Colorimetry characterization of molecular reorientation transition in thin nematic cells.

The characterization of equilibria and their transition is fundamental in dynamic systems. Experimentally, the characterization of transitions is complex due to time scales separation, the effect of thermal fluctuations, and inherent experimental imperfections. Liquid crystal devices are derived from the manipulation of the molecular reorientation and transition between them by employing external electrical and magnetic fields. Here, we investigate and determine the Fréedericksz transition using hue measurements of the transmitted light in thin nematic liquid crystal cells. Based on birefringent retardation experienced by transmitted light due to molecular reorientation, the color adjustment of the nematic liquid crystal cells under white light illumination is characterized. By monitoring the hue of the transmitted light, the bifurcation diagram is determined. As a function of the voltage frequency, the critical transition voltage is characterized. The critical voltage increases with the applied frequency.

Dissipative structures induced by photoisomerization in a dye-doped nematic liquid crystal layer.

Order-disorder phase transitions driven by temperature or light in soft matter materials exhibit complex dissipative structures. Here, we investigate the spatio-temporal phenomena induced by light in a dye-doped nematic liquid crystal layer. Experimentally, for planar anchoring of the nematic layer and high enough input power, photoisomerization processes induce a nematic-isotropic phase transition mediated by interface propagation between the two phases. In the case of a twisted nematic layer and for intermediate input power, the light induces a spatially modulated phase, which exhibits stripe patterns. The pattern originates as an instability mediated by interface propagation between the modulated and the homogeneous nematic states. Theoretically, the phase transition, emergence of stripe patterns and front dynamics are described on the basis of a proposed model for the dopant concentration coupled with the nematic order parameter. Numerical simulations show quite a fair agreement with the experimental observations.This article is part of the theme issue 'Dissipative structures in matter out of equilibrium: from chemistry, photonics and biology (part 2)'.

Light-matter interaction induces a shadow vortex.

By sending a light beam on a homeotropic nematic liquid-crystal cell subjected to a voltage with a photosensitive wall, a stable matter vortex can be induced at the center of the beam. When the applied voltage is decreased, the vortex disappears from the illuminated region; however, the system shows a stationary molecular texture. Based on a forced Ginzburg-Landau amplitude equation, we show that the vortex with a core of exponentially suppressed amplitude always remains in a shadow region below instability threshold and that the observed texture is induced by its phase distribution. This is a different type of vortex phase singularity solution. Numerical simulations and experimental observations show a quite fair agreement.

Chaoticon: localized pattern with permanent dynamics.

An analytical mechanism that support localized spatio-temporal chaos is provided. We consider a simple model-the Nagumo Kuramoto model-which contains the crucial ingredients for observing localized spatio-temporal chaos, namely, the spatio-temporal chaotic pattern and its coexistence with a uniform state. This model allows us to unveil the front dynamics and to show that it can be described by a chaotic motor corresponding to the deterministic counterpart of a Brownian motor. Front interaction is identified as the mechanism at the origin of the localized spatio-temporal chaotic structures.

Spatiotemporal chaotic localized state in liquid crystal light valve experiments with optical feedback.

The existence, stability properties, and dynamical evolution of localized spatiotemporal chaos are studied. We provide evidence of spatiotemporal chaotic localized structures in a liquid crystal light valve experiment with optical feedback. The observations are supported by numerical simulations of the Lifshitz model describing the system. This model exhibits coexistence between a uniform state and a spatiotemporal chaotic pattern, which emerge as the necessary ingredients to obtain localized spatiotemporal chaos. In addition, we have derived a simplified model that allows us to unveil the front interaction mechanism at the origin of the localized spatiotemporal chaotic structures.

Effects of translational coupling on dissipative localized states.

Nonequilibrium localized states under the influence of translational coupling are studied experimentally and theoretically. We show that localized structures are deformed and advected in the direction of the coupling, thus undergoing different instabilities. Experimentally, localized structures are obtained in a light valve with optical feedback. By introducing a tilt of one mirror in the feedback loop, localized structures acquire a translational coupling. To understand the phenomenon in a universal framework we consider a prototypical model of localized states with translational coupling in one and two spatial dimensions. The model allows us to analytically characterize the propagation speed and the deformation exhibited by the localized state profiles as well as to figure out different mechanisms of destabilization of these dissipative structures. The results are in good qualitative agreement with the experimental and numerical observations.

Bouncing localized structures in a liquid-crystal light-valve experiment.

Experimental evidence of bouncing localized structures in a nonlinear optical system is reported. Oscillations in the position of the localized states are described by a consistent amplitude equation, which we call the Lifshitz normal form equation, in analogy with phase transitions. Localized structures are shown to arise close to the Lifshtiz point, where nonvariational terms drive the dynamics into complex and oscillatory behaviors.