An optofluidic antenna for enhancing the sensitivity of single-emitter measurements.

Many single-molecule investigations are performed in fluidic environments, for example, to avoid unwanted consequences of contact with surfaces. Diffusion of molecules in this arrangement limits the observation time and the number of collected photons, thus, compromising studies of processes with fast or slow dynamics. Here, we introduce a planar optofluidic antenna (OFA), which enhances the fluorescence signal from molecules by about 5 times per passage, leads to about 7-fold more frequent returns to the observation volume, and significantly lengthens the diffusion time within one passage. We use single-molecule multi-parameter fluorescence detection (sm-MFD), fluorescence correlation spectroscopy (FCS) and Förster resonance energy transfer (FRET) measurements to characterize our OFAs. The antenna advantages are showcased by examining both the slow (ms) and fast (50 µs) dynamics of DNA four-way (Holliday) junctions with real-time resolution. The FRET trajectories provide evidence for the absence of an intermediate conformational state and introduce an upper bound for its lifetime. The ease of implementation and compatibility with various microscopy modalities make OFAs broadly applicable to a diverse range of studies.

Organic Molecules as Origin of Visible-Range Single Photon Emission from Hexagonal Boron Nitride and Mica.

The discovery of room-temperature single-photon emitters (SPEs) hosted by two-dimensional hexagonal boron nitride (2D hBN) has sparked intense research interest. Although emitters in the vicinity of 2 eV have been studied extensively, their microscopic identity has remained elusive. The discussion of this class of SPEs has centered on point defects in the hBN crystal lattice, but none of the candidate defect structures have been able to capture the great heterogeneity in emitter properties that is observed experimentally. Employing a widely used sample preparation protocol but disentangling several confounding factors, we demonstrate conclusively that heterogeneous single-photon emission at ∼2 eV associated with hBN originates from organic molecules, presumably aromatic fluorophores. The appearance of those SPEs depends critically on the presence of organic processing residues during sample preparation, and emitters formed during heat treatment are not located within the hBN crystal as previously thought, but at the hBN/substrate interface. We further demonstrate that the same class of SPEs can be observed in a different 2D insulator, fluorophlogopite mica.

Observation of dipolar transport in one-dimensional photonic lattices.

We experimentally study the transport properties of dipolar and fundamental modes on one dimensional (1D) coupled waveguide arrays. By carefully modulating a wide optical beam, we are able to effectively excite dipolar or fundamental modes to study discrete diffraction (single-site excitation) and gaussian beam propagation (multi-site excitation plus a phase gradient). We observe that dipolar modes experience a larger spreading area due to an effective larger coupling constant, which is found to be more than two times larger than the one for fundamental modes. Additionally, we study the effect of non-diagonal disorder and find that while fundamental modes are already trapped on a weakly disorder array, dipoles are still able to propagate across the system.

Transport in Sawtooth photonic lattices.

We investigate, theoretically and experimentally, a photonic realization of a Sawtooth lattice. This special lattice exhibits two spectral bands, with one of them experiencing a complete collapse to a highly degenerate flat band for a special set of inter-site coupling constants. We report the observation of different transport regimes, including strong transport inhibition due to the appearance of the non-diffractive flat band. Moreover, we excite localized Shockley surface states residing in the gap between the two linear bands.

Observation of Localized States in Lieb Photonic Lattices.

We present the first experimental demonstration of a new type of localized state in the continuum, namely, compacton-like linear states in flat-band lattices. To this end, we employ photonic Lieb lattices, which exhibit three tight-binding bands, with one being perfectly flat. Discrete predictions are confirmed by realistic continuous numerical simulations as well as by direct experiments. Our results could be of great importance for fundamental physics as well as for various applications where light needs to be conducted in a diffractionless and localized manner over long distances.