Fluorescence decay enhancement and FRET inhibition in self-assembled hybrid gold CdSe/CdS/CdZnS colloidal nanocrystal supraparticles.

We report on the synthesis of hybrid light emitting particles with a diameter ranging between 100 and 500 nm, consisting in a compact semiconductor CdSe/CdS/CdZnS nanocrystal aggregate encapsulated by a controlled nanometric size silica and gold layers. We first characterize the Purcell decay rate enhancement corresponding to the addition of the gold nanoshell as a function of the particle size and find a good agreement with the predictions of numerical simulations. Then, we show that the contribution corresponding to Förster resonance energy transfer is inhibited.

Electromagnetic analysis for optical coherence tomography based through silicon vias metrology.

This paper reports on progress in the analysis of time-domain optical coherence tomography (OCT) applied to the dimensional metrology of through-silicon vias (TSVs), which are vertical interconnect accesses in silicon, enabling three-dimensional (3D) integration in microelectronics, and estimates the deviations from earlier, simpler models. The considered TSV structures are 1D trenches and circular holes etched into silicon with a large aspect ratio. As a prerequisite for a realistic modeling, we work with spectra obtained from reference interferograms measured at a planar substrate, which fully includes the dispersion of the OCT apparatus. Applying a rigorous modal approach, we estimate the differences to a pure ray tracing technique. Accelerating our computations, we focus on the relevant fundamental modes and apply a Fabry-Perot model as an efficient approximation. Exploiting our results, we construct and present an iterative procedure based on the minimization of a merit function, which concludes TSV heights reliably, accurately, and rapidly from measured interferograms.

Quasinormal mode solvers for resonators with dispersive materials.

Optical resonators are widely used in modern photonics. Their spectral response and temporal dynamics are fundamentally driven by their natural resonances, the so-called quasinormal modes (QNMs), with complex frequencies. For optical resonators made of dispersive materials, the QNM computation requires solving a nonlinear eigenvalue problem. This raises a difficulty that is only scarcely documented in the literature. We review our recent efforts for implementing efficient and accurate QNM solvers for computing and normalizing the QNMs of micro- and nanoresonators made of highly dispersive materials. We benchmark several methods for three geometries, a two-dimensional plasmonic crystal, a two-dimensional metal grating, and a three-dimensional nanopatch antenna on a metal substrate, with the perspective to elaborate standards for the computation of resonance modes.

Broad working bandwidth and "endlessly" single-mode guidance within hybrid silicon photonics.

The successes of nonlinear photonics and hybrid silicon photonics with a growing variety of functional materials entail ever-enlarging bandwidths. It is best exemplified by parametric comb frequency generation. Such operation challenges the dielectric channel waveguide as the basis for guidance, because of the adverse advent of higher order modes at short wavelengths. Surprisingly, the popular mechanism of endlessly single-mode guidance [Opt. Lett.22, 961 (1997).] operating in photonic crystal fibers has not been transposed within silicon photonics yet. We outline here the strategy and potential of this approach within planar and hybrid silicon photonics, whereby in-plane and vertical confinement are shown to be amenable to near-single-mode behavior in the typical silicon band, i.e., λ=1.1 µm to ∼5 µm.

Design of highly efficient metallo-dielectric patch antennas for single-photon emission.

Quantum emitters such as NV-centers or quantum dots can be used as single-photon sources. To improve their performance, they can be coupled to microcavities or nano-antennas. Plasmonic antennas offer an appealing solution as they can be used with broadband emitters. When properly designed, these antennas funnel light into useful modes, increasing the emission rate and the collection of single-photons. Yet, their inherent metallic losses are responsible for very low radiative efficiencies. Here, we introduce a new design of directional, metallo-dielectric, optical antennas with a Purcell factor of 150, a total efficiency of 74% and a collection efficiency of emitted photons of 99%.

Efficient and intuitive method for the analysis of light scattering by a resonant nanostructure.

We present a semi-analytical formalism capable of handling the coupling of electromagnetic sources, such as point dipoles or free-propagating fields, with various kinds of dissipative resonances with radiation leakage, Ohmic losses or both. Due to its analyticity, the approach is very intuitive and physically-sound. It is also very economic in computational resources, since once the resonances of a plasmonic or photonic resonator are known, their excitation coefficients are obtained analytically, independently of the polarization, frequency or location of the excitation source. To evidence that the present formalism is very general and versatile, we implement it with the commercial software COMSOL, rather than with our in-house numerical tools.

Confined Tamm plasmon lasers.

We demonstrate that confined Tamm plasmon modes can be advantageously exploited for the realization of new kind of metal/semiconductor lasers. Laser emission is demonstrated for Tamm structures with various diameters of the metallic disks which provide the confinement. A reduction of the threshold with the size is observed. The competition between the acceleration of the spontaneous emission and the increase of the losses leads to an optimal size, which is in good agreement with calculations.

Controlling spontaneous emission with plasmonic optical patch antennas.

We experimentally demonstrate the control of the spontaneous emission rate and the radiation pattern of colloidal quantum dots deterministically positioned in a plasmonic patch antenna. The antenna consists of a thin gold microdisk separated from a planar gold layer by a few tens of nanometers thick dielectric layer. The emitters are shown to radiate through the entire patch antenna in a highly directional and vertical radiation pattern. Strong acceleration of spontaneous emission is observed, depending on the antenna geometry. Considering the double dipole structure of the emitters, this corresponds to a Purcell factor up to 80 for dipoles perpendicular to the disk.

Theory of the spontaneous optical emission of nanosize photonic and plasmon resonators.

We provide a self-consistent electromagnetic theory of the coupling between dipole emitters and dissipative nanoresonators. The theory that relies on the concept of quasinormal modes with complex frequencies provides an accurate closed-form expression for the electromagnetic local density of states of any photonic or plasmonic resonator with strong radiation leakage, absorption, and material dispersion. It represents a powerful tool to calculate and conceptualize the electromagnetic response of systems that are governed by a small number of resonance modes. We use the formalism to revisit Purcell's factor. The new formula substantially differs from the usual one; in particular, it predicts that a spectral detuning between the emitter and the resonance does not necessarily result in a Lorentzian response in the presence of dissipation. Comparisons with fully vectorial numerical calculations for plasmonic nanoresonators made of gold nanorods evidence the high accuracy of the predictions achieved by our semianalytical treatment.

Statistical fluctuations of transmission in slow light photonic-crystal waveguides.

We report statistical fluctuations for the transmissions of a series of photonic-crystal waveguides (PhCWs) that are supposedly identical and that only differ because of statistical structural fabrication-induced imperfections. For practical PhCW lengths offering tolerable -3dB attenuation with moderate group indices (n(g) approximately 60), the transmission spectra contains very narrow peaks (Q approximately 20,000) that vary from one waveguide to another. The physical origin of the peaks is explained by calculating the actual electromagnetic-field pattern inside the waveguide. The peaks that are observed in an intermediate regime between the ballistic and localization transports are responsible for a smearing of the local density of states, for a rapid broadening of the probability density function of the transmission, and bring a severe constraint on the effective use of slow light for on-chip optical information processing. The experimental results are quantitatively supported by theoretical results obtained with a coupled-Bloch-mode approach that takes into account multiple scattering and localization effects.

Metal-coated nanocylinder cavity for broadband nonclassical light emission.

A novel metal-coated nanocylinder-cavity architecture fully compatible with III-V GaInAs technology and benefiting from a broad spectral range enhancement of the local density of states is proposed as an integrated source of nonclassical light. Because of a judicious selection of the mode volume, the cavity combines good collection efficiency (≈45%), large Purcell factors (≈15) over a 80 nm spectral range, and a low sensitivity to inevitable spatial mismatches between the single emitter and the cavity mode. This represents a decisive step towards the implementation of reliable solid-state devices for the generation of entangled photon pairs at infrared wavelengths.

Loss engineered slow light waveguides.

Slow light devices such as photonic crystal waveguides (PhCW) and coupled resonator optical waveguides (CROW) have much promise for optical signal processing applications and a number of successful demonstrations underpinning this promise have already been made. Most of these applications are limited by propagation losses, especially for higher group indices. These losses are caused by technological imperfections ("extrinsic loss") that cause scattering of light from the waveguide mode. The relationship between this loss and the group velocity is complex and until now has not been fully understood. Here, we present a comprehensive explanation of the extrinsic loss mechanisms in PhC waveguides and address some misconceptions surrounding loss and slow light that have arisen in recent years. We develop a theoretical model that accurately describes the loss spectra of PhC waveguides. One of the key insights of the model is that the entire hole contributes coherently to the scattering process, in contrast to previous models that added up the scattering from short sections incoherently. As a result, we have already realised waveguides with significantly lower losses than comparable photonic crystal waveguides as well as achieving propagation losses, in units of loss per unit time (dB/ns) that are even lower than those of state-of-the-art coupled resonator optical waveguides based on silicon photonic wires. The model will enable more advanced designs with further loss reduction within existing technological constraints.

Disorder-induced multiple scattering in photonic-crystal waveguides.

In this Letter, we study slow-light transport in photonic-crystal waveguides in the presence of structural imperfections. In contrast with previous theoretical works that rely on perturbation theories, the present formalism takes into account multiple scattering and localization effects. It allows for a quantitative prediction of the main statistical transport coefficients, including averaged values as well as probability distributions. In particular, we evidence that, as the group velocity decreases, the attenuation probability distribution exhibits a rapid broadening that one should consider for designing slow-light devices.

Solid-state single photon sources: the nanowire antenna.

We design several single-photon-sources based on the emission of a quantum dot embedded in a semiconductor (GaAs) nanowire. Through various taper designs, we engineer the nanowire ends to realize efficient metallic-dielectric mirrors and to reduce the divergence of the far-field radiation diagram. Using fully-vectorial calculations and a comprehensive Fabry-Perot model, we show that various realistic nanowire geometries may act as nanoantennas (volume of approximately 0.05 lambda(3)) that assist funnelling the emitted photons into a single monomode channel. Typically, very high extraction efficiencies above 90% are predicted for a collection optics with a numerical aperture NA=0.85. In addition, since no frequency-selective effect is used in our design, this large efficiency is achieved over a remarkably broad spectral range, Deltalambda=70 nm at lambda=950 nm.

Efficient photonic mirrors for semiconductor nanowires.

Using a fully vectorial frequency-domain aperiodic Fourier modal method, we study nanowire metallic mirrors and their photonic performance. We show that the performance of standard quarter-wave Bragg mirrors at subwavelength diameters is surprisingly poor, while engineered metallic mirrors that incorporate a thin dielectric adlayer may offer reflectance larger than 90% even for diameters as small as lambda/5.

Hybridization of electromagnetic numerical methods through the G-matrix algorithm.

For the sake of numerical performance, we hybridize two common approaches often used in electromagnetic computations, namely the finite-element method and the aperiodic Fourier modal method. To that end, we propose an extension of the classical S-matrix formalism to numerical situations, which requires handling different mathematical representations of the electromagnetic fields. As shown with a three-dimensional example, the proposed G-matrix formalism is stable and allows for an enhanced performance in terms of numerical accuracy and efficiency.

Coupling into slow-mode photonic crystal waveguides.

We study efficient injectors for coupling light from z-invariant ridge waveguides into slow Bloch modes of single-row defect photonic crystal waveguides. Two-dimensional vectorial computations performed with a Bloch mode theory approach predict that very high efficiencies (>90%) can be achieved for injector lengths of only a few wavelengths in length, even for small group velocities in the range of c/100-c/400. This result suggests that photonic crystal devices operating with slow waves can be interfaced with classical waveguides without sacrificing compactness.

Very large spontaneous-emission Beta factors in photonic-crystal waveguides.

Through a new rigorous Bloch-mode formalism, we theoretically study the generation of photons in single-row-defect photonic-crystal waveguides. In contrast with previous related works relying on a reinforcement of the spontaneous emission (SE) through microcavity effects, we explore situations for which the SE into radiation modes is reduced to a very low level while the SE into the guided mode is maintained at a level comparable to that in the bulk material. Remarkably large SE beta factors in excess of 95% are obtained, and since no resonance effect is involved, this efficiency is achieved over a 40-nm-large spectral interval at lambda approximately 950 nm.

Near-field analysis of surface waves launched at nanoslit apertures.

With the aim of analyzing the properties of the waves that are scattered by nanoslits on metallic surfaces, we provide a direct observation of the near-field in a slit-doublet experiment at optical wavelengths. We show that two distinct waves are involved: a surface plasmon polariton and another wave with a free-space character. From the recorded data, we have extracted the amplitudes and phases of these waves, their damping characteristic lengths and their relative weights as a function of the separation distance from the slit. The analysis is fully supported by a quantitative agreement with vector-theory computational results.

Compact and efficient injection of light into band-edge slow-modes.

We design compact (a few wavelength long) and efficient (>99%) injectors for coupling light into slow Bloch modes of periodic thin film stacks and of periodic slab waveguides. The study includes the derivation of closed-form expressions for the injection efficiency as a function of the group-velocity of injected light, and the proof that 100% coupling efficiencies for arbitrary small group velocities is possible with an injector length scaling as log(c/vg). The trade-off between the injector bandwidth and the group velocity of the injected light is also considered.