Direct generation of multicolor Bessel beams from a Pr3+: WPFG fiber laser.

Multicolor visible high-order Bessel (Bessel-vortex) beams which have a helical wavefront and a long confocal length have garnered significant interest for applications in materials processing and biomedical technologies. In this paper, we demonstrate the direct generation of multicolor (523, 605 and 637 nm) Bessel-vortex beams from a Pr3+-doped water-proof fluoro-aluminate glass (Pr3+: WPFG) fiber laser with an intracavity lens which induces chromatic and spherical aberration. The handedness of the generated Bessel-vortex beam is selectively controlled through lateral displacement of the intra-cavity lens.

Creation of galaxy-shaped vortex relief structures in azo-polymers with petal-like beams.

We demonstrate the formation of surface relief structures in azo-polymers which exhibit multiple spiral arms, through irradiation of a rotating petal-like beam formed by the coherent superposition of Laguerre-Gaussian modes with opposite handedness. Intriguingly, the fabricated relief structures reflect full geometric parameters of the irradiated petal beam, such as handedness, topological charge, initial azimuthal phase and even ellipticity, corresponding to azimuthal and polar angles along equator and meridian planes of an orbital Poincaré sphere. The handedness, or direction of rotation, of the fabricated structures with multiple spiral arms could be controlled via the rotation and polarization directions of the irradiating laser field. This effect highlights an exotic coupling between the optical intensity gradient induced mass transport of the irradiated material and the spin angular momentum characteristics of the irradiating optical field. The azimuthal orientation of the surface relief structures could also be tuned by altering the initial relative phase between the coherently superposed Laguerre-Gaussian modes with opposite handedness, constituting the irradiating petal laser field. This work offers new insights into fundamental interactions which occur between light and matter, and we believe, will pave the way towards advanced technologies, such as ultrahigh density optical data storage.

Cascaded vector vortex mode generation from a solid-state Raman laser.

Cascaded vector vortex mode generation from a Ba(NO3)2 Raman laser cavity pumped by a vector LG0,2 green laser was demonstrated for the first time to our knowledge. The generated Stokes outputs exhibited a second-order vector vortex beam as evidenced by linearly polarized flower-shaped spatial forms with four petals. The achieved optical conversion efficiencies of the first, second, and third Stokes outputs were 6.59%, 4.22%, and 0.11%, respectively, at a maximum pump energy of 3.6 mJ (360 mW).

Broadband high-resolution terahertz single-pixel imaging.

We report a simple single-pixel imaging system with a low mean squared error in the entire terahertz frequency region (3-13 THz) that employs a thin metallic ring with a series of directly perforated random masks and a subpixel mask digitization technique. This imaging system produces high pixel resolution reconstructed images, up to 1200 × 1200 pixels, and imaging area of 32 × 32 mm2. It can be extended to develop advanced imaging systems in the near-ultraviolet to terahertz region.

Direct generation of 1108†nm and 1173†nm Laguerre-Gaussian modes from a self-Raman Nd:GdVO4 laser.

We demonstrate a continuous-wave self-Raman Nd:GdVO4 Laguerre-Gaussian (LG) mode laser based on different Raman shifts of 382 cm-1 and 882 cm-1 by shaping the pumping beam with the use of an axicon lens and a focusing lens. Selective generation of LG mode beams at 1108 nm or 1173 nm, or simultaneously 1108 nm and 1173 nm, was achieved by carefully adjusting the alignment of the laser cavity. The maximum Raman LG mode output powers at the wavelengths of 1108 nm (the first-Stokes emission of the 382 cm-1 Raman shift) and 1173 nm (the first-Stokes emission of the 882 cm-1 Raman shift) were measured to be 49.8 mW and 133.4 mW at the absorbed pump power of 5.69 W, respectively. The generated LG modes, formed via the incoherent superposition of two LG mode beams with positive and negative topological charges, carry zero orbital angular momentum. Such LG mode laser sources have the potential to fill in the wavelength gap of lasers in the visible and infrared regions.

Zero-spindle spectral drill: real-time spectral measurement in a fixed Fabry-Pérot cavity.

An optical configuration for Fabry-Pérot cavity scanning using a geometric phase shifter, known as the "spectral drill," is improved to acquire a spectrum in real-time. Previously, the resonance condition of the spectral drill is swept by the mechanical rotation of a phase plate comprising a geometric phase shifter, and the acquisition time is limited. In this work, using a q-plate and a camera instead of phase plate rotation and a photo detector, we remove all the spinning mechanics and increase the acquisition rate by a factor 720. This technique will be applied to locking laser frequency.

Photopolymerization with high-order Bessel light beams.

We study photopolymerization with high-order Bessel light beams with phase singularities on-axis. Self-trapping and self-focusing of propagation-invariant light beams in a photopolymer allow the fabrication of extended helical microfibers with a length scale of a centimeter, which is more than an order of magnitude larger than the propagation distance of the Bessel light beams. We show the evolution of microfibers rotating at a rate proportional to the incident optical power, while the periodicity of the helical structures remains constant, irrespective of the laser power. This suggests that optical momentum transfer plays a predominant role in the growth and rotation of such fiber structures.

Investigation of laser-induced-metal phase of MoTe2 and its contact property via scanning gate microscopy.

Although semiconductor to metal phase transformation of MoTe2 by high-density laser irradiation of more than 0.3 MW cm-2 has been reported, we reveal that the laser-induced-metal (LIM) phase is not the 1T' structure derived by a polymorphic-structural phase transition but consists instead of semi-metallic Te induced by photo-thermal decomposition of MoTe2. The technique is used to fabricate a field effect transistor with a Pd/2H-MoTe2/LIM structure having an asymmetric metallic contact, and its contact properties are studied via scanning gate microscopy. We confirm that a Schottky barrier (a diffusion potential) is always formed at the Pd/2H-MoTe2 boundary and obstacles a carrier transport while an Ohmic contact is realized at the 2H-MoTe2/LIM phase junction for both n- and p-type carriers.

Generation of coupled orbital angular momentum modes from an optical vortex parametric laser source.

We report on the generation of flower (wheel) modes, which manifest coupled orbital angular momentum (OAM) modes, from a vortex pumped optical parametric oscillator simply by employing a pump source with a short temporal coherence time. This vortex oscillator was also developed to generate a further higher-order vortex signal output with ℓs=2-4 by replacement of the pump source with a longer coherence time. The signal and idler outputs were tuned within wavelength ranges of 745-955 nm and 1200-1855 nm, respectively. The maximum signal output energy of 1.2 mJ was measured with an optical efficiency of 15.6%.

Optical vortex-induced forward mass transfer: manifestation of helical trajectory of optical vortex.

The orbital angular momentum of an optical vortex field is found to twist high viscosity donor material to form a micron-scale 'spin jet'. This unique phenomenon manifests the helical trajectory of the optical vortex. Going beyond both the conventional ink jet and laser induced forward mass transfer (LIFT) patterning technologies, it also offers the formation and ejection of a micron-scale 'spin jet' of the donor material even with an ultrahigh viscosity of 4 Pa·s. This optical vortex laser induced forward mass transfer (OV-LIFT) patterning technique will enable the development of next generation printed photonic/electric/spintronic circuits formed of ultrahigh viscosity donor dots containing functional nanoparticles, such as quantum dots, metallic particles and magnetic ferrite particles, with ultrahigh spatial resolution. It can also potentially explore a completely new needleless drug injection.

Generation of high-quality terahertz OAM mode based on soft-aperture difference frequency generation.

We demonstrate the generation of high-quality tunable terahertz (THz) vortices in an eigenmode by employing soft-aperture difference frequency generation of vortex and Gaussian modes. The generated THz vortex output exhibits a high-quality orbital angular momentum (OAM) mode with a topological charge of ℓTHz = ±1 in a frequency range of 2-6 THz. The maximum average power of the THz vortex output obtained was ∼3.3 µW at 4 THz.

Direct generation of red and orange optical vortex beams from an off-axis diode-pumped Pr3+:YLF laser.

We demonstrate the direct generation of visible vortex beams at 640 nm and 607 nm by employing an off-axis pumping scheme in a diode end-pumped Pr3+:YLF laser. A detailed numerical analysis, based on the coherent superposition of Hermite-Gaussian modes with different amplitudes and phases, is perfectly consistent with the experimentally observed lasing modes. The maximum vortex output powers have been measured to be 808 mW and 211 mW at a pump power of 3.16 W, for the wavelengths of 640 nm and 607 nm, respectively. We also demonstrate the handedness control of the generated vortex beam. Such a visible vortex laser can potentially be applied in super-resolution fluorescent microscopes and micro-fabrication research.

Nanoscale chiral surface relief of azo-polymers with nearfield OAM light.

An optical vortex with orbital angular momentum (OAM) can be used to induce microscale chiral structures in various materials. Such chiral structures enable the generation of a nearfield vortex, i.e. nearfield OAM light on a sub-wavelength scale, thereby leading to further nanoscale mass-transport. We report on the formation of a nanoscale chiral surface relief in azo-polymers due to nearfield OAM light. The resulting nanoscale chiral relief exhibits a diameter of ca. 400 nm, which corresponds to less than 1/5-1/6th of the original chiral structure (ca. 2.1 µm). Such a nanoscale chiral surface relief is established by the simple irradiation of uniform visible plane-wave light with an intensity of <500 mW/cm2.

Ultra-widely tunable mid-infrared (6-18 µm) optical vortex source.

We demonstrate the generation of an ultra-widely tunable mid-infrared (6-18 µm) optical vortex output with a moderate pulse energy from a AgGaSe2 difference frequency generator pumped by an optical vortex parametric oscillator. The handedness of the vortex output can be controlled/selected by swapping the lasing frequencies of the signal and idler outputs and rotating the AgGaSe2 crystal by 90 deg.

Tunable near-infrared optical vortex parametric laser with versatile orbital angular momentum states.

We demonstrate a tunable vortex laser with versatile orbital angular momentum (OAM) states based on a singly resonant optical parametric oscillator formed of a noncritical phase-matching LiB3O5 crystal. The selective generation of a signal (idler) output with three OAMs, including an upconverted (negative) OAM, is achieved simply by appropriate shortening (or extending) of the cavity. The compact cavity configuration also allows for the generation of the signal (idler) output with various OAMs by simply tuning the signal wavelength. The vortex output is tuned within the wavelength region of 0.74 to 1.84 µm with a maximum pulse energy of 2.16 mJ from a pump energy of 9.3 mJ.

Ultraviolet optical vortex generation using a pair of ß-BaB2O4 crystals with inverted orientations.

Picosecond pulsed frequency-doubled optical vortices were generated using a pair of ß-BaB2O4 crystals with their c axes inverted. This arrangement produced high-quality ultraviolet vortex output with low spatial separation of the phase singularity at a conversion efficiency of ∼40%. We also discuss the theoretical spatial form and beam propagation of the ultraviolet vortex output.

Azo-polymer film twisted to form a helical surface relief by illumination with a circularly polarized Gaussian beam.

A helical surface relief can be created in an azo-polymer film simply by illuminating circularly polarized light with spin angular momentum and without any orbital angular momentum. The helicity of the surface relief is determined by the sign of the spin angular momentum. The illumination of circularly polarized light induces orbital motion of the azo-polymer to shape the helical surface relief as an intermediate form; a subsequent transformation to a non-helical bump-shaped relief with a central peak creates a final form with additional exposure time. The mechanism for the formation of such a helical surface relief was also theoretically analyzed using the formula for the optical radiation force in a homogeneous and isotropic material.

Highly intense monocycle terahertz vortex generation by utilizing a Tsurupica spiral phase plate.

Optical vortex, possessing an annular intensity profile and an orbital angular momentum (characterized by an integer termed a topological charge) associated with a helical wavefront, has attracted great attention for diverse applications due to its unique properties. In particular for terahertz (THz) frequency range, several approaches for THz vortex generation, including molded phase plates consisting of metal slit antennas, achromatic polarization elements and binary-diffractive optical elements, have been recently proposed, however, they are typically designed for a specific frequency. Here, we demonstrate highly intense broadband monocycle vortex generation near 0.6 THz by utilizing a polymeric Tsurupica spiral phase plate in combination with tilted-pulse-front optical rectification in a prism-cut LiNbO3 crystal. A maximum peak power of 2.3 MW was obtained for THz vortex output with an expected topological charge of 1.15. Furthermore, we applied the highly intense THz vortex beam for studying unique nonlinear behaviors in bilayer graphene towards the development of nonlinear super-resolution THz microscopy and imaging system.

Beam propagation of efficient frequency-doubled optical vortices.

Frequency doubling of optical vortices is demonstrated with an optical-optical efficiency exceeding 70%, using a spiral phase plate at a fundamental vortex energy of 10.6 mJ. Beam propagation of the doubled vortex output is also investigated both experimentally and theoretically. Spatial transforms in the output during propagation are observed.

Octave-band tunable optical vortex parametric oscillator.

We developed an octave-band tunable optical vortex laser based on a 532 nm optical vortex pumped optical parametric oscillator with a simple linear-cavity configuration by employing cascaded non-critical phase-matching LiB3O5 crystals. The optical vortex output was tunable from 735 to 1903 nm. For a pump energy of 9 mJ, an optical vortex pulse energy of 0.24-2.36 mJ was obtained, corresponding to an optical-optical efficiency of 0.3-26%.