New solid state laser system for SPES: Selective Production of Exotic Species project at Laboratori Nazionali di Legnaro.

The Selective Production of Exotic Species project is under construction at Laboratori Nazionali di Legnaro-INFN. The aim of the collaboration is to produce highly pure Radioactive Ion Beams (RIBs) from fission fragments of a uranium carbide (UCx) target activated by a cyclotron proton beam. In order to select a specific atomic species, the main tool to be applied is the resonant laser ionization technique. We have just completed the installation of a dedicated all solid state laser system whose elements are tunable to transitions of all the elements/isotopes of interest for the project. The new laser system is based on three Titanium:sapphire laser sources, independently pumped by three Nd:YLF pump lasers, and it can be coupled to two high harmonic generation (second harmonic generation, third harmonic generation, and fourth harmonic generation) setups. The power, wavelength, and position of the laser beams are continuously monitored and stabilized by using automated active systems to improve the beam production stability of RIBs. This paper presents the main features of the laser system and examples of application of a laser ion source, including a first demonstration of photoionization of stable silver, one of the most requested elements for RIB application.

EUV polarimetry for thin film and surface characterization and EUV phase retarder reflector development.

The knowledge and the manipulation of light polarization state in the vacuum ultraviolet and extreme ultraviolet (EUV) spectral regions play a crucial role from materials science analysis to optical component improvements. In this paper, we present an EUV spectroscopic ellipsometer facility for polarimetry in the 90-160 nm spectral range. A single layer aluminum mirror to be used as a quarter wave retarder has been fully characterized by deriving the optical and structural properties from the amplitude component and phase difference δ measurements. The system can be suitable to investigate the properties of thin films and optical coatings and optics in the EUV region.

Analysis of buried interfaces in multilayer mirrors using grazing incidence extreme ultraviolet reflectometry near resonance edges.

Accurate measurements of optical properties of multilayer (ML) mirrors and chemical compositions of interdiffusion layers are particularly challenging to date. In this work, an innovative and nondestructive experimental characterization method for multilayers is discussed. The method is based on extreme ultraviolet (EUV) reflectivity measurements performed on a wide grazing incidence angular range at an energy near the absorption resonance edge of low-Z elements in the ML components. This experimental method combined with the underlying physical phenomenon of abrupt changes of optical constants near EUV resonance edges enables us to characterize optical and structural properties of multilayers with high sensitivity. A major advantage of the method is to perform detailed quantitative analysis of buried interfaces of multilayer structures in a nondestructive and nonimaging setup. Coatings of Si/Mo multilayers on a Si substrate with period d=16.4 nm, number of bilayers N=25, and different capping structures are investigated. Stoichiometric compositions of Si-on-Mo and Mo-on-Si interface diffusion layers are derived. Effects of surface oxidation reactions and carbon contaminations on the optical constants of capping layers and the impact of neighboring atoms' interactions on optical responses of Si and Mo layers are discussed.

Stability of extreme ultraviolet multilayer coatings to low energy proton bombardment.

In this work we present results of an new experiment related to low energy protons bombardments on nano-structured optical coatings. Multilayer structures protected by different capping layers have been fabricated and exposed to low energy protons (1 keV). The experimental parameters have been selected considering the potential application of the coatings to solar mission instrumentation. Future solar missions will investigate the Sun from very close distances and optical components are constantly exposed to low energy ion particles irradiation. The experiment was repeated fixing the proton flux while varying the total dose accumulated. Results show that physical processes occurred at the uppermost interfaces can strongly damage the structure.

Reflectance measurements and optical constants in the extreme ultraviolet-vacuum ultraviolet regions for SiC with a different C/Si ratio.

Reflectance versus incidence angle measurements have been performed from 5 to 152 nm on samples of SiC with a different C/Si ratio deposited with rf magnetron sputtering. The optical constants of the material at different wavelengths have been determined by using a curve-fitting technique of reflectance values versus incidence angle. Complementary measurements of the incident beam polarization, film thickness, surface roughness, and stoichiometry were performed to complete the analysis of the samples.

Spectroscopic characterization of vacuum ultraviolet free electron laser pulses.

Because of the stochastic nature of self-amplified spontaneous emission (SASE), it is crucial to measure for single pulses the spectral characteristics of ultrashort pulses from the vacuum ultraviolet free electron laser (FLASH) at DESY, Germany. To meet this particular challenge, we have employed both photon and photoelectron spectroscopy. Each FEL pulse is composed of an intense and spectrally complex fundamental, centered at a photon energy of about 38.5 eV, with a bandwidth of 0.5% accompanied by higher harmonics, each carrying an intensity of typically 0.3 to 0.6% of that of the fundamental. The correlation between the harmonics and the fundamental is in remarkable agreement with a simple statistical model of SASE FEL radiation.

Polarization and higher-order content measurement of a soft-x-ray monochromatized beam with Mo-Si multilayers.

A Mo-Si multilayer mirror has been used for determination of the ellipticity and higher-order content of a synchrotron beam. The method is based on the angular measure of multilayer reflectivity in the region of Bragg first- and second-order reflections. Beam parameters were derived by a fitting procedure.

Design and experimental characterization of a high-resolution instrument for measuring the extreme-UV absorption of laser plasmas.

The performances of a spectrometer for the observation of laser plasma absorption with high spectral and spatial resolution are described. Aspherical optics are used to correct the astigmatism in an extended spectral region. In this way only a small portion of the absorbing medium is probed, thus giving a good selection of the ionization stage acting as the absorption. Moreover, in the focal plane the plasma emission from the absorbing medium is spatially separated from the probe beam, with a consequent enhancement of the measurement sensitivity. The predicted optical performances from a ray tracing are compared with experimental observations for both spectral and spatial resolution.

Thin-film photodetectors for the vacuum ultraviolet spectral region.

We report on thin-film photodetectors optimized for detecting the vacuum UV and rejection of the visible spectrum of electromagnetic radiation. The devices are made of hydrogenated amorphous silicon and silicon carbide on a glass substrate. At room temperature the photodetectors exhibit quantum efficiencies of 52% at lambda = 58.4 nm, 1% at lambda = 400 nm, and 0.1% at lambda = 650 nm. The response time for UV pulses from an N(2) laser gives signals of 6-mus full width at half-maximum and 500-ns rise time.

Optical performances of the Ultraviolet Coronagraph Spectrometer of the Solar Heliospheric Observatory.

The optical performances of the spectrometer assembly for the Ultraviolet Coronagraph Spectrometer of the Solar and Heliospheric Observatory mission have been tested. The flight unit of the spectrometer assembly, consisting of the structure equipped with the entrance slits assembly, the grating drive mechanisms mounting two toroidal gratings, and the photon-counting detectors, has been integrated and aligned; also the flight unit of the White Light Channel has been integrated and aligned in the spectrometer assembly. Tests with both visible and UV radiation have been performed. Aberration and stray-light measurements have shown that the instrument performs satisfactorily, almost in compliance with the scientific requirements; also some measurements of the polarimeter modulation curve and the relative error have shown performances within the specified requirements.

Stigmatic observations of laser-produced plasmas with a grazingincidence spectrograph.

A stigmatic spectrograph composed of a toroidal mirror and a concave grating both working at grazing incidence has been built and applied to the observation of laser-produced plasmas. Spatial resolution of 20-30 microm over a region of 1-mm extension and spectral resolution of approximately 1500 have been obtained with a considerable increase in speed of the spectrograph. By varying the relative positions of the optical elements, it is possible to change the wavelength of stigmatic condition in the range 10-300 A. Examples of observations of a beryllium plasma are shown.