Reconfigurable design of a thermo-optically addressed liquid-crystal phase modulator by a neural network.

We present a machine learning approach to program the light phase modulation function of an innovative thermo-optically addressed, liquid-crystal based, spatial light modulator (TOA-SLM). The designed neural network is trained with a little amount of experimental data and is enabled to efficiently generate prescribed low-order spatial phase distortions. These results demonstrate the potential of neural network-driven TOA-SLM technology for ultrabroadband and large aperture phase modulation, from adaptive optics to ultrafast pulse shaping.

Spectral coherence properties of continuum generation in bulk crystals.

The stability of the phase difference between two white-light continua, generated from the same 180-fs pulses at ≃1035 nm, is assessed by a modified Bellini-Hänsch interferometer. Mutual spectral phase stability is studied and quantified as a function of several parameters: pulse energy, position of the nonlinear crystal with respect to the beam waist and interaction length. Our results show that intrapulse decoherence may significantly contribute to the measured CEP noise floor. In addition, spectrally-resolved intensity-to-phase coupling coefficients are measured and stability regions are identified.

Femtosecond laser-induced damage threshold of nematic liquid crystals at 1030 nm.

The laser-induced damage threshold (LIDT) of nematic liquid crystals is investigated in the femtosecond regime at ≃1030nm. The thickness and breakdown of freely suspended thin films (≃100nm) of different mixtures (MLC2073, MLC2132, and E7) is monitored in real time by spectral-domain interferometry. The duration of laser pulses was varied from 180 fs to 1.8 ps for repetition rates ranging from single shot to 1 MHz. The dependence of the LIDT with pulse duration suggests a damage mechanism dominated by ionization mechanisms at low repetition rate and by linear absorption at high repetition rate. In the single-shot regime, LIDTs exceeding 1J/cm2 are found for the three investigated mixtures. The LIDT of polyvinyl alcohol is also investigated by the same method.

Spectral pulse shaping of a 5 Hz, multi-joule, broadband optical parametric chirped pulse amplification frontend for a 10 PW laser system.

We present a broadband optical parametric chirped pulse amplification (OPCPA) system delivering 4 J pulses at a repetition rate of 5 Hz. It will serve as a frontend for the 1.5 kJ, <150 fs, 10 PW laser beamline currently under development by a consortium of National Energetics and Ekspla. The spectrum of the OPCPA system is precisely controlled by arbitrarily generated waveforms of the pump lasers. To fully exploit the high flexibility of the frontend, we have developed a 1D model of the system and an optimization algorithm that predicts suitable pump waveform settings for a desired output spectrum. The OPCPA system is shown to have high efficiency, a high-quality top-hat beam profile, and an output spectrum demonstrated to be shaped consistently with the theoretical model.

Design of a 10 PW (150 J/15 fs) peak power laser system with Ti:sapphire medium through spectral control.

We designed a 10 PW (150 J-15 fs) laser system based on the use of titanium-doped sapphire power amplifiers. The solution is to provide an overall compensating spectral gain narrowing and shifting technique for obtaining a controlled output spectrum.

Highly efficient nonlinear filter for femtosecond pulse contrast enhancement and pulse shortening.

We propose a highly efficient scheme for temporal filters devoted to femtosecond pulse contrast enhancement. The filter is based on cross-polarized wave generation with a spatially suger-Gaussian-shaped beam. In a single nonlinear crystal scheme the energy conversion to the cross-polarized pulse can reach 28%. We demonstrate that the process enables a significant spectral broadening. For an efficiency of 23% the pulse shortening is estimated to 2.2, leading to an intensity transmission of the nonlinear filter of 50%.

Superresolved femtosecond laser ablation.

The determinist behavior of the femtosecond ablation process allows morphing features well under the diffraction limit by utilizing the thresholding effect, down to the nanometer scale. Because there are a vast range of applications where scaling down the size of the features is a major concern, we investigate the use of superresolving pupil plane filters. As is well known, these filters redistribute the focused optical intensity for a narrower bright spot and, as a trade-off, increase the sidelobes. However, this drawback can be rendered insignificant if all the outer optical power is kept under the determinist threshold value. Two types of pure absorbing binary filter have been tried, giving credence to a size reduction of the ablations in fused silica.

Pump-noise transfer in optical parametric chirped-pulse amplification.

We report on direct observation of temporal contrast degradation of short pulses amplified by optical parametric chirped-pulse amplification. We show that, despite injection seeding, quantum-noise-induced fast modulations (< 50 ps) of the temporal profile of the pump pulse are imprinted on the spectrum of the amplified chirped pulse and give rise to a large picosecond pedestal in the time domain.

10(-10) temporal contrast for femtosecond ultraintense lasers by cross-polarized wave generation.

We take advantage of nonlinear properties associated with chi(3) tensor elements in BaF2 cubic crystal to improve the temporal contrast of femtosecond laser pulses. The technique presented is based on cross-polarized wave (XPW) generation. We have obtained a transmission efficiency of 10% and 10(-10) contrast with an input pulse in the millijoule range. This filter does not affect the spectral shape or the phase of the cleaned pulse. It also acts as an efficient spatial filter. In this method the contrast enhancement is limited only by the extinction ratio of the polarization discrimination device.

Experimental evidence of 25-fs laser pulse distortion in singlet beam expanders.

We report the measurement of spatiotemporal distortions of an ultrashort pulse in singlet beam expanders. With a simple second-order autocorrelator the temporal broadening of the pulse from 23 to 40 fs, due to propagation time difference (PTD), is determined. The delay due to PTD between different parts of the beam is also measured. This effect was theoretically studied for the first time by Bor [J. Mod. Opt. 35, 1907 (1988)]. These experimental results are in good agreement with the calculations of a dedicated three-dimensional ray-tracing program developed to simulate the spatial and temporal transformation of femtosecond pulses in optical systems.

High-efficiency, simple setup for pulse cleaning at the millijoule level by nonlinear induced birefringence.

Nonlinear elliptical polarization rotation is used to improve the contrast of femtosecond pulses by several orders of magnitude. Using nonlinear induced birefringence in air, we produced cleaned pulses with an energy of a few hundreds of microjoules. This technique presents several major advantages, such as convenience and stability of the setup. We investigated the phase profile required for obtaining high-energy pulses. No phase distortion is observed, and the spatial quality of the beam is preserved.