Observation of Vacuum-Induced Collective Quantum Beats.

We demonstrate collectively enhanced vacuum-induced quantum beat dynamics from a three-level V-type atomic system. Exciting a dilute atomic gas of magneto-optically trapped ^{85}Rb atoms with a weak drive resonant on one of the transitions, we observe the forward-scattered field after a sudden shut-off of the laser. The subsequent radiative dynamics, measured for various optical depths of the atomic cloud, exhibits superradiant decay rates, as well as collectively enhanced quantum beats. Our work is also the first experimental illustration of quantum beats arising from atoms initially prepared in a single excited level as a result of the vacuum-induced coupling between excited levels.

Non-Markovian Collective Emission from Macroscopically Separated Emitters.

We study the collective radiative decay of a system of two two-level emitters coupled to a one-dimensional waveguide in a regime where their separation is comparable to the coherence length of a spontaneously emitted photon. The electromagnetic field propagating in the cavity-like geometry formed by the emitters exerts a retarded backaction on the system leading to strongly non-Markovian dynamics. The collective spontaneous emission rate of the emitters exhibits an enhancement or inhibition beyond the usual Dicke superradiance and subradiance due to self-consistent coherent time-delayed feedback.

Spin-Wave Multiplexed Atom-Cavity Electrodynamics.

We introduce multiplexed atom-cavity quantum electrodynamics with an atomic ensemble coupled to a single optical cavity mode. Multiple Raman dressing beams establish cavity-coupled spin-wave excitations with distinctive spatial profiles. Experimentally, we demonstrate the concept by observing spin-wave vacuum Rabi splittings, selective superradiance, and interference in the cavity-mediated interactions of two spin waves. We highlight that the current experimental configuration allows rapid, interchangeable cavity coupling to 4 profiles with an overlap parameter of less than 10%, enough to demonstrate, for example, a quantum repeater network simulation in the cavity. With further improvements to the optical multiplexing setup, we infer the ability to access more than 10^{3} independent spin-wave profiles.

Quantum-Limited Atomic Receiver in the Electrically Small Regime.

We use a quantum sensor based on thermal Rydberg atoms to receive data encoded in electromagnetic fields in the extreme electrically small regime, with a sensing volume over 10^{7} times smaller than the cube of the electric field wavelength. We introduce the standard quantum limit for data capacity, and experimentally observe quantum-limited data reception for bandwidths from 10 kHz up to 30 MHz. In doing this, we provide a useful alternative to classical communication antennas, which become increasingly ineffective when the size of the antenna is significantly smaller than the wavelength of the electromagnetic field.

Spin-optomechanical coupling between light and a nanofiber torsional mode.

Light that carries linear or angular momentum can interact with a mechanical object, giving rise to optomechanical effects. In particular, a photon can transfer its intrinsic angular momentum to an object when the object either absorbs the photon or changes the photon polarization, as in an action/reaction force pair. Here, we demonstrate resonant driving of torsional mechanical modes of a single-mode tapered optical nanofiber using spin angular momentum. The nanofiber torsional mode spectrum is characterized by polarimetry, showing narrow natural resonances (Q≈2,000). By sending amplitude-modulated light through the nanofiber, we resonantly drive individual torsional modes as a function of the light polarization. By varying the input polarization to the fiber, we find the largest amplification of a mechanical oscillation (>35 dB) is observed when driving the system with light containing longitudinal spin on the nanofiber waist. These results present optical nanofibers as a platform suitable for quantum spin-optomechanics experiments.

Twists in nonlinear magneto-optic rotation with cold atoms.

We observe a narrow secondary dispersive feature nested within conventional nonlinear magneto-optical rotation (NMOR) signals obtained with a laser-cooled rubidium vapor. A similar feature has been previously named a "twist" by Budker et. al., in the context of warm vapor optical magnetometry [Phys. Rev. A. 81, 5788-5791 (1998)], and was ascribed to simultaneous optical pumping through multiple nearby hyperfine levels. In this work the twist is observed in a cold atom vapor, where the hyperfine levels are individually addressable, and thus is due to a different mechanism. We experimentally and numerically characterize this twist in terms of magnetic field strength, polarization, and optical intensity and find good agreement between our data and numerical models. We find that the twist width is proportional to the magnetic field in the transverse direction, and therefore two independent directions of the magnetic field can be measured simultaneously. This technique is useful as a simple and rapid in-situ method for nulling background magnetic fields.

Dynamics of trapped atoms around an optical nanofiber probed through polarimetry.

The evanescent field outside an optical nanofiber (ONF) can create optical traps for neutral atoms. We present a non-destructive method to characterize such trapping potentials. An off-resonance linearly polarized probe beam that propagates through the ONF experiences a slow axis of polarization produced by trapped atoms on opposite sides along the ONF. The transverse atomic motion is imprinted onto the probe polarization through the changing atomic index of refraction. By applying a transient impulse, we measure a time-dependent polarization rotation of the probe beam that provides both a rapid and non-destructive measurement of the optical trapping frequencies.

Energy Transfer Sensitization of Luminescent Gold Nanoclusters: More than Just the Classical Förster Mechanism.

Luminescent gold nanocrystals (AuNCs) are a recently-developed material with potential optic, electronic and biological applications. They also demonstrate energy transfer (ET) acceptor/sensitization properties which have been ascribed to Förster resonance energy transfer (FRET) and, to a lesser extent, nanosurface energy transfer (NSET). Here, we investigate AuNC acceptor interactions with three structurally/functionally-distinct donor classes including organic dyes, metal chelates and semiconductor quantum dots (QDs). Donor quenching was observed for every donor-acceptor pair although AuNC sensitization was only observed from metal-chelates and QDs. FRET theory dramatically underestimated the observed energy transfer while NSET-based damping models provided better fits but could not reproduce the experimental data. We consider additional factors including AuNC magnetic dipoles, density of excited-states, dephasing time, and enhanced intersystem crossing that can also influence ET. Cumulatively, data suggests that AuNC sensitization is not by classical FRET or NSET and we provide a simplified distance-independent ET model to fit such experimental data.

Spatially-resolved Rayleigh scattering for analysis of vector mode propagation in few-mode fibers.

We use high-resolution imaging of Rayleigh scattered light through the side of few-mode optical fibers to measure the local spatial structure of propagating vector fields. We demonstrate the technique by imaging both pure modes and superpositions of modes in the LP01 and LP11 families. Direct imaging not only gives high-resolution beat length measurements, but also records the local propagation dynamics including those due to perturbations. The imaging setup uses polarization discrimination to monitor both the transverse and the longitudinal polarization components simultaneously.

Rapid complex mode decomposition of vector beams by common path interferometry.

We have used common path interferometry for rapid determination of the electric field and complex modal content of vector beams, which have spatially-varying polarization. We combine a reference beam with a signal beam prior to a polarization beam splitter for stable interferograms that preserve intermodal phase shifts even in noisy environments. Interferometric decomposition into optical modes (IDIOM) provides a direct, sensitive measure of the complete electric field, enabling rapid modal decomposition and is ideally suited to single-frequency laser sources. We apply the technique to beams exiting optical fibers that support up to 10 modes. We also use the technique to characterize the fibers by determining a scattering matrix that transforms an input superposition of modes into an output superposition. Furthermore, because interferograms are linear in the field, this technique is very sensitive and can accurately reconstruct beams with signal-to-noise << 1.

Quantum memory in warm rubidium vapor with buffer gas.

The realization of quantum memory using warm atomic vapor cells is appealing because of their commercial availability and the perceived reduction in experimental complexity. In spite of the ambiguous results reported in the literature, we demonstrate that quantum memory can be implemented in a single cell with buffer gas using the geometry where the write and read beams are nearly copropagating. The emitted Stokes and anti-Stokes photons display cross-correlation values greater than 2, characteristic of quantum states, for delay times up to 4 µs.

Suppression of the zero-order diffracted beam from a pixelated spatial light modulator by phase compression.

Phase compression is used to suppress the on-axis zero-order diffracted (ZOD) beam from a pixelated phase-only spatial light modulator (SLM) by a simple modification to the computer generated hologram (CGH) loaded onto the SLM. After CGH design, the phase of each SLM element is identically compressed by multiplying by a constant scale factor and rotated on the complex unit-circle to produce a cancellation beam that destructively interferes with the ZOD beam. Experiments achieved a factor of 3 reduction of the ZOD beam using two different liquid-crystal SLMs. Numerical simulation analyzed the reconstructed image quality and diffraction efficiency versus degree of phase compression and showed that phase compression resulted in little image degradation or power loss.

Cold atom guidance in a capillary using blue-detuned, hollow optical modes.

We demonstrate guiding of cold 85Rb atoms through a 100-micron-diameter hollow core dielectric waveguide using cylindrical hollow modes. We have transported atoms using blue-detuned light in the 1st order, azimuthally-polarized TE01 hollow mode, and the 2nd order hollow modes (HE31, EH11, and HE12), and compared these results with guidance in the red-detuned, fundamental HE11 mode. The blue-detuned hollow modes confine atoms to low intensity along the capillary axis, far from the walls. We determine scattering rates in the guides by directly measuring the effect of recoil on the atoms. We observe higher atom numbers guided using red-detuned light in the HE11 mode, but a 10-fold reduction in scattering rate using the 2nd order modes, which have an r4 radial intensity profile to lowest order. We show that the red-detuned guides can be used to load atoms into the blue-detuned modes when both high atom number and low perturbation are desired.

Spatially resolved magnetometry using cold atoms in dark optical tweezers.

We use Faraday spectroscopy of atoms confined to crossed hollow beam tweezers to map magnetic fields over 3 millimeters with 200 micron resolution in a single trap loading cycle. The hollow beams are formed using spatial light modulation, and the trap location is scanned using acousto-optic deflectors. We demonstrate the technique by mapping a linear quadrupole magnetic field with 10 nT sensitivity.

Azimuthally and radially polarized light with a nematic SLM.

We demonstrate a technique for generating azimuthally and radially polarized beams using a nematic liquid crystal spatial light modulator and a pi phase step. The technique is similar in concept to prior techniques that interfere TEM(01) and TEM(10) laser modes, but the presented technique removes the requirement of interferometric stability. We calculate an overlap integral of >0.96 with >70% efficiency from an input Gaussian mode. The technique can easily switch between beams with azimuthal and radial polarization.

Efficient excitation of the TE(01) hollow metal waveguide mode for atom guiding.

We demonstrate excitation of the azimuthally-polarized TE(01) cylindrical waveguide mode in hollow glass and metal waveguides with 780 nm light. Experimentally, we demonstrate formation of the vectorial vortex beams, and measure attenuation lengths of the TE(01) mode in hollow optical fibers with diameters of 50-100 microns. By silver-coating the inner walls of the dielectric fibers, we demonstrate a approximately 200% increase in the attenuation length.

Cold atom Raman spectrography using velocity-selective resonances.

We have studied velocity-selective resonances in the presence of a uniform magnetic field and shown how they can be used for rapid, single-shot assessment of the ground state magnetic sublevel spectrum in a cold atomic vapor. Cold atoms are released from a magneto-optical trap in the presence of a small bias magnetic field ( approximately 300 mG) and exposed to a laser field comprised of two phase-locked counterpropagating beams connecting the two ground state hyperfine manifolds. An image of the expanded cloud shows the velocity-selected resonances as distinct features, each corresponding to specific magnetic sublevel, in a direct, intuitive manner. We demonstrate the technique with both 87Rb and 85Rb, and show the utility of the technique by optically pumping into particular magnetic sublevels. The results are shown to agree with a theoretical model, and are compared to traditional Raman spectroscopy.

A single-shot imaging magnetometer using cold atoms.

We demonstrate a technique for imaging magnetic fields using velocity-selective two-photon resonances in a cold atom cloud. Freely expanding (85)Rb atoms released from a magneto-optical trap are exposed to a brief (approximately 1 ms), off-resonant, retro-reflected laser pulse in a lin-perp-lin configuration. Two-photon resonance between magnetic sublevels occurs only for atoms in narrow velocity classes dependent on the magnetic field strength. The momentum of resonant atoms is altered by the pulse, and this two-photon momentum change is easily visible after further ballistic expansion. When the momentum pulse is applied to an atom cloud with finite size, magnetic field variations across the sample result in position-dependent features in images of the expanded cloud. We demonstrate the technique by imaging magnetic field variations over approximately 5 mm with approximately 250 microm spatial resolution.

Focusing properties of high charge number vortex laser beams.

We investigate experimentally and numerically the propagation characteristics of laser beams formed by imparting an azimuthal phase lphi to a Gaussian beam, where l is an integer. We find that when high-l beams of a finite extent are focused through a lens, the beams achieve peak intensity and are most sharply defined before and after the focal plane. Additionally, in these regions of highest intensity the effect of aberrations on the beam quality is greatly reduced, which we also demonstrate experimentally and numerically. We present a simple geometrical picture that provides excellent estimates of the beam radius and propagation distance to the plane of peak intensity.

Experimental measurements of solitary pulse characteristics from an all-normal-dispersion Yb-doped fiber laser.

We demonstrate a solitary pulse output from an 8.3-MHz mode-locked Yb-doped fiber laser, operating entirely in the normal dispersion regime. The typical output hyperbolic-secant pulses have a 14-ps pulse width and a 1.2-mW average output power. The spectrum has steep band edges with a 6.1-nm width and a tunable center wavelength between 1050 and 1080 nm. Using a frequency-resolved optical gating setup, we show that the pulse intensity and phase profiles are consistent with a chirped soliton. Energy quantization is observed, thus demonstrating the non-parabolic nature of these pulses. The laser output is compressed to near the transform limit (approximately 430 fs).