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1.
Proc Natl Acad Sci U S A ; 118(7)2021 Feb 16.
Article in English | MEDLINE | ID: mdl-33563764

ABSTRACT

A central question in the underdoped cuprates pertains to the nature of the pseudogap ground state. A conventional metallic ground state of the pseudogap region has been argued to host quantum oscillations upon destruction of the superconducting order parameter by modest magnetic fields. Here, we use low applied measurement currents and millikelvin temperatures on ultrapure single crystals of underdoped [Formula: see text] to unearth an unconventional quantum vortex matter ground state characterized by vanishing electrical resistivity, magnetic hysteresis, and nonohmic electrical transport characteristics beyond the highest laboratory-accessible static fields. A model of the pseudogap ground state is now required to explain quantum oscillations that are hosted by the bulk quantum vortex matter state without experiencing sizable additional damping in the presence of a large maximum superconducting gap; possibilities include a pair density wave.

2.
Proc Natl Acad Sci U S A ; 117(23): 12707-12712, 2020 Jun 09.
Article in English | MEDLINE | ID: mdl-32457161

ABSTRACT

The dielectric and magnetic polarizations of quantum paraelectrics and paramagnetic materials have in many cases been found to initially increase with increasing thermal disorder and hence, exhibit peaks as a function of temperature. A quantitative description of these examples of "order-by-disorder" phenomena has remained elusive in nearly ferromagnetic metals and in dielectrics on the border of displacive ferroelectric transitions. Here, we present an experimental study of the evolution of the dielectric susceptibility peak as a function of pressure in the nearly ferroelectric material, strontium titanate, which reveals that the peak position collapses toward absolute zero as the ferroelectric quantum critical point is approached. We show that this behavior can be described in detail without the use of adjustable parameters in terms of the Larkin-Khmelnitskii-Shneerson-Rechester (LKSR) theory, first introduced nearly 50 y ago, of the hybridization of polar and acoustic modes in quantum paraelectrics, in contrast to alternative models that have been proposed. Our study allows us to construct a detailed temperature-pressure phase diagram of a material on the border of a ferroelectric quantum critical point comprising ferroelectric, quantum critical paraelectric, and hybridized polar-acoustic regimes. Furthermore, at the lowest temperatures, below the susceptibility maximum, we observe a regime characterized by a linear temperature dependence of the inverse susceptibility that differs sharply from the quartic temperature dependence predicted by the LKSR theory. We find that this non-LKSR low-temperature regime cannot be accounted for in terms of any detailed model reported in the literature, and its interpretation poses an empirical and conceptual challenge.

3.
Rep Prog Phys ; 75(10): 102501, 2012 Oct.
Article in English | MEDLINE | ID: mdl-22986620

ABSTRACT

We survey recent experimental results including quantum oscillations and complementary measurements probing the electronic structure of underdoped cuprates, and theoretical proposals to explain them. We discuss quantum oscillations measured at high magnetic fields in the underdoped cuprates that reveal a small Fermi surface section, comprising quasiparticles that obey Fermi-Dirac statistics, unaccompanied by other states of comparable thermodynamic mass at the Fermi level. The location of the observed Fermi surface section at the nodes is indicated by a body of evidence including the collapse in Fermi velocity measured by quantum oscillations, which is found to be associated with the nodal density of states observed in angular resolved photoemission, the persistence of quantum oscillations down to low fields in the vortex state, the small value of density of states from heat capacity and the multiple frequency quantum oscillation pattern consistent with nodal magnetic breakdown of bilayer-split pockets. A nodal Fermi surface pocket is further consistent with the observation of a density of states at the Fermi level concentrated at the nodes in photoemission experiments, and the antinodal pseudogap observed by photoemission, optical conductivity, nuclear magnetic resonance (NMR) Knight shift, as well as other complementary diffraction, transport and thermodynamic measurements. One of the possibilities considered is that the small Fermi surface pockets observed at high magnetic fields can be understood in terms of Fermi surface reconstruction by a form of small wavevector charge order, observed over long lengthscales in experiments such as NMR and x-ray scattering, potentially accompanied by an additional mechanism to gap the antinodal density of states.


Subject(s)
Copper/chemistry , Models, Chemical , Technetium/chemistry , Electric Conductivity
4.
Philos Trans A Math Phys Eng Sci ; 369(1941): 1687-711, 2011 Apr 28.
Article in English | MEDLINE | ID: mdl-21422021

ABSTRACT

We review recent progress in the study of quantum oscillations as a tool for uniquely probing low-energy electronic excitations in high-T(c) cuprate superconductors. Quantum oscillations in the underdoped cuprates reveal that a close correspondence with Landau Fermi-liquid behaviour persists in the accessed regions of the phase diagram, where small pockets are observed. Quantum oscillation results are viewed in the context of momentum-resolved probes such as photoemission, and evidence examined from complementary experiments for potential explanations for the transformation from a large Fermi surface into small sections. Indications from quantum oscillation measurements of a low-energy Fermi surface instability at low dopings under the superconducting dome at the metal-insulator transition are reviewed, and potential implications for enhanced superconducting temperatures are discussed.

5.
J Phys Condens Matter ; 21(1): 012208, 2009 Jan 07.
Article in English | MEDLINE | ID: mdl-21817209

ABSTRACT

We report the discovery of superconductivity at high pressure in SrFe(2)As(2) and BaFe(2)As(2). The superconducting transition temperatures are up to 27 K in SrFe(2)As(2) and 29 K in BaFe(2)As(2), the highest obtained for materials with pressure-induced superconductivity thus far.

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