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1.
Sci Adv ; 7(51): eabj6565, 2021 Dec 17.
Article in English | MEDLINE | ID: mdl-34910518

ABSTRACT

Stretchable optoelectronics made of elastomeric semiconductors could enable the integration of intelligent systems with soft materials, such as those of the biological world. Organic semiconductors and photodiodes have been engineered to be elastomeric; however, for photodetector applications, it remains a challenge to identify an elastomeric bulk heterojunction (e-BHJ) photoactive layer that combines a low Young's modulus and a high strain at break that yields organic photodiodes with low electronic noise values and high photodetector performance. Here, a blend of an elastomer, a donor-like polymer, and an acceptor-like molecule yields a skin-like e-BHJ with a Young's modulus of a few megapascals, comparable to values of human tissues, and a high strain at break of 189%. Elastomeric organic photodiodes based on e-BHJ photoactive layers maintain low electronic noise current values in the tens of femtoamperes range and noise equivalent power values in the tens of picowatts range under at least 60% strain.

2.
Sci Adv ; 4(1): eaao1705, 2018 01.
Article in English | MEDLINE | ID: mdl-29340301

ABSTRACT

Organic thin-film transistors (OTFTs) can be fabricated at moderate temperatures and through cost-effective solution-based processes on a wide range of low-cost flexible and deformable substrates. Although the charge mobility of state-of-the-art OTFTs is superior to that of amorphous silicon and approaches that of amorphous oxide thin-film transistors (TFTs), their operational stability generally remains inferior and a point of concern for their commercial deployment. We report on an exhaustive characterization of OTFTs with an ultrathin bilayer gate dielectric comprising the amorphous fluoropolymer CYTOP and an Al2O3:HfO2 nanolaminate. Threshold voltage shifts measured at room temperature over time periods up to 5.9 × 105 s do not vary monotonically and remain below 0.2 V in microcrystalline OTFTs (µc-OTFTs) with field-effect carrier mobility values up to 1.6 cm2 V-1 s-1. Modeling of these shifts as a function of time with a double stretched-exponential (DSE) function suggests that two compensating aging mechanisms are at play and responsible for this high stability. The measured threshold voltage shifts at temperatures up to 75°C represent at least a one-order-of-magnitude improvement in the operational stability over previous reports, bringing OTFT technologies to a performance level comparable to that reported in the scientific literature for other commercial TFTs technologies.

3.
Cyberpsychol Behav ; 11(4): 505-9, 2008 Aug.
Article in English | MEDLINE | ID: mdl-18694331

ABSTRACT

This research studied the interactivity and cultural differences provided by online versions of daily newspapers. It examined interactivity features on the 116 online versions of South Korean and U.S. newspapers on the basis of users' activities when they read the online newspaper. Within intercultural context, this study found that online versions of Korean newspapers use more "active" interactivity features than do U.S. online versions. However, online versions of U.S. newspapers demonstrated more "inactive" interactivity features than Korean online newspapers. New findings about interactivity and culture in online newspapers are discussed.


Subject(s)
Community Participation/statistics & numerical data , Internet/statistics & numerical data , Journalism , Newspapers as Topic/statistics & numerical data , Online Systems/statistics & numerical data , Bibliometrics , Cross-Cultural Comparison , Humans
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