Spatial Properties of High-Order Harmonic Beams from Plasma Mirrors: A Ptychographic Study.

Spatial properties of high-order harmonic beams produced by high-intensity laser-matter interactions carry rich information on the physics of the generation process, and their detailed understanding is essential for applications of these light beams. We present a thorough study of these properties in the case of harmonic generation from plasma mirrors, up to the relativistic interaction regime. In situ ptychographic measurements of the amplitude and phase spatial profiles of the different harmonic orders in the target plane are presented, as a function of the key interaction parameters. These measurements are used to validate analytical models of the harmonic spatial phase in different generation regimes, and to benchmark ultrahigh-order Maxwell solvers of particle-in-cell simulation codes.

Optically controlled solid-density transient plasma gratings.

A general approach for optically controlled spatial structuring of overdense plasmas generated at the surface of initially plain solid targets is presented. We demonstrate it experimentally by creating sinusoidal plasma gratings of adjustable spatial periodicity and depth, and study the interaction of these transient structures with an ultraintense laser pulse to establish their usability at relativistically high intensities. We then show how these gratings can be used as a "spatial ruler" to determine the source size of the high-order harmonic beams produced at the surface of an overdense plasma. These results open new directions both for the metrology of laser-plasma interactions and the emerging field of ultrahigh intensity plasmonics.

Optical properties of relativistic plasma mirrors.

The advent of ultrahigh-power femtosecond lasers creates a need for an entirely new class of optical components based on plasmas. The most promising of these are known as plasma mirrors, formed when an intense femtosecond laser ionizes a solid surface. These mirrors specularly reflect the main part of a laser pulse and can be used as active optical elements to manipulate its temporal and spatial properties. Unfortunately, the considerable pressures exerted by the laser can deform the mirror surface, unfavourably affecting the reflected beam and complicating, or even preventing, the use of plasma mirrors at ultrahigh intensities. Here we derive a simple analytical model of the basic physics involved in laser-induced deformation of a plasma mirror. We validate this model numerically and experimentally, and use it to show how such deformation might be mitigated by appropriate control of the laser phase.

Spectral characterization of laser-driven solid-based high harmonics in the coherent wake emission regime.

Laser-produced surface high-harmonic generation is an attractive source of extreme ultraviolet radiation due to its coherent properties and high peak power. By operating at subrelativistic laser intensities in the coherent wake emission regime, the harmonic spectrum was experimentally studied versus laser properties. At higher laser intensities (>10(17) W/cm(2)) a higher spectral cutoff was observed, with accompanying blueshifting and spectral broadening of the individual orders. A model based on an expanding critical surface provides qualitative agreement with the observations.

Direct observation of density-gradient effects in harmonic generation from plasma mirrors.

High-order harmonics and attosecond pulses of light can be generated when ultraintense, ultrashort laser pulses reflect off a solid-density plasma with a sharp vacuum interface, i.e., a plasma mirror. We demonstrate experimentally the key influence of the steepness of the plasma-vacuum interface on the interaction, by measuring the spectral and spatial properties of harmonics generated on a plasma mirror whose initial density gradient scale length L is continuously varied. Time-resolved interferometry is used to separately measure this scale length.