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1.
Nat Geosci ; 16(7): 577-583, 2023.
Article in English | MEDLINE | ID: mdl-37441270

ABSTRACT

Future increases in stratospheric water vapour risk amplifying climate change and slowing down the recovery of the ozone layer. However, state-of-the-art climate models strongly disagree on the magnitude of these increases under global warming. Uncertainty primarily arises from the complex processes leading to dehydration of air during its tropical ascent into the stratosphere. Here we derive an observational constraint on this longstanding uncertainty. We use a statistical-learning approach to infer historical co-variations between the atmospheric temperature structure and tropical lower stratospheric water vapour concentrations. For climate models, we demonstrate that these historically constrained relationships are highly predictive of the water vapour response to increased atmospheric carbon dioxide. We obtain an observationally constrained range for stratospheric water vapour changes per degree of global warming of 0.31 ± 0.39 ppmv K-1. Across 61 climate models, we find that a large fraction of future model projections are inconsistent with observational evidence. In particular, frequently projected strong increases (>1 ppmv K-1) are highly unlikely. Our constraint represents a 50% decrease in the 95th percentile of the climate model uncertainty distribution, which has implications for surface warming, ozone recovery and the tropospheric circulation response under climate change.

2.
Nature ; 549(7671): 211-218, 2017 09 13.
Article in English | MEDLINE | ID: mdl-28905899

ABSTRACT

As a result of the 1987 Montreal Protocol and its amendments, the atmospheric loading of anthropogenic ozone-depleting substances is decreasing. Accordingly, the stratospheric ozone layer is expected to recover. However, short data records and atmospheric variability confound the search for early signs of recovery, and climate change is masking ozone recovery from ozone-depleting substances in some regions and will increasingly affect the extent of recovery. Here we discuss the nature and timescales of ozone recovery, and explore the extent to which it can be currently detected in different atmospheric regions.

3.
Earth Syst Sci Data ; 8(2): 461-490, 2016.
Article in English | MEDLINE | ID: mdl-28966693

ABSTRACT

In this paper, we describe the construction of the Stratospheric Water and Ozone Satellite Homogenized (SWOOSH) database, which includes vertically resolved ozone and water vapor data from a subset of the limb profiling satellite instruments operating since the 1980s. The primary SWOOSH products are zonal-mean monthly-mean time series of water vapor and ozone mixing ratio on pressure levels (12 levels per decade from 316 to 1 hPa). The SWOOSH pressure level products are provided on several independent zonal-mean grids (2.5, 5, and 10°), and additional products include two coarse 3-D griddings (30° long × 10° lat, 20° × 5°) as well as a zonal-mean isentropic product. SWOOSH includes both individual satellite source data as well as a merged data product. A key aspect of the merged product is that the source records are homogenized to account for inter-satellite biases and to minimize artificial jumps in the record. We describe the SWOOSH homogenization process, which involves adjusting the satellite data records to a "reference" satellite using coincident observations during time periods of instrument overlap. The reference satellite is chosen based on the best agreement with independent balloon-based sounding measurements, with the goal of producing a long-term data record that is both homogeneous (i.e., with minimal artificial jumps in time) and accurate (i.e., unbiased). This paper details the choice of reference measurements, homogenization, and gridding process involved in the construction of the combined SWOOSH product and also presents the ancillary information stored in SWOOSH that can be used in future studies of water vapor and ozone variability. Furthermore, a discussion of uncertainties in the combined SWOOSH record is presented, and examples of the SWOOSH record are provided to illustrate its use for studies of ozone and water vapor variability on interannual to decadal timescales. The version 2.5 SWOOSH data are publicly available at doi:10.7289/V5TD9VBX.

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