We provide a comprehensive analysis of radiative forcing from the road transport, shipping, aviation, and rail subsectors, using both past- and forward-looking perspectives. We find that, since preindustrial times, transport has contributed approximately 15% and 31% of the total man-made CO2 and O3 forcing, respectively. A forward-looking perspective shows that the current emissions from transport are responsible for approximately 16% of the integrated net forcing over 100 years from all current man-made emissions. The dominating contributor to positive forcing (warming) is CO2, followed by tropospheric O3. By subsector, road transport is the largest contributor to warming. The transport sector also exerts cooling through reduced methane lifetime and atmospheric aerosol effects. Shipping causes net cooling, except on future time scales of several centuries. Much of the forcing from transport comes from emissions not covered by the Kyoto Protocol.


Subject(s)
Air Pollutants/analysis , Air Pollution/legislation & jurisprudence , Air Pollution/prevention & control , Carbon Dioxide/analysis , Conservation of Energy Resources/legislation & jurisprudence , Conservation of Energy Resources/methods , Vehicle Emissions/analysis , Aerosols , Air Pollution/economics , Atmosphere , Carbon Dioxide/chemistry , Carbon Dioxide/economics , Climate , Conservation of Energy Resources/economics , Greenhouse Effect , Models, Theoretical , Ozone/chemistry , Reference Values , Transportation
10.
Philos Trans A Math Phys Eng Sci ; 365(1856): 1903-14, 2007 Jul 15.
Article in English | MEDLINE | ID: mdl-17513272

ABSTRACT

Multi-gas climate agreements require a metric by which emissions of gases with different lifetimes and radiative properties can be placed on a common scale. The Kyoto Protocol to the United Nations Framework Convention on Climate Change uses the global warming potential (GWP) as such a metric. The GWP has attracted particular criticism as being inappropriate in the context of climate policy which seeks to restrict warming below a given target, because it gives equal weight to emissions irrespective of the target and the proximity to the target. The use of an alternative metric, the time-dependent global temperature change potential (GTP), is examined for its suitability and the prospects for it including very short-lived species. It retains the transparency and relative ease of use, which are attractive features of the GWP, but explicitly includes a dependence on the target of climate policy. The weighting of emissions using the GTP is found to be significantly dependent on the scenarios of future emissions and the sensitivity of the climate system. This may indicate that the use of any GTP-based weighting in future policymaking would necessitate regular revisions, as the global-mean temperature moves towards a specified target.


Subject(s)
Greenhouse Effect , Models, Theoretical , Public Policy
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