Flexible, fast, and benchmarked vectorial model for focused laser beams.

In-bulk processing of materials by laser radiation has largely evolved over the last decades and still opens up new scientific and industrial potentials. The development of any in-bulk processing application relies on the knowledge of laser propagation and especially the volumetric field distribution near the focus. Many commercial programs can simulate this, but, to adapt them, or to develop new methods, one usually must create a specific software. Besides, most of the time people also need to measure the actual field distribution near the focus to evaluate their assumptions in the simulation. To easily get access to this knowledge, we present our high-precision field distribution measuring method and release our in-house software InFocus [https://github.com/QF06/InFocus], under the Creative Commons 4.0 license. Our measurements provide 300 nm longitudinal resolution and diffraction limited lateral resolution. The in-house software allows fast vectorial analysis of the focused volumetric field distribution in bulk. Simulations of the linear propagation of light under different conditions (focusing optics, wavelength, spatial shape, and propagation medium) are in excellent agreement with propagation imaging experiments. The aberrations provoked by the refractive index mismatch as well as those induced by the focusing optics are both taken into account. The results indicate that our proposed model is suitable for the precise evaluation of energy deposition.

Tailoring modulation instabilities and four-wave mixing in dispersion-managed composite liquid-core fibers.

We show that the ultrafast nonlinear dynamics in supercontinuum generation can be tailored via mixture-based liquid core fibers. Samples containing mixtures of inorganic solvents allow changing dispersion from anomalous to normal, i.e., shifting zero dispersion across pump laser wavelength. A significant control over modulation instability and four-wave mixing has been demonstrated experimentally in record-long (up to 60 cm) samples in agreement with simulations when using sub-psec pulses at 1.555 µm. The smallest concentration ratio yields indications of soliton-fission based supercontinuum generation at soliton numbers that are beyond the coherence limit. The presented dispersion tuning scheme allows creating unprecedented dispersion landscapes for accessing unexplored nonlinear phenomena and selected laser sources.

Phenomenological modelling of non-volatile memory threshold voltage shift induced by nonlinear ionization with a femtosecond laser.

The behaviour of semiconductor materials and devices subjected to femtosecond laser irradiation has been under scrutiny, for many reasons, during the last decade. In particular, recent works have shown that the specific functionality and/or geometry of semiconductor devices, among which non-volatile memory (NVM) devices hold a special place, could be used to improve the knowledge about ultrafast laser-semiconductor interactions. So far, such an approach has been applied to draw conclusions about the spatio-temporal properties of laser propagation in bulk materials. Here, by comparing the evolution of the electrical characteristics of Flash cells under the cumulative effect of repeated femtosecond laser pulses with first-order physical considerations and TCAD (Technology Computer Aided Design) simulations, we clearly establish the role of the carriers created by nonlinear ionization on the functionality of the structures. The complete electrical analysis informs indirectly on the energy of the laser-produced free-carriers which, to date, was almost inaccessible by an experimental method applicable to the bulk of a material. Establishing the link between the carrier energy and laser parameters is of major importance to improve the comprehension of the nonlinear ionization mechanisms associated to intense laser-semiconductor interactions and applied in various fields from microelectronics to laser micromachining.

Wavelength dependence of the mechanisms governing the formation of nanosecond laser-induced damage in fused silica.

The influence of the wavelength on the morphology of nanosecond laser-induced damage on the exit surface of fused silica is investigated. A combination between the typical features of damage sites initiated at 1064 nm and 355 nm is observed at 532 nm, including ring patterns sporadically exhibited, in good agreement with calculations of the development of an electron avalanche at this wavelength. The associated ring appearance speed scales as the cube root of the laser intensity, and is ~10.5 km/s while it is ~20 km/s when initiated by infrared pulses. The whole set of results sheds light on the different wavelength-dependent mechanisms governing damage formation.

Nanosecond laser damage initiation at 0.35 µm in fused silica.

In nanosecond regime, the laser-induced damage density at the exit surface of fused silica optics at the wavelength of 0.35 µm shows a characteristic behavior: in a specific fluence range, the surface damage density begins to grow exponentially as a function of fluence and then tends to saturate at high fluences. Up to now, no satisfactory explanation of these peculiarities could be provided. We herein detail a statistical model based on laser-matter interaction, where two types of absorbing precursors are involved in the energy deposit: subsurface micro-cracks and surface impurities. We show that the reported model predicts this characteristic damage density for a large range of fluences and different polishing processes.

Multi-wavelength growth of nanosecond laser-induced surface damage on fused silica gratings.

The nanosecond laser-induced damage growth phenomenon on the exit surface of fused silica grating is investigated at 1064 nm and 355 nm separately and also simultaneously. Experiments are first carried out on damage sites on a plane fused silica sample showing two different morphologies, and a damage type is selected for ensuring the repeatability of the subsequent tests. Comparing the mono-wavelength growth results on a grating and a plane fused silica sample, the periodic surface structure is found to be an aggravating factor for damage growth. This is highly supported by calculations of the enhancement of the optical electric field intensity thanks to Finite-Difference Time-Domain simulations. Finally, the mono-wavelength results enable us to quantify a coupling occurring in the multi-wavelength configuration, which could originate from the heating of the plasma (more likely produced in the ultraviolet) preferentially by the infrared pulse. This study provides interesting results about the involvement of the surface topography in damage growth, and paves the way towards the comprehension of this phenomenon at high-energy nanosecond laser facilities where fused silica gratings are simultaneously irradiated at several wavelengths.

Crossing the threshold of ultrafast laser writing in bulk silicon.

An important challenge in the field of three-dimensional ultrafast laser processing is to achieve permanent modifications in the bulk of silicon and narrow-gap materials. Recent attempts by increasing the energy of infrared ultrashort pulses have simply failed. Here, we establish that it is because focusing with a maximum numerical aperture of about 1.5 with conventional schemes does not allow overcoming strong nonlinear and plasma effects in the pre-focal region. We circumvent this limitation by exploiting solid-immersion focusing, in analogy to techniques applied in advanced microscopy and lithography. By creating the conditions for an interaction with an extreme numerical aperture near 3 in a perfect spherical sample, repeatable femtosecond optical breakdown and controllable refractive index modifications are achieved inside silicon. This opens the door to the direct writing of three-dimensional monolithic devices for silicon photonics. It also provides perspectives for new strong-field physics and warm-dense-matter plasma experiments.Ultrafast laser processing is a versatile three-dimensional photonic structuring method but it has been limited to wide band gap materials like glasses. Here, Chanal et al. demonstrate direct refractive-index modification in the bulk of silicon by extreme localization of the energy deposition.

Investigations on laser damage growth in fused silica with simultaneous wavelength irradiation.

The laser-induced damage growth phenomenon is experimentally studied for damage sites on the exit surface of fused silica. The sites are irradiated by nanosecond laser pulses at 1064 and 355 nm separately and also simultaneously. The results in the single wavelength configurations are expressed in terms of the probability of growth and growth coefficient. For growing sites, a fluence correction expression is proposed in order to take into account the millimetric Gaussian profile of the beams. The use of this expression is necessary to obtain results that are consistent with the ones obtained in the existing literature with large homogeneous beams. In the multiple wavelengths configuration, the results are expressed as a function of the laser fluences at each wavelength and are found to be closely related to the parameters determined in the single wavelength experiments. A coupling between the two wavelengths is quantified, and could originate from the formation and the expansion of a plasma produced both in the center and at the periphery of the damage sites.