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1.
ACS EST Air ; 1(3): 200-222, 2024 Mar 08.
Article in English | MEDLINE | ID: mdl-38482269

ABSTRACT

The Alaskan Layered Pollution And Chemical Analysis (ALPACA) field experiment was a collaborative study designed to improve understanding of pollution sources and chemical processes during winter (cold climate and low-photochemical activity), to investigate indoor pollution, and to study dispersion of pollution as affected by frequent temperature inversions. A number of the research goals were motivated by questions raised by residents of Fairbanks, Alaska, where the study was held. This paper describes the measurement strategies and the conditions encountered during the January and February 2022 field experiment, and reports early examples of how the measurements addressed research goals, particularly those of interest to the residents. Outdoor air measurements showed high concentrations of particulate matter and pollutant gases including volatile organic carbon species. During pollution events, low winds and extremely stable atmospheric conditions trapped pollution below 73 m, an extremely shallow vertical scale. Tethered-balloon-based measurements intercepted plumes aloft, which were associated with power plant point sources through transport modeling. Because cold climate residents spend much of their time indoors, the study included an indoor air quality component, where measurements were made inside and outside a house to study infiltration and indoor sources. In the absence of indoor activities such as cooking and/or heating with a pellet stove, indoor particulate matter concentrations were lower than outdoors; however, cooking and pellet stove burns often caused higher indoor particulate matter concentrations than outdoors. The mass-normalized particulate matter oxidative potential, a health-relevant property measured here by the reactivity with dithiothreiol, of indoor particles varied by source, with cooking particles having less oxidative potential per mass than pellet stove particles.

2.
Environ Microbiol ; 25(12): 3364-3386, 2023 Dec.
Article in English | MEDLINE | ID: mdl-37897125

ABSTRACT

Methane-cycling is becoming more important in high-latitude ecosystems as global warming makes permafrost organic carbon increasingly available. We explored 387 samples from three high-latitudes regions (Siberia, Alaska and Patagonia) focusing on mineral/organic soils (wetlands, peatlands, forest), lake/pond sediment and water. Physicochemical, climatic and geographic variables were integrated with 16S rDNA amplicon sequences to determine the structure of the overall microbial communities and of specific methanogenic and methanotrophic guilds. Physicochemistry (especially pH) explained the largest proportion of variation in guild composition, confirming species sorting (i.e., environmental filtering) as a key mechanism in microbial assembly. Geographic distance impacted more strongly beta diversity for (i) methanogens and methanotrophs than the overall prokaryotes and, (ii) the sediment habitat, suggesting that dispersal limitation contributed to shape the communities of methane-cycling microorganisms. Bioindicator taxa characterising different ecological niches (i.e., specific combinations of geographic, climatic and physicochemical variables) were identified, highlighting the importance of Methanoregula as generalist methanogens. Methylocystis and Methylocapsa were key methanotrophs in low pH niches while Methylobacter and Methylomonadaceae in neutral environments. This work gives insight into the present and projected distribution of methane-cycling microbes at high latitudes under climate change predictions, which is crucial for constraining their impact on greenhouse gas budgets.


Subject(s)
Euryarchaeota , Microbiota , Microbiota/genetics , Euryarchaeota/genetics , Wetlands , Soil/chemistry , Methane
3.
Sci Data ; 9(1): 674, 2022 Nov 04.
Article in English | MEDLINE | ID: mdl-36333353

ABSTRACT

High latitudes are experiencing intense ecosystem changes with climate warming. The underlying methane (CH4) cycling dynamics remain unresolved, despite its crucial climatic feedback. Atmospheric CH4 emissions are heterogeneous, resulting from local geochemical drivers, global climatic factors, and microbial production/consumption balance. Holistic studies are mandatory to capture CH4 cycling complexity. Here, we report a large set of integrated microbial and biogeochemical data from 387 samples, using a concerted sampling strategy and experimental protocols. The study followed international standards to ensure inter-comparisons of data amongst three high-latitude regions: Alaska, Siberia, and Patagonia. The dataset encompasses different representative environmental features (e.g. lake, wetland, tundra, forest soil) of these high-latitude sites and their respective heterogeneity (e.g. characteristic microtopographic patterns). The data included physicochemical parameters, greenhouse gas concentrations and emissions, organic matter characterization, trace elements and nutrients, isotopes, microbial quantification and composition. This dataset addresses the need for a robust physicochemical framework to conduct and contextualize future research on the interactions between climate change, biogeochemical cycles and microbial communities at high-latitudes.


Subject(s)
Greenhouse Gases , Microbiota , Carbon Dioxide/analysis , Methane/analysis , Soil , Wetlands
4.
Waste Manag ; 121: 373-382, 2021 Feb 15.
Article in English | MEDLINE | ID: mdl-33422924

ABSTRACT

A previously developed surface probe method, which allows for instantaneous methane (CH4) flux measurement, was used to establish CH4 emission maps of a municipal landfill with a final clay cover and equipped with a gas recollection system. In addition to spatial variations, the method was applied at 7 different times over a total timeframe of 65 h and under similar weather conditions to determine the intrinsic temporal variations of CH4 emissions; i.e., the temporal variation related to the dynamic of the landfill rather than the one driven by external factors. Furthermore, continuous CH4 fluxes, with a data acquisition frequency of 1 Hz, were measured during 12 h at a single position, and for one hour at 22 locations of the landfill, spanning a large range of CH4 emission magnitudes. A simple model for the numerical characterization of spatiotemporal variability of the landfill emission was used and allowed us to separately quantify the temporal and spatial variability. This model showed that, in the landfill tested, the temporal distribution of CH4 emissions resulted more homogeneous than the spatial distribution. Other attributes of the temporal and spatial distributions of CH4 emissions were also established including the anisotropic nature of the spatial distribution and, contrastingly, the stochastic temporal variability of such emissions.


Subject(s)
Air Pollutants , Refuse Disposal , Air Pollutants/analysis , Methane/analysis , Waste Disposal Facilities
5.
Rev Sci Instrum ; 90(7): 075005, 2019 Jul.
Article in English | MEDLINE | ID: mdl-31370483

ABSTRACT

Electric motors are being investigated in-depth for their application in aerospace. Part of this investigation is the characterization of the loadings from the propulsion devices, in a stationary setup, usually accomplished through the utilization of load cells. The majority of the load cells used in this application are designed around a resistance-based strain gauge. However, electric motors radiate electromagnetic interference (EMI) when in operation, which degrades the signal retrieved through the strain gauge, due to the gauge's metallic construction acting as an antenna for the EMI. To demonstrate the advantage of fiber Bragg gratings (FBGs), with their immunity to EMI, a load cell implementing both sensor technologies was designed and subjected to the same mechanical loading and EMI, with a flywheel coupled to a brushless DC motor. The load cell had a sensitivity of 8.59 ± 0.18 N and 2.49 ± 2.49 N through the strain gauge and FBG system, respectively. The strain gauge signal contained the mechanical loading signal embedded in wideband noise and spikes (that increased linearly with motor angular velocity), while the FBG signal did not, with little noise. The raw strain gauge signal, at a maximum, had a signal power ratio (mechanical signal power divided by the overall signal power mean) of 21.06 at 104.72 rad/s; the FBG signal, at a minimum, had a signal power ratio of 40.09 at 52.36 rad/s. Therefore, on the basis of the mechanical tests performed in this work, the recommended sensor of choice for electric propulsion in aerospace applications is the FBG.

7.
PLoS One ; 10(9): e0137209, 2015.
Article in English | MEDLINE | ID: mdl-26368123

ABSTRACT

As the acreages of agricultural lands increase, changes in surface energetics and evapotranspiration (ET) rates may arise consequently affecting regional climate regimes. The objective of this study was to evaluate summertime ET dynamics and surface energy processes in a subarctic agricultural farm in Interior Alaska. The study includes micrometeorological and hydrological data. Results covering the period from June to September 2012 and 2013 indicated consistent energy fractions: LE/Rnet (67%), G/Rnet (6%), H/Rnet (27%) where LE is latent heat flux, Rnet is the surface net radiation, G is ground heat flux and H is the sensible heat flux. Additionally actual surface evapotranspiration from potential evaporation was found to be in the range of 59 to 66%. After comparing these rates with those of most prominent high latitude ecosystems it is argued here that if agroecosystem in high latitudes become an emerging feature in the land-use, the regional surface energy balance will significantly shift in comparison to existing Arctic natural ecosystems.


Subject(s)
Agriculture , Ecosystem , Plant Transpiration , Water Cycle , Alaska , Arctic Regions , Climate , Meteorological Concepts
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