Quantitative gas pressure measurement by molecular spectroscopy using chip-based supercontinuum in the mid-infrared.

We demonstrate the quantitative pressure measurement of gas molecules in the mid-infrared using chip-based supercontinuum and cepstrum analysis without additional measurements for baseline normalization. A supercontinuum generated in an on-chip waveguide made of chalcogenide glass having high nonlinearity passes through CO gas and provides a transmission spectrum. The gas absorption information is deconvoluted from the original supercontinuum spectral information containing temporal fluctuation by cepstrum analysis and extracted simply by applying a bandpass filter in the temporal domain. The gas pressure estimated from the extracted absorption information is consistent with the value measured by a pressure gauge within a difference of 1.25%, despite spectral fluctuations in the supercontinuum baseline comparable to the spectral depth of the gas absorption lines.

Spontaneous soliton mode-locking of a microcomb assisted by Raman scattering.

We successfully control the interaction dynamics between optical parametric oscillation (OPO) and stimulated Raman scattering, leading to the generation of distinct frequency comb states in a microresonator. Through Raman-scattered photons, a Raman comb with a sech2 envelope is demonstrated having a broad RF beat note linewidth of several hundred kHz. Moreover, under a specific coupling regime, we successfully generate self-locked Raman single-solitons which is confirmed by a narrow RF beat note of 25 Hz. Remarkably, this spontaneous Raman soliton is deterministically generated through adiabatic pump frequency detuning without the requirement of external locking mechanisms. Additionally, we identify a frequency comb with an unconventional envelope that can be fitted with a Lorentzian × sech2 function, generated via an anti-Stokes process with respect to the Raman comb.

Self-stabilized soliton generation in a microresonator through mode-pulled Brillouin lasing.

Reducing the complexity required for starting and maintaining a soliton state has been a major task to fully miniaturize soliton microcombs including the accompanying external operating systems. Here we experimentally examine the generative process of a self-stabilized soliton in which a continuous-wave pump detuned on the thermally stable blue side of a resonance generates a Brillouin lasing signal that relays the pump power to the soliton pulses via intracavity mode-coupling without breaking thermal self-stability. Based on a simple setup consisting of a free-running laser and a microcavity without any external feedback systems by virtue of internal thermal locking, single-soliton pulses of 11 GHz repetition rate were deterministically generated. We demonstrate that the single-soliton pulses can be passively maintained over several days in a laboratory environment with a phase noise performance of -137dBc/Hz at 100 kHz.