Dynamical charge density fluctuations pervading the phase diagram of a Cu-based high-T c superconductor.

Charge density modulations have been observed in all families of high-critical temperature (T c) superconducting cuprates. Although they are consistently found in the underdoped region of the phase diagram and at relatively low temperatures, it is still unclear to what extent they influence the unusual properties of these systems. Using resonant x-ray scattering, we carefully determined the temperature dependence of charge density modulations in YBa2Cu3O7-δ and Nd1+ x Ba2- x Cu3O7-δ for several doping levels. We isolated short-range dynamical charge density fluctuations in addition to the previously known quasi-critical charge density waves. They persist up to well above the pseudogap temperature T*, are characterized by energies of a few milli-electron volts, and pervade a large area of the phase diagram.

Electronic polymers and soft-matter-like broken symmetries in underdoped cuprates.

Empirical evidence in heavy fermion, pnictide and other systems suggests that unconventional superconductivity appears associated to some form of real-space electronic order. For the cuprates, despite several proposals, the emergence of order in the phase diagram between the commensurate antiferromagnetic state and the superconducting state is not well understood. Here we show that in this regime doped holes assemble in 'electronic polymers'. Within a Monte Carlo study, we find that in clean systems by lowering the temperature the polymer melt condenses first in a smectic state and then in a Wigner crystal both with the addition of inversion symmetry breaking. Disorder blurs the positional order leaving a robust inversion symmetry breaking and a nematic order, accompanied by vector chiral spin order and with the persistence of a thermodynamic transition. Such electronic phases, whose properties are reminiscent of soft-matter physics, produce charge and spin responses in good accord with experiments.

Spin excitations of ferronematic order in underdoped cuprate superconductors.

High-temperature superconductors exhibit a characteristic hourglass-shaped spectrum of magnetic fluctuations which most likely contribute to the pairing glue in the cuprates. Recent neutron scattering experiments in strongly underdoped compounds have revealed a significant low energy anisotropy of these fluctuations which we explain by a model in which topological defects of the antiferromagnet clump to producing domain wall segments with ferronematic order. This state does not invoke global charge order but breaks C4 rotational and inversion symmetry. The incommensurability of the low doping charge-disordered state is in good agreement with experiment and interpolates smoothly with the incommensurability of the stripe phase at higher doping. Within linear spin-wave theory the dynamic structure factor is in very good agreement with inelastic neutron scattering data and can account for the observed energy dependent anisotropy.

Coulomb-frustrated phase separation phase diagram in systems with short-range negative compressibility.

Using numerical techniques and asymptotic expansions we obtain the phase diagram of a paradigmatic model of Coulomb-frustrated phase separation in systems with negative short-range compressibility. The transition from the homogeneous phase to the inhomogeneous phase is generically first order in isotropic three-dimensional systems except for a critical point. Close to the critical point, inhomogeneities are predicted to form a bcc lattice with subsequent transitions to a triangular lattice of rods and a layered structure. Inclusion of a strong anisotropy allows for second- and first-order transition lines joined by a tricritical point.

Charge-fluctuation contribution to the Raman response in superconducting cuprates.

We calculate the Raman response contribution due to soft collective modes, finding a strong dependence on the photon polarizations and on the characteristic wave vectors of the modes. We compare our results with recent Raman spectroscopy experiments in underdoped cuprates, La2-xSrxCuO4 and (Y1.97Ca0.3)Ba2CuO6.05, where anomalous low-energy peaks are observed, which soften upon lowering the temperature. We show that the specific dependence on doping and on photon polarizations of these peaks can naturally arise from charge collective excitations at finite wavelength.

Phase separation close to the density-driven Mott transition in the Hubbard-Holstein model.

The density-driven Mott transition is studied by means of dynamical mean-field theory in the Hubbard-Holstein model, where the Hubbard term leading to the Mott transition is supplemented by an electron-phonon (e-ph) term. We show that an intermediate e-ph coupling leads to a first-order transition at T=0, which is accompanied by a phase separation between a metal and an insulator. The compressibility in the metallic phase is substantially enhanced. At quite larger values of the coupling, a polaronic phase emerges coexisting with a nonpolaronic metal.

Anomalous optical absorption in the normal state of overdoped cuprates near the charge-ordering instability.

We argue that the hump observed in the optical conductivity at or below a few hundreds of cm(-1), in overdoped cuprates such as the electron-doped Nd(2-x)Ce(x)CuO(4-y) at x > or approximately equal to 0.15 and the hole-doped Bi2Sr2CuO6 and La2-xSrxCuO4, cannot be accounted for within a single-fluid description. We propose instead an interpretation based on the direct excitation of charge collective modes, which become nearly critical in the proximity to a charge-ordering instability. Their critical character entails a peculiar temperature dependence and a pseudoscaling form of the optical spectra, which agree with the experimental data.

Vertex corrections near the stripe phase.

We calculate the vertex corrections within a model for fermion quasiparticles coupled with charge and spin fluctuations, which provide the relevant scattering mechanism near the stripe instability in high- T(c) cuprates. The logarithmic divergence of the vertex, which characterizes the spin-fermion model near the antiferromagnetic instability, is ruled out, due to the incommensuration of the charge and spin modulation within the stripe phase, as revealed by neutron scattering. This simplifies the skeleton structure of the problem. The vertex is negative in the relevant kinematical regime, effectively reducing the interaction strength. Our results apply to generic incommensurate instabilities of electronic origin.

Anomalous isotopic effect near the charge-ordering quantum criticality.

Within the Hubbard-Holstein model, we evaluate the crossover lines marking the opening of pseudogaps in the cuprates, which, in our scenario, are ruled by the proximity to a charge-ordering quantum criticality (stripe formation). We find that their isotopic dependence, due to critical fluctuations, implies a substantial positive shift of the pseudogap-formation temperature T(*). We infer that the isotopic shift of the superconducting T(c) is nearly absent in the optimally and overdoped regimes and is negative and increasing upon underdoping. The dynamical nature of the charge-ordering transition may explain the spread of the experimental values of T(*).