A new approach to radon temporal correction factor based on active environmental monitoring devices.

The present study aims to identify novel means of increasing the accuracy of the estimated annual indoor radon concentration based on the application of temporal correction factors to short-term radon measurements. The necessity of accurate and more reliable temporal correction factors is in high demand, in the present age of speed. In this sense, radon measurements were continuously carried out, using a newly developed smart device accompanied by CR-39 detectors, for one full year, in 71 residential buildings located in 5 Romanian cities. The coefficient of variation for the temporal correction factors calculated for combinations between the start month and the duration of the measurement presented a low value (less than 10%) for measurements longer than 7 months, while a variability close to 20% can be reached by measurements of up to 4 months. Results obtained by generalized estimating equations indicate that average temporal correction factors are positively associated with CO2 ratio, as well as the interaction between this parameter and the month in which the measurement took place. The impact of the indoor-outdoor temperature differences was statistically insignificant. The obtained results could represent a reference point in the elaboration of new strategies for calculating the temporal correction factors and, consequently, the reduction of the uncertainties related to the estimation of the annual indoor radon concentration.

Comprehensive survey on radon mitigation and indoor air quality in energy efficient buildings from Romania.

Over the last 10 years applied scientific research has been carried out in Romania to tacked the residential radon issues. The increased interest to reduce the carbon footprint of buildings has lead to the implementation and use of new architectural solutions aimed to save energy in houses and other buildings. As a consequence, the degree of retrofit in existing buildings and energy efficiency of new buildings promoted the need to not only mitigate indoor radon, but improve indoor air quality overall. The present study found that the while the best performance in radon reduction was confirmed to be based on sub-slab depressurization (61% - 95% reduction), centralized and decentralized mechanical supply and exhaust ventilation with heat recovery yielded a good efficiency in overall improvement of indoor air quality (CO2, VOC, RH, temperature). The outcome of our research, as well as future perspectives, take into account the recommended harmonization of energy efficiency programs with those of public health by finding and applying the best technologies in compliance with energy saving and indoor environmental quality.

ASSESSMENT OF ANNUAL EFFECTIVE DOSE FROM EXPOSURE TO NATURAL RADIOACTIVITY SOURCES IN A CASE-CONTROL STUDY IN BIHOR COUNTY, ROMANIA.

The purpose of the article is to evaluate the annual effective dose for 80 women divided into two samples; one sample located in the former uranium Baita-Stei area, hereinafter referred to as case sample, respectively for a control sample, located in the same county, but exposed in most cases to indoor radon activity concentrations <300 Bq m-3. In this regard, the homemade 'RaThoGamma' kit was used, which contained two thermoluminescent dosimeters, a CR-39 track detector (RSKS) for indoor radon activity concentration, two CR-39 track detectors (Radtrak2®/ Radtrak2T®) for radon and thoron activity concentrations as well as Direct Radon Progeny Sensors/Direct Thoron Progeny Sensors for measuring time-averaged radon and thoron progenies concentrations. In addition, a total of 80 water samples were collected in order to evaluate the ingestion dose due to radon and radium activity concentrations in drinking water. The maximum total annual effective dose in the control sample was 14.1 mSv, while in the case sample the maximum annual effective dose was 60.5 mSv. This difference is mainly due to radon progenies inhalation. Other pathways did not show a statistically significant difference between the two samples, showing a minor contribution to the annual effective dose.

THE CHALLENGE IN USING THE RETROSPECTIVE ASSESSMENT OF RESIDENTIAL RADON CONCENTRATION.

In the present study, the contemporary indoor radon activity concentration and the surface-deposited 210Po activity were measured in 65 Romanian dwellings. The activity of trapped 210Po on the glass surface was measured using the (CR-LR) difference technique. The retrospective radon activity concentration estimated on the basis of age-adjusted 210Po activity was found to have a geometric mean of 318 Bq m-3, being higher than the geometric mean (250 Bq m-3) of the contemporary indoor radon measurements, measured with two types of track detectors (RSKS and Radtrak2®). By applying Lin's concordance correlation coefficient, a substantial strength of agreement (rC = 0.94) was obtained between RSKS and Radtrak2® results, respectively a poor agreement (rC = 0.71) between the retrospective and contemporary methods. The ratio between contemporary and retrospective radon concentrations has a geometric mean of 0.8 and range from 0.2 to 3.9.

DISTRIBUTION OF RADON GAS IN ROMANIAN SHOW CAVES AND RADIATION SAFETY.

In many countries, caves can pose an economic interest for the authorities and stakeholders. The development of a show cave requires, apart from the conservation issues, to ensure the human safety by minimising the exposure to radon for cave personnel and visitors. Radon levels can vary widely from cave to cave, being directly correlated with different internal and external factors. It is therefore important to monitor radon levels before establishing the number of personnel required, so that they are not exposed to health-threatening levels of radiation. A long-term radon survey was carried out for this purpose in five show caves of Romania. The study pointed out the existence of high-radon potential areas inside the caves with concentrations reaching up to 4024 Bqm-3, thus posing radiological hazard to cave personnel and researchers who develop activities underground. Further research focused on personal dosimetry will be necessary for an efficient management of occupational risk.

THE GEOGENIC RADON POTENTIAL MAP OF THE ASPIRING 'BUZAU LAND' GEOPARK.

Mapping the geogenic radon potential in Buzau County is part of a research project aiming to apply research for sustainable development and economic growth following the principles of geoconservation in order to support the 'Buzau Land' UNESCO Geopark initiative. The mapping of geogenic radon will be used as an overview for planning purposes. The main geological formations of the studied area were identified as Cretaceous and Paleogene flysch, included in a thin-skinned nappes pile and consisting of alternating sandstones, marls, clays and, subordinately, conglomerates, all tightly folded or faulted. Significant variations in the concentration of radon were therefore determined in the ground. However, no high values were determined, the maximum measured activity concentration being 101.6 kBq m-3.

COMPARATIVE STUDY OF RADON AND THORON MEASUREMENTS IN FOUR ROMANIAN SHOW CAVES.

Measurements have been carried out using four types of passive detectors in four of the most popular show caves in Romania. Three types of detectors (RSKS, RadTrak and CD) were used for radon measurements and two (Raduet and CD) for thoron measurement. Activity concentrations in air were measured in the same locations for two seasons, autumn and winter. Measured values for the different caves varied between below detection limit (5 Bq m-3) and 4024 Bq m-3 for radon and from below 10 to 583 Bq m-3 for thoron. The results indicate a very good correlation between RSKS and RadTrak detectors (r = 0.96). The most significant difference between radon concentrations measured with different types of detectors (RSKS and CD) was higher than 150%. The study suggests that the activity concentration of radon in caves, measured using track detectors, could not be influenced by the type of detector used if the microclimate factor is acknowledged.

New study on the correlation between carbon dioxide concentration in the environment and radon monitor devices.

The influence of high geogenic carbon dioxide concentrations on monitoring devices might present a significant challenge to the measurement of radon concentrations in environments with a high level of carbon dioxide concentration such as volcano sites, mofettes, caves, etc. In this study, the influence of carbon dioxide concentration on several different types of radon monitor devices - including Alpha Spectrometry (Sarad RTM 2200, EQF 3220, RAD7), Ionizing Chamber (AlphaGUARD PQ2000 PRO) and Active Cell (Active scintillation cell, Pylon 300A) - was examined to represent new aspects of radon measuring in environments with carbon dioxide. In light of the results, all measuring devices were exposed to variable conditions affected by carbon dioxide concentration, except for the AlphaGUARD, which was kept in a steady state throughout the experiment. It was observed that alpha spectroscopy devices were affected by carbon dioxide, since measured radon concentrations decreased in the presence of 70% and 90% carbon dioxide concentrations by 26.5 ± 2% and 14.5 ± 2.5% for EQF 3220, and 32 ± 2% and 35.5 ± 2% for RTM 2200. However, the ionizing chamber instrument was unaffected by changes in carbon dioxide concentration. It was determined that the RAD7 performed relatively inefficiently in the presence of carbon dioxide concentrations higher than 67% by an overall efficiency factor of approximately 0.52, confirming that it is not an admissible radon monitor instrument in environments with high carbon dioxide concentrations.

Radon and radium concentration in water from North-West of Romania and the estimated doses.

In the present study, the measurements of radon were carried out using the LUK-VR system based on radon gas measurements with Lucas cells. The radium concentration in water was determined, with the same device, immediately after was established the radon equilibrium with radium. The results presented here are from a survey carried out in the N-W region of Transylvania (Romania) in which were investigated the radon concentrations in natural (spring, well and surface) and drinking (tap) waters. The results showed radon concentrations within the range of 0.4-187.3 Bq l(-1) with an average value of 15.9 Bq l(-1) whereas radium concentration varied between 0.05 and 0.825 Bq l(-1) with an average value of 0.087 Bq l(-1) for all types of water covered within this survey. The corresponding annual effective ingestion dose due to radon and radium from water was determined from drinking water used by the population inhabiting the area.

Thoron and radon measurements in Romanian schools.

A new thoron/radon survey was started in the north-western part of Romania, covering three counties, using discriminative detectors (RADUET). All detectors were deployed throughout 3 months, covering the spring period. The measured radon and thoron concentration ranged from 31 to 414 Bq m(-3) and from below the detection limit to 235 Bq m(-3), respectively. In this survey, 35 schools were submitted to investigation; 21 of the schools included in this study presented radon concentrations higher than 100 Bq m(-3), the reference level recommended by the World Health Organization in 2009. The seasonal effective dose calculated from these exposures, overlapping all three counties, ranged between 0.32 and 0.54 mSv.