Large area ion beam sputtered dielectric ultrafast mirrors for petawatt laser beamlines.

The latest advances in petawatt laser technology within the ELI Beamlines project have stimulated the development of large surface area dielectrically coated mirrors meeting all demanding requirements for guiding the compressed 30 J, 25 fs HAPLS laser beam at 10 Hz repetition rate and a center wavelength of 810 nm entirely in vacuum. We describe the production and evaluation of Ta2O5/HfO2/SiO2 ion beam sputtered coated (440 × 290 × 75) mm3 beam transport mirrors. No crazing was observed after thirty vacuum-air cycles. A laser induced damage threshold of 0.76 J/cm2 (fluence on mirror surface) was achieved and maintained at high shot rates.

Quantizing nanolaminates as versatile materials for optical interference coatings.

In this paper, the theoretical foundation of quantizing nanolaminates is explained, and the dependence of the optical band gap on quantum-well thickness is demonstrated. The production is investigated by applying molecular dynamics growth simulation and by correlating the results with layers deposited by ion beam sputtering and atomic layer deposition. The properties of manufactured nanolaminates are then compared to the theoretical behavior, and good agreement is found.

Enhancement of the damage resistance of ultra-fast optics by novel design approaches.

Dielectric components are essential for laser applications. Chirped mirrors are applied to compress the temporal pulse broadening crucial in the femtosecond regime. However, the design sensitivity and the electric field distribution of chirped mirrors is complex often resulting in low laser induced damage resistances. An approach is presented to increase the damage resistance of pulse compressing mirrors up to 190% in the NIR spectral range. Layers with critical high field intensity of a binary mirror design are substituted by ternary composites and quantized nanolaminates, respectively. The deposition process is improved by an in situ technique monitoring the phase of reflectance.

Tunable optical properties of amorphous Tantala layers in a quantizing structure.

Plasma deposition techniques like ion-beam-sputtering (IBS) are state of the art to manufacture high quality optical components for laser applications. Besides the well optimized process and monitoring systems, the coating material selection is integral to achieve optimum optical performances. Applying the IBS technology, an approach is presented to create novel materials by the direct application of binary oxides in a quantizing structure. By reducing the physical thickness of the high refractive index material to a few nm, within a classical high-low index stack, the electron confinement can be changed. Optical characterizations of the manufactured samples with decreasing quantum well thicknesses result in an increasing blue shift of the absorption gap and offer a method to approximate the effective mass of the high refractive index material in conjunction with theoretical models. Laser-induced damage threshold tests of coating samples prepared with different well thicknesses indicate an increase of the measured threshold values with optical gap energy.

Fourier-transform spectral interferometry for in situ group delay dispersion monitoring of thin film coating processes.

A fast Fourier-based measurement system to determine phase, group delay, and group delay dispersion during optical coating processes is proposed. The in situ method is based on a Michelson interferometer with a broad band light source and a very fast spectrometer. To our knowledge, group delay dispersion measurements directly on the moving substrates during a deposition process for complex interference coatings have been demonstrated for the first time. Especially for the very precise production of chirped mirrors it is advantageous to get information about the phase properties of the grown layer stack to react on errors and retrieve more information about the coating process.

Pulse characterization by THG d-scan in absorbing nonlinear media.

We report on few-cycle pulse characterization based on third harmonic generation dispersion scan (THG d-scan) measurements using thin films of different TiO(2)-SiO(2) compositions as nonlinear media. By changing the TiO(2) concentration in the thin film the band gap and therefore the position of the absorption edge were varied. The retrieved pulse durations from different nonlinear media agree within 5%, and the reconstructed pulse shapes prove to be immune against the absorption edges as well. The reason is the robust retrieval algorithm which takes the influence of wavelength dependent nonlinearity into account by a spectral weight function.