Dual-comb optomechanical spectroscopy.

Optical cavities are essential for enhancing the sensitivity of molecular absorption spectroscopy, which finds widespread high-sensitivity gas sensing applications. However, the use of high-finesse cavities confines the wavelength range of operation and prevents broader applications. Here, we take a different approach to ultrasensitive molecular spectroscopy, namely dual-comb optomechanical spectroscopy (DCOS), by integrating the high-resolution multiplexing capabilities of dual-comb spectroscopy with cavity optomechanics through photoacoustic coupling. By exciting the molecules photoacoustically with dual-frequency combs and sensing the molecular-vibration-induced ultrasound waves with a cavity-coupled mechanical resonator, we measure high-resolution broadband ( > 2 THz) overtone spectra for acetylene gas and obtain a normalized noise equivalent absorption coefficient of 1.71 × 10-11 cm-1·W·Hz-1/2 with 30 GHz simultaneous spectral bandwidth. Importantly, the optomechanical resonator allows broadband dual-comb excitation. Our approach not only enriches the practical applications of the emerging cavity optomechanics technology but also offers intriguing possibilities for multi-species trace gas detection.

Dissipative coupling-induced phonon lasing.

Phonon lasers, as the counterpart of photonic lasers, have been intensively studied in a large variety of systems; however, (all) most of them are based on the directly coherent pumping. Intuitively, dissipation is unfavorable for lasing. Here, we experimentally demonstrate a mechanism of generating phonon lasing from the dissipative coupling in a multimode optomechanical system. By precisely engineering the dissipations of two membranes and tuning the intensity modulation of the cavity light, the two-membrane-in-the-middle system exhibits non-Hermitian characteristics and the cavity-mediated interaction between two nanomechanical resonators becomes purely dissipative. The level attraction and damping repulsion are clearly exhibited as the signature of dissipative coupling. After the exceptional point, a non-Hermitian phase transition, where eigenvalues and the corresponding eigenmodes coalesce, two phonon modes are simultaneously excited into the self-sustained oscillation regime by increasing the interaction strength over a critical value (threshold). In distinct contrast to conventional phonon lasers, the measurement of the second-order phonon correlation reveals the oscillatory and biexponential phases in the nonlasing regime as well as the coherence phase in the lasing regime. Our study provides a method to study phonon lasers in a non-Hermitian open system and could be applied to a wide range of disciplines, including optics, acoustics, and quantum many-body physics.

Realization of a coupled-mode heat engine with cavity-mediated nanoresonators.

We report an experimental demonstration of a coupled-mode heat engine in a two-membrane-in-the-middle cavity optomechanical system. The normal mode of the cavity-mediated strongly coupled nanoresonators is used as the working medium, and an Otto cycle is realized by extracting work between two phononic thermal reservoirs. The heat engine performance is characterized in both normal mode and bare mode pictures, which reveals that the correlation of two membranes plays a substantial role during the thermodynamic cycle. Moreover, a straight-twin nanomechanical engine is implemented by engineering the normal modes and operating two cylinders out of phase. Our results demonstrate an essential class of heat engine in cavity optomechanical systems and provide an ideal platform platform for investigating heat engines of interacting subsystems in small scales with controllability and scalability.

Phonon heat transport in cavity-mediated optomechanical nanoresonators.

The understanding of heat transport in nonequilibrium thermodynamics is an important research frontier, which is crucial for implementing novel thermodynamic devices, such as heat engines and refrigerators. The convection, conduction, and radiation are the well-known basic ways to transfer thermal energy. Here, we demonstrate a different mechanism of phonon heat transport between two spatially separated nanomechanical resonators coupled by the cavity-enhanced long-range interactions. The single trajectory for thermalization and non-equilibrium dynamics is monitored in real-time. In the strong coupling regime, the instant heat flux spontaneously oscillates back and forth in the nonequilibrium steady states. The universal bound on the precision of nonequilibrium steady-state heat flux, i.e. the thermodynamic uncertainty relation, is verified in such a temperature gradient driven far-off equilibrium system. Our results give more insight into the heat transfer with nanomechanical oscillators, and provide a playground for testing fundamental theories in non-equilibrium thermodynamics.

Self-Organized Synchronization of Phonon Lasers.

Self-organized synchronization is a ubiquitous collective phenomenon, in which each unit adjusts their rhythms to achieve synchrony through mutual interactions. The optomechanical systems, due to their inherently engineerable nonlinearities, provide an ideal platform to study self-organized synchronization. Here, we demonstrate the self-organized synchronization of phonon lasers in a two-membrane-in-the-middle optomechanical system. The probe of each individual membrane enables us to monitor the real-time transient dynamics of synchronization, which reveals that the system enters into the synchronization regime via a torus birth bifurcation line. The phase-locking phenomenon and the transition between in-phase and antiphase regimes are directly observed. Moreover, such a system greatly facilitates the controllable synchronous states, and consequently a phononic memory is realized by tuning the system parameters. This result is an important step towards the future studies of many-body collective behaviors in multiresonator optomechanics with long distances, and might find potential applications in quantum information processing and complex networks.

Temporal rocking in a nonlinear hybrid optomechanical system.

We explore theoretically the optomechanical interaction between a light field and a mechanical mode mediated by a Kerr nonlinear medium inside a Fabry-Perot cavity. When the system is driven by a strong and fast amplitude-modulated light field, i.e., in the so-called temporal rocking region, the cavity field and the mechanical oscillator show the characteristics of multistability. The rocking breaks down the continuous phase symmetry of the cavity field to a bistable case of two equivalent states with exact π phase difference. In addition, the rocking can significantly enhance the optomechanical coupling between the light field and the mechanical oscillator, which can be used as a new handle to control the normal mode splitting of the mechanical spectrum. Moreover, the optomechanical cooling rate can be greatly modified by the rocking. With the optimized rocking parameters, the mechanical oscillator can be cooled down to its ground state more efficiently. Such a temporal rocking optomechanical system has potential applications in all-optical switching and enhancement of quantum effects.

Controllable photonic crystal with periodic Raman gain in a coherent atomic medium.

With two sets of standing-wave fields built in a thermal rubidium vapor cell, we have established a controllable photonic crystal with periodic gain in a coherently prepared N-type four-level atomic configuration. First, the photonic lattice constructed by a resonant standing-wave coupling field results in a spatially modulated susceptibility and makes the signal field diffract in a discrete manner under the condition of electromagnetically induced transparency. Then, with the addition of the standing-wave pump field, the N-type atomic medium can induce a periodic Raman gain on the signal field, which can be effectively controlled by tuning the pertinent atomic parameters. The experimental demonstration of such a real-time reconfigurable photonic crystal structure with periodic Raman gain can pave the way for realizing desired applications predicted in the gain-modulated periodic optical systems.

Atom-Based Sensing of Weak Radio Frequency Electric Fields Using Homodyne Readout.

We utilize a homodyne detection technique to achieve a new sensitivity limit for atom-based, absolute radio-frequency electric field sensing of 5 µV cm-1 Hz-1/2. A Mach-Zehnder interferometer is used for the homodyne detection. With the increased sensitivity, we investigate the dominant dephasing mechanisms that affect the performance of the sensor. In particular, we present data on power broadening, collisional broadening and transit time broadening. Our results are compared to density matrix calculations. We show that photon shot noise in the signal readout is currently a limiting factor. We suggest that new approaches with superior readout with respect to photon shot noise are needed to increase the sensitivity further.

Observation of Parity-Time Symmetry in Optically Induced Atomic Lattices.

We experimentally demonstrate PT-symmetric optical lattices with periodical gain and loss profiles in a coherently prepared four-level N-type atomic system. By appropriately tuning the pertinent atomic parameters, the onset of PT-symmetry breaking is observed through measuring an abrupt phase-shift jump between adjacent gain and loss waveguides. The experimental realization of such a readily reconfigurable and effectively controllable PT-symmetric waveguide array structure sets a new stage for further exploiting and better understanding the peculiar physical properties of these non-Hermitian systems in atomic settings.

Strong Coupling of Rydberg Atoms and Surface Phonon Polaritons on Piezoelectric Superlattices.

We propose a hybrid quantum system where the strong coupling regime can be achieved between a Rydberg atomic ensemble and propagating surface phonon polaritons on a piezoelectric superlattice. By exploiting the large electric dipole moment and long lifetime of Rydberg atoms as well as tightly confined surface phonon polariton modes, it is possible to achieve a coupling constant far exceeding the relevant decay rates. The frequency of the surface mode can be selected so that it is resonant with a Rydberg transition by engineering the piezoelectric superlattice. We describe a way to observe the Rabi splitting associated with the strong coupling regime under realistic experimental conditions. The system can be viewed as a new type of optomechanical system.

Observation of discrete diffraction patterns in an optically induced lattice.

We have experimentally observed the discrete diffraction of light in a coherently prepared multi-level atomic medium. This is achieved by launching a probe beam into an optical lattice induced from the interference of two coupling beams. The diffraction pattern can be controlled through the atomic parameters such as two-photon detuning and temperature, as well as orientations of the coupling and probe beams. Clear diffraction patterns occur only near the two-photon resonance.

Two-photon dynamics in coherent Rydberg atomic ensemble.

We study the interaction of two photons in a Rydberg atomic ensemble under the condition of electromagnetically induced transparency, combining a semiclassical approach for pulse propagation and a complete quantum treatment for quantum state evolution. We find that the blockade regime is not suitable for implementing photon-photon cross-phase modulation due to pulse absorption and dispersion. However, approximately ideal cross-phase modulation can be realized based on relatively weak interactions, with counterpropagating and transversely separated pulses.

Spatial domain interactions between ultraweak optical beams.

We have observed spatial interactions between two ultraweak optical beams that are initially collinear and nonoverlapping. The weak beams are steered towards each other by a spatially varying cross-Kerr refractive index waveguide written by a strong laser beam in a three-level coherently prepared atomic medium. After fusing together, the combined beam shows controllable phase-dependent behaviors. This is the first observation of solitonlike interactions between weak beams and can be useful for all-optically tunable beam combining, switching, and gating for weak photonic signals.

Synchronous control of dual-channel all-optical multistate switching.

We have experimentally observed optical multistabilities (OMs) simultaneously on both the signal and generated Stokes fields in an optical ring cavity with a coherently prepared multilevel atomic medium. The two observed OMs, which are governed by different physical processes, are coupled via the multilevel atomic medium and exhibit similar threshold behaviors. By modulating the cavity input (signal) field with positive or negative pulses, dual-channel all-optical multistate switching has been realized and synchronously controlled, which can be useful for increasing communication and computation capacities.

Noise correlations in a doubly-resonant atomic optical parametric oscillator.

The simultaneous generations of bright Stokes and anti-Stokes fields are realized by using only one pump field in a Doppler-broadened atomic medium confined in an optical ring cavity. A vacuum-induced absorption phenomenon is also observed in such a system. By utilizing an external Fabry-Perot cavity to separate the Stokes and anti-Stokes fields, we investigate the noise correlation and anticorrelation properties between the Stokes, anti-Stokes, and the pump fields.

Realization of all-optical multistate switching in an atomic coherent medium.

We have experimentally observed optical multistability (OM) in an optical ring cavity containing three-level Λ-type Doppler-broadened rubidium atoms. The shape of the OM curve can be significantly modified by changing the power of the control laser field. An all-optical multistate switching or coding element is realized and flexibly controlled by adding a pulse sequence to the input (probe) intensity.

All-optical switching in an N-type foul-level atom-cavity system.

We report an experimental observation of all-optical switching in an N-type atom-cavity system with a rubidium atomic vapor cell inside an optical ring cavity. Both absorptive and dispersive switching can be realized on dark- or bright-polariton peaks by a weak switching laser beam (with the extinction ratio better than 20:1). The switching mechanism can be explained as the combination of quantum interference and intracavity dispersion properties.