Your browser doesn't support javascript.
loading
Show: 20 | 50 | 100
Results 1 - 20 de 40
Filter
1.
Sci Total Environ ; 940: 173612, 2024 Aug 25.
Article in English | MEDLINE | ID: mdl-38823719

ABSTRACT

Numerous studies have examined the impact of temperature on mortality, yet research on the combined effect of temperature and humidity on non-accidental deaths remains limited. This study investigates the synergistic impact of high temperature and humidity on non-accidental deaths in China, assessing the influence of urban development and urbanization level. Utilizing the distributed lag nonlinear model (DLNM) of quasi-Poisson regression, we analyzed the relationship between Wet Bulb Globe Temperature (WBGT) and non-accidental deaths in 30 Chinese cities from 2010 to 2016, including Guangzhou during 2012-2016. We stratified temperature and humidity across these cities to evaluate the influence of varying humidity levels on deaths under high temperatures. Then, we graded the duration of heat and humidity in these cities to assess the impact of deaths with different durations. Additionally, the cities were categorized based on gross domestic product (GDP), and a vulnerability index was calculated to examine the impact of urban development and urbanization level on non-accidental deaths. Our findings reveal a pronounced synergistic effect of high temperature and humidity on non-accidental deaths, particularly at elevated humidity levels. The synergies of high temperature and humidity are extremely complex. Moreover, the longer the duration of high temperature and humidity, the higher the risk of non-accidental death. Furthermore, areas with higher urbanization exhibited lower relative risks (RR) associated with the synergistic effects of heat and humidity. Consequently, it is imperative to focus on damp-heat related mortality among vulnerable populations in less developed regions.


Subject(s)
Cities , Hot Temperature , Humidity , Urbanization , China/epidemiology , Humans , Mortality
2.
Sci Total Environ ; 919: 170783, 2024 Apr 01.
Article in English | MEDLINE | ID: mdl-38340852

ABSTRACT

In transportation microenvironments, humans exposed to particulate matter (PM) inside vehicles can experience higher levels of daily exposure. To make inside-vehicle PM exposure measurements more feasible and easy under real driving conditions, and to quantify the relationship between the concentrations and influencing factors, we assessed PM1, PM2.5, and PM10. levels. Additionally, we collected key influencing factors to develop predictive models. The measurements of PM1, PM2.5, and PM10 concentrations showed that the ventilation setting was a significant influencing factor. The concentrations decreased significantly under the recirculation setting (RC) compared to the outside air setting (OA). The inside-to-outside (I/O) ratios of PM were 1.69 to 1.93-fold higher than those of RC under OA conditions. However, a substantial reduction in the I/O ratios was observed when RC was employed. Although both the concentrations and I/O ratios exhibited significant differences, they demonstrated strong potential relationships. PM2.5 I/O ratios accounted for over 85 % of the variation in the PM1 and PM10 I/O ratios. The developed models for the I/O ratios of PM accounted for >40 and 60 % of the variation in the measured I/O ratios for RC and OA, respectively. We used the vehicle age, vehicle interior volume, speed, cabin temperature, cabin humidity, and their higher-order terms as predictive variables. It is important to note that the influential predictive feature importance differed under RC and OA, and considering the vehicle characteristics between vehicles of the same type may be necessary when using RC. Overall, these findings indicate that the inside-vehicle PM exposure can be measured more easily under real driving conditions by considering the key influencing factors and utilizing the developed predictive models.

3.
Environ Pollut ; 334: 122131, 2023 Oct 01.
Article in English | MEDLINE | ID: mdl-37429486

ABSTRACT

Although ambient fine particulate matter (PM2.5) concentrations and their components are commonly used as proxies for personal exposure monitoring, developing an accurate and cost-effective method to use these proxies for personal exposure measurement continues to pose a significant challenge. Herein, we propose a scenario-based exposure model to precisely estimate personal exposure level of heavy metal(loid)s (HMs) using scenario HMs concentrations and time-activity patterns. Personal exposure levels and ambient pollution levels for PM2.5 and HMs differed significantly with corresponding personal/ambient ratios of approximately 2, and exposure scenarios could narrow the assessment error gap by 26.1-45.4%. Using a scenario-based exposure model, we assessed the associated health risks of a large sample population and identified that the carcinogenic risk of As exceeded 1 × 10-6, while we observed non-carcinogenic risks from As, Cd, Ni, and Mn in personal exposure to PM2.5. We conclude that the scenario-based exposure model is a preferential alternative for monitoring personal exposure compared to ambient concentrations. This method ensures the feasibility of personal exposure monitoring and health risk assessments in large-scale studies.


Subject(s)
Air Pollutants , Metals, Heavy , Air Pollutants/toxicity , Air Pollutants/analysis , Environmental Monitoring/methods , Particulate Matter/analysis , Metals, Heavy/toxicity , Metals, Heavy/analysis , Environmental Pollution , Risk Assessment , China
4.
Sci Total Environ ; 871: 162090, 2023 May 01.
Article in English | MEDLINE | ID: mdl-36764537

ABSTRACT

Ambient monitoring may cause estimation errors, and wearable monitoring is expensive and labor-intensive when assessing PM2.5 personal exposure. Estimation errors have limited the development of exposure science and environmental epidemiology. Thus, we developed a scenario-based exposure (SBE) model that covered 8 outdoor exposure scenarios and 1 indoor scenario with corresponding time-activity patterns in Baoding City. The linear regression analysis of the SBE yielded an R2 value of 0.913 with satisfactory accuracy and reliability. To apply the SBE model to large-scale studies, we predicted time-activity patterns with the random forest model and atmosphere-to-scenario ratios with the linear regression model to obtain the essential parameters of the SBE model; their R2 was 0.65-0.93. The developed model would economize the study expenditure of field sampling for personal PM2.5 and deepen the understanding of the influences of indoor and outdoor factors on personal PM2.5. Using this method, we found that the personal PM2.5 exposure of Chinese residents was 10.50-347.02 µg/m3 in 2020, higher than the atmospheric PM2.5 concentration. Residents in North and Central China, especially the Beijing-Tianjin-Hebei region and the Fen-Wei Plains, had higher personal PM2.5 exposure than those in other areas.


Subject(s)
Air Pollutants , Air Pollution, Indoor , Air Pollution , Air Pollutants/analysis , Particulate Matter/analysis , Environmental Monitoring/methods , Random Forest , Reproducibility of Results , China , Air Pollution/analysis , Environmental Exposure/analysis , Air Pollution, Indoor/analysis
5.
Sci Total Environ ; 854: 158713, 2023 Jan 01.
Article in English | MEDLINE | ID: mdl-36113791

ABSTRACT

Heavy metal exposure via food consumption is inadequately investigated and deserves considerable attention. We collected hundreds of food ingredients and daily meals and assessed their probabilistic health risk using a Monte Carlo simulation based on an ingestion rate investigation. The detected concentrations of four heavy metals (Cr, Cd, Pb, and Hg) in all daily meal samples were within the limits stipulated in the National Food Safety Standard (GB 2762-2017), while that for As level was excessive in 0.3 % of daily meal samples. The same results were also observed in most food ingredient samples, and a standard-exceeding ratio of 23 % of As was observed in aquatic food or products, especially seafood, which was with the highest concentration reaching 1.24 mg/kg. Combining the detected heavy metal amounts with the ingestion rate investigation, the hazard quotients (HQs) of As, Cr, Cd, Pb, and Hg in daily meals and food ingredients were all calculated as lower than 1 (no obvious harm), while the incremental lifetime cancer risk (ILCR) of As and Cr (>1 × 10-4), indicating that the residual As posed potential health effects to human health. It was noteworthy that the proportion of aquatic foods only accounted for 6.3 % of daily meals, but they occupied 41.1 % of the heavy metal exposure, which could be attributed to the high amounts of heavy metals in aquatic foods. This study not only provided basic data of heavy metal exposure and potential health risks through daily oral dietary intake, but also illuminated the contribution of different kinds of food ingredients. Specifically, the study highlighted the contamination of aquatic foods with As, especially seafood such as shellfish and bivalves.


Subject(s)
Food Ingredients , Mercury , Metals, Heavy , Humans , Cadmium , Rivers , Lead , Food Contamination/analysis , Metals, Heavy/analysis , Risk Assessment/methods , Mercury/analysis , Meals , Environmental Monitoring , China
6.
Sci Total Environ ; 833: 155209, 2022 Aug 10.
Article in English | MEDLINE | ID: mdl-35421500

ABSTRACT

Time-weighted average (TWA) exposure has been used as a surrogate for personal air exposure in some large-scale studies. However, the uncertainties of TWA exposure remain to be determined, although its boundedness has been widely recognized. This study aims to evaluate the reliability and accuracy of TWA exposure based on personal exposure. A total of 180 combined indoor-outdoor-personal air samples were collected of six cities during the non-heating and heating periods. The personal exposure levels of Hg, As, Cd, and Pb were 0.16, 21.20, 0.74, and 34.47 ng/m3 in the non-heating period, respectively, but were 0.20, 34.53, 3.45, and 18.59 ng/m3 in the heating period, respectively. The ratios of TWA and personal exposure of heavy metal(loid)s ranged from 0.91 to 1.53. Indoor pollution was the most significant factor of TWA exposure, accounting for 78.3-97.6% and 88.4-98.6% in the heating and non-heating period, respectively. Based on the results of redundancy analysis and risk assessment by TWA exposure, we concluded that TWA exposure could be used for qualitative investigation, as a substitute for personal exposure, but it may result in large bias when used for quantitative investigation. Larger sample size and more exposure scenarios can reduce the estimation error of TWA.


Subject(s)
Air Pollutants , Air Pollution, Indoor , Metals, Heavy , Air Pollutants/analysis , Air Pollution, Indoor/analysis , Cities , Environmental Exposure/analysis , Environmental Monitoring , Environmental Pollution/analysis , Heating , Metals, Heavy/analysis , Reproducibility of Results
7.
Huan Jing Ke Xue ; 42(5): 2143-2152, 2021 May 08.
Article in Chinese | MEDLINE | ID: mdl-33884783

ABSTRACT

The presence of heavy metals in indoor dust is a world-wide concern owing to its negative impact on humans. In this study, we collected indoor dust samples from urban and rural residential areas during the heating season in Taiyuan City. We then identified the concentrations of 11 heavy metals (Cd, Co, Cr, Pb, Mn, Ni, Cu, Zn, V, As, and Hg) using inductively coupled plasma-mass spectrometry. Based on the concentrations, we categorized the pollution levels of indoor dust using the geo-accumulation index and the pollution load index. We further identified the sources of heavy metals using the enrichment factor and principal component analysis. Finally, we evaluated the potential ecological risks of heavy metals via the potential ecological index. The results illustrated that ① with the exception of Co, Mn, and V, the mean concentrations of Cd, Cr, Cu, Ni, Pb, As, Zn, and Hg in indoor dust were higher than the soil background values of Shanxi Province. There was a significant difference (P<0.05) in the concentrations of Co, Cr, Cu, Mn, Ni, and Hg between the urban and rural areas. ② Overall, the pollution degree of heavy metals in indoor dust was identified as moderate in the urban area of Taiyuan City, but slight in the rural area. The indoor dust sample in the urban area was not contaminated by Co, Mn, and V. However, it was slightly polluted by As, Ni, and Hg. In addition, it was close to moderately polluted by Cd, Cr, Cu, Pb, and Zn. In the rural area, the pollution degrees of all the metals, except for Hg and V, in indoor dust were lower than those in the urban area. ③ The As, Cd, Cu, Pb, Zn, and Hg in indoor dust for both urban and rural areas might have mainly originated from anthropogenic sources. The pollution sources were mainly transportation and industry in the urban area and coal combustion and indoor smoking in the rural area. The Co, Cr, Mn, Ni, and V in indoor dust in Taiyuan City might have mainly originated from natural sources. ④ The ecological risk of heavy metal pollution in indoor dust for both the urban and rural areas of Taiyuan City was relatively high, with integrated ecological risk indexes of 359.43 and 471.02 in the urban and rural areas, respectively. In addition, Cd and Hg were the largest contributors.


Subject(s)
Dust , Metals, Heavy , China , Cities , Dust/analysis , Environmental Monitoring , Heating , Humans , Metals, Heavy/analysis , Risk Assessment , Seasons
8.
Huan Jing Ke Xue ; 42(4): 1688-1695, 2021 Apr 08.
Article in Chinese | MEDLINE | ID: mdl-33742804

ABSTRACT

Research on health and the economic losses caused by PM2.5 pollution nationwide is critical for pollution control planning. First, the spatiotemporal distribution of PM2.5 and exposure levels were simulated and analyzed using the air quality model (WRF-Chem) in China in 2016. Then, the health burden and economic loss caused by PM2.5 pollution were estimated using environmental health risk and environmental value assessment methods. Finally, the health and economic benefits from achieving specific PM2.5 control targets were estimated. In 2016 in China, high levels of PM2.5 were concentrated in Beijing-Tianjin-Hebei and the surrounding areas, the Yangtze River Delta, the Sichuan Basin, and the desert areas in northwest China. Furthermore, 71.49% of the total population of China was exposed to an environment with PM2.5 concentrations higher than 35 µg·m-3. Subsequently, the national PM2.5-related mortality was 1.06 million, accounting for 10.9% of the total deaths in China. Stroke and ischemic heart disease accounted for approximately 80% of the total PM2.5-related deaths caused by the five diseases studied. Meanwhile, the PM2.5 pollution resulted in economic losses of 705.93 billion yuan, which was 0.95% of the Gross Domestic Product (GDP) in 2016. There were significant spatial differences in the health burden and economic loss, which primarily occurred in regions with high PM2.5 levels or population density. Moreover, reducing PM2.5 to 35 µg·m-3 would only result in a 17.11% reduction in the health burden and economic loss, while a more exacting standard (reducing PM2.5 to 10 µg·m-3) would bring 80.47% of the health and economic benefits. It is suggested that environmental managers further strengthen their control to better protect the health and wealth benefits of residents, especially for sensitive groups, such as patients with cardio-cerebrovascular diseases, particularly in areas with high premature mortality.


Subject(s)
Air Pollutants , Air Pollution , Air Pollutants/adverse effects , Air Pollutants/analysis , Air Pollution/adverse effects , Air Pollution/analysis , Beijing , China/epidemiology , Environmental Pollution , Humans , Particulate Matter/adverse effects , Particulate Matter/analysis
9.
Occup Environ Med ; 2021 Feb 26.
Article in English | MEDLINE | ID: mdl-33637624

ABSTRACT

OBJECTIVES: This study aimed to evaluate whether PM2.5 exposure in a highly polluted area (>100 µg/m3) affects glucose and lipid metabolism in healthy adults. METHODS: We recruited 110 healthy adults in Baoding city, Hebei, China, and followed them up between 2017 and 2018. Personal air samplers were used to monitor personal PM2.5 levels. Eight glucose and lipid metabolism parameters were quantified. We performed the linear mixed-effect models to investigate the relationships between PM2.5 and glucose and lipid metabolism parameters. Stratified analyses were further performed according to sex and body mass index (BMI). RESULTS: The concentration of PM2.5 was the highest in spring, with a median of 232 µg/m3 and the lowest in autumn (139 µg/m3). After adjusting for potential confounders, we found that for each twofold increase in PM2.5, the median of insulin concentration decreased by 5.89% (95% CI -10.91% to -0.58%; p<0.05), and ox-LDL increased by 6.43% (95% CI 2.21% to 10.82%; p<0.05). Stratified analyses indicated that the associations were more pronounced in females, overweight and obese participants. CONCLUSIONS: Exposure to high PM2.5 may have deleterious effects on glucose and lipid metabolism. Females, overweight and obese participants are more vulnerable.

10.
Innovation (Camb) ; 2(1): 100071, 2021 Feb 28.
Article in English | MEDLINE | ID: mdl-33521765

ABSTRACT

The COVID-19 outbreak has already become a global pandemic and containing this rapid worldwide transmission is of great challenge. The impacts of temperature and humidity on the COVID-19 transmission rate are still under discussion. Here, we elucidated these relationships by utilizing two unique scenarios, repeated measurement and natural experiment, using the COVID-19 cases reported from January 23 - February 21, 2020, in China. The modeling results revealed that higher temperature was most strongly associated with decreased COVID-19 transmission at a lag time of 8 days. Relative humidity (RH) appeared to have only a slight effect. These findings were verified by assessing SARS-CoV-2 infectivity under the relevant conditions of temperature (4°C-37°C) and RH (> 40%). We concluded that temperature increase made an important, but not determined, contribution to restrain the COVID-19 outbreak in China. It suggests that the emphasis of other effective controlling polices should be strictly implemented to restrain COVID-19 transmission in cold seasons.

11.
Chemosphere ; 267: 129146, 2021 Mar.
Article in English | MEDLINE | ID: mdl-33338725

ABSTRACT

The effects of ambient fine particulate matter (PM2.5) exposure on blood pressure have been widely reported. However, there remains uncertainty regarding the underlying roles of particulate matter components. We aimed to investigate the association between ambient PM2.5 exposure and blood pressure, as well as the potential effects of trace metal(loid)s, in a repeated-measurement study that enrolled women of childbearing age. Our study included 35 participants from Hebei Province, China, each of whom was visited for five times. During each visit, we conducted questionnaire surveys, measured blood pressure, and collected blood. The daily PM2.5 exposure of participants was estimated according to their residential addresses using a spatiotemporal model that combined monitoring data with satellite measurements and chemical-transport model simulations. This model was used to calculate average PM2.5 concentrations in 1, 3, 7, 15, 30, and 60 days prior to each visit. Serum concentrations of various trace metal(loid)s were measured. A linear mixed-effects model was used to investigate associations among study variables. Overall, the mean (standard deviation) 60 days PM2.5 concentration over all five visits was 108.1(43.3) µg/m3. PM2.5 concentration was positively associated with both systolic and diastolic blood pressures. Likewise, ambient PM2.5 concentration was positively associated with serum concentrations of manganese and arsenic, and negatively associated with serum concentrations of nickel, tin, and chromium. Only the serum concentration of molybdenum was negatively associated with systolic blood pressure. We concluded that ambient PM2.5 exposure may contribute to elevated blood pressure, potentially by interfering with internal intake of various metal(loid)s in the human body.


Subject(s)
Air Pollutants , Air Pollution , Air Pollutants/analysis , Air Pollution/analysis , Blood Pressure , China , Environmental Exposure , Female , Humans , Metals , Particulate Matter/analysis
12.
Sci Total Environ ; 762: 143126, 2021 Mar 25.
Article in English | MEDLINE | ID: mdl-33121772

ABSTRACT

To investigate the characteristics and health risks of heavy metals in household dust in urban and rural areas during heating and non-heating period in 2016-2017, 762 dust samples and 381 questionnaires from 381 households were collected from Dalian, Taiyuan, Lanzhou, Shanghai, Wuhan, and Chengdu in China. The results indicated that Dalian was the most polluted city, while Shanghai and Chengdu were the least polluted cities during the study period. Longer ventilation times led to higher concentrations of heavy metals, and the weighting of heating duration exceeded that of heating type. Soil was the dominant contributor to household dust for Hg, Ni, Cu, Zn, and As, whereas Pb primarily originated from traffic. The non-carcinogenic and carcinogenic risks associated with heavy metals in household dust were acceptable, with ingestion being the primary exposure route. The risk of adverse health effects caused by heavy metal intake via household dust in urban areas was higher than that in rural areas, and increased during household heating period. Ingestion was the most significant route leading to adverse health effects due to heavy metals in household dust. The exception was the carcinogenic risk associated with Ni, which is known to enter the human body mainly via inhalation.


Subject(s)
Dust , Metals, Heavy , China , Cities , Dust/analysis , Environmental Monitoring , Humans , Metals, Heavy/analysis , Risk Assessment
13.
Chemosphere ; 263: 127925, 2021 Jan.
Article in English | MEDLINE | ID: mdl-32818847

ABSTRACT

Long-term exposure to fine particulate matter (PM2.5) poses a great threat to public health in China. To this end, the Chinese government promulgated the Air Pollution Prevention and Control Action Plan (the Action Plan) in 2013. However, the health benefits of the Action Plan have not been well explained. In this paper, the underlying causes of changes in premature mortality attributable to PM2.5 pollution and the response of this mitigation policy in China were explored using sensitivity analysis. The simulated annual average PM2.5 concentration reduced by 24.9% over mainland China from 2008 to 2016. Subsequently, national premature mortality would decrease by 14.4% from 1.14 million (95% CI: 0.54, 1.55) in 2008 to 0.98 million (95% CI: 0.44, 1.38) in 2016. Specifically, premature mortality reduced by 209,600 cases (-18.3%) owing to PM2.5 reduction during 2008-2016, of which 188,500 cases were from 2014 to 2016 due to the Action Plan in 2013. Note that the health benefits were limited when compared with air quality improvements, mainly due to that the IER functions have a stable curve at higher concentration intervals. Meanwhile, premature mortality would have increased by 14.2% from 2008 to 2016 owing to demographic changes, substantially weakening the impact of the decrease in PM2.5 and baseline mortality. The effectiveness of China's new air pollution mitigation policy was proved through the research. However, considering the non-linear response of mortality to PM2.5 changes and the aggravation of demography trends, stronger emission control steps should be further taken to protect public health in China.


Subject(s)
Air Pollution/statistics & numerical data , Environmental Exposure/statistics & numerical data , Particulate Matter/analysis , Air Pollutants/analysis , Air Pollution/analysis , China/epidemiology , Environmental Exposure/analysis , Humans , Mortality/trends , Mortality, Premature , Public Health
14.
Environ Int ; 143: 105950, 2020 10.
Article in English | MEDLINE | ID: mdl-32673910

ABSTRACT

BACKGROUND: Childhood obesity is a global health issue, and limited evidence suggests that air pollution may be a contributing factor. This study aims to examine whether exposure to fine particulate matter (PM2.5) is associated with obesity status in a nationally representative sample of schoolchildren in China. METHODS: The study population consisted of 41,439 schoolchildren of 6-17 years old, recruited from 30 provinces in China using a multi-stage stratified sampling method. Weights and heights were measured for all the participants, and sociodemographic information was collected using a questionnaire. The obesity status was classified following the Chinese national standards. The PM2.5 exposure was estimated as the 5-year average concentration at the school location for each participant. The association between obesity status and PM2.5 exposure was examined using weighted logistic regressions adjusted for potential confounders. RESULTS: The prevalence of normal weight, overweight, and obesity were 78.5%, 12.4%, and 9.0%, respectively. PM2.5 exposure averaged 59.8 ± 17.6 µg/m3 with a range of 30.5-115.2 µg/m3 among all the participants. The risk of obesity increased by 10.0% (95% confidence interval: 3.0-16.0%) per 10 µg/m3 increase in PM2.5 exposure. The PM2.5-associated risk was significantly elevated in older age groups and children living in urban areas (interaction p-values < 0.05). CONCLUSIONS: This national survey revealed that approximately 1 in 5 Chinese schoolchildren were overweight or obese. Exposure to PM2.5 in the ambient air was significantly associated with childhood obesity. The findings suggest the need for further research to uncover the roles of PM2.5 exposure in childhood obesity development.


Subject(s)
Air Pollutants , Air Pollution , Pediatric Obesity , Adolescent , Aged , Air Pollutants/adverse effects , Air Pollutants/analysis , Air Pollution/adverse effects , Air Pollution/analysis , Child , China/epidemiology , Cross-Sectional Studies , Environmental Exposure/adverse effects , Humans , Particulate Matter/adverse effects , Particulate Matter/analysis , Pediatric Obesity/epidemiology
15.
Sci Total Environ ; 742: 140643, 2020 Nov 10.
Article in English | MEDLINE | ID: mdl-32640394

ABSTRACT

Although recent assessments have quantified the impact of ambient PM2.5 on public health in China, air quality managers would benefit from assessing specific differences in premature mortality and its responses to air quality improvement. Using PM2.5 data simulated by an observation-fused air quality model and an integrated exposure-response model for the full range of PM2.5, we determined the premature mortality attributable to ambient PM2.5 across mainland China in 2016. Overall, the total number of PM2.5-related deaths nationwide was 1.31 million, of which lung cancer, chronic obstructive pulmonary disease, ischemic heart disease, and stroke represented 0.13, 0.13, 0.42, and 0.62 million, respectively. Per capita PM2.5-related mortality in China was 95 per 100,000 person-years, and that of elderly people aged ≥75 years (1166 deaths per 100,000) was much higher than that of young people aged 25-44 years (11 deaths per 100,000). Additionally, there were significant spatial differences in premature deaths, which mainly occurred in regions with high PM2.5 levels or/and population density. Halving deaths across mainland China required an average of 63% reduction of PM2.5 nationwide and a decrease by 73% in high concentration regions exceeding 70 µg/m3 and 19% in low concentration locales below 10 µg/m3. Moreover, reducing PM2.5 to the WHO interim target I (IT-1) of 35 µg/m3 would only result in a 12.6% reduction in premature mortality, while a more exacting standard (reducing PM2.5 to 10 µg/m3) would avoid 73.0% of mortality. In particular, there is a large potential for reducing the high PM2.5-related mortality in heavily polluted locales. In conclusion, to further reduce premature mortality across mainland China, targets stricter than the IT-1 and tight policies to improve air quality and protect public health are necessary, especially for vulnerable groups such as the elderly and patients with cardio-cerebrovascular diseases, particularly in areas with high premature mortality.


Subject(s)
Air Pollutants/analysis , Air Pollution , Adolescent , Adult , Aged , China , Environmental Exposure , Humans , Mortality, Premature , Particulate Matter/analysis
16.
ChemSusChem ; 13(18): 4954-4966, 2020 Sep 18.
Article in English | MEDLINE | ID: mdl-32666698

ABSTRACT

Selective transformation of glycerol to propanal (PA) provides a feasible route towards the sustainable synthesis of high value-added chemicals. In this work, zirconium phosphate (ZrP) was studied as support and Ru and Co as metal sites for glycerol hydrogenolysis in a continuous-flow reactor. It was found that ZrP-supported Co-O species had a moderate selectivity to PA (49.5 %) in glycerol hydrogenolysis. Notably, once Ru species were doped into CoO/ZrP, the resulting catalyst exhibited not only an outstanding catalytic performance for glycerol hydrogenolysis to PA (a selectivity of 80.2 % at full conversion), but also a high stability at least a 50 h long-term performance. The spent catalyst could be regenerated by calcining in air to remove carbonaceous deposits. Characterization indicated that the acid sites on ZrP played a very critical role in the dehydration of glycerol into acrolein (AE), that the distribution of Co was uniform, basically consistent with that of Zr, P and Ru, and that an especially close contact between Co-O and Ru species was formed on Ru/CoO/ZrP catalyst. The further activity tests and characterizations confirmed that there was a strong interaction between the dispersed Co-O species and Ru0 nanoparticles, which endowed Ru sites with high electronic density. This effect could play a role in facilitating the dissociation of H2 , and thus in promoting the hydrogenation reaction. Besides, DFT calculations suggested that the Co-O species can adsorb more strongly the C=C bond of the intermediate AE on a highly coordinatively unsaturated Co (Cocus ) site and thus lead to preferential hydrogenation at the C=C bond of AE to PA.

17.
Chemosphere ; 252: 126533, 2020 Aug.
Article in English | MEDLINE | ID: mdl-32217410

ABSTRACT

Despite frequent detection of atrazine (ATZ) and its degradates (including hydroxyatrazine, ATZ-OH; deethylatrazine, DEA; deisopropylatrazine, DIA; and deethyldeisopropylatrazine, DACT) in a variety of water bodies, documentation of their occurrence and distribution in tap water in China is still scarce. A nationwide survey about ATZ and its degradates (ATZs) in tap water from 31 provinces in 7 regions of mainland China and Hong Kong was conducted during June 2019. At least one of the analytes was found in all the water samples (n = 884). The median sum concentrations of ATZs (ΣATZs) was 21.0 ng/L (range: 0.02 ng/L-3.04 µg/L). The predominant compounds of ATZs in tap water were ATZ and DEA, with a detection frequency of 99.5% and 98.0%, respectively, followed by ATZ-OH (87.3%), DACT (84.0%), and DIA (78.1%). Significant regional variations (p < 0.05) were found in the concentrations of ATZs in tap water, and the highest concentration of ΣATZs (median: 254 ng/L, range: 0.44 ng/L-3.04 µg/L) was found in Northeastern China, followed by Eastern (37.2 ng/L, 0.02-706 ng/L), Northern (30.2 ng/L, 0.04-317 ng/L), Central (29.3 ng/L, 0.04-256 ng/L), Southern (25.0 ng/L, 0.04-297 ng/L), Southwestern (17.2 ng/L, 0.02-388 ng/L), and Northwestern China (3.22 ng/L, 0.06-214 ng/L). The level of ΣATZs in groundwater from rural area of China was about 1/3 of that found in tap water. ATZs cannot be removed by boiling tap water. The highest estimated daily intake of ΣATZs (248 ng/kg-body weight/day) was found in the infant population of Changchun, Jilin, Northeastern China.


Subject(s)
Atrazine/analysis , Environmental Exposure/analysis , Water Pollutants, Chemical/analysis , Water Pollution, Chemical/statistics & numerical data , Atrazine/analogs & derivatives , China , Environmental Exposure/statistics & numerical data , Groundwater , Herbicides/analysis , Hong Kong , Humans , Triazines/analysis , Water
18.
Environ Sci Pollut Res Int ; 27(12): 13524-13533, 2020 Apr.
Article in English | MEDLINE | ID: mdl-32030582

ABSTRACT

By collecting daily data on measles cases, air pollutants, and meteorological data from 2005 to 2009 in Chengguan District of Lanzhou City, semi-parametric generalized additive model (GAM) was used to quantitatively study the impact of air pollutants and meteorological factors on daily measles cases. The results showed that air pollutants and meteorological factors had effect on the number of daily measles cases, and there was a certain lag effect. Except for SO2 and relative humidity, other factors showed statistically significant associations with daily measles cases: NO2 lag 6 days, PM10 and maximum temperature lag 5 days, minimum temperature and average temperature and average air pressure lag 4 days, visibility, and wind speed lag 3 days had the greatest impact on the number of daily measles cases. Under the optimum lag conditions, the number of daily measles cases increased by 15.1%, 17.6%, 7.0%, 116.6%, 98.6%, 85.7%, and 14.4% with the increase of 1 IQR in SO2, NO2, PM10, maximum temperature, minimum temperature, average temperature, and wind speed; with the increase of 1 IQR in average pressure, relative humidity, visibility, and daily measles cases decreased by 12.8%, 9.7%, and 13.1%, respectively. And different factors showed different seasonal effects. The effects of SO2 and temperature factors on daily measles cases were greater in spring and winter, but PM10 in summer.


Subject(s)
Air Pollutants/analysis , Air Pollution/analysis , Measles , China , Cities , Humans , Meteorological Concepts , Particulate Matter/analysis
19.
Environ Int ; 137: 105504, 2020 04.
Article in English | MEDLINE | ID: mdl-32032774

ABSTRACT

China has made great efforts towards air pollutant concentration control during the past five years, which has led to positive outcomes. However, air pollutant concentration focused efforts were considered separately from human exposure risk. And this might result in a misunderstanding that reducing exposure risk can only rely on the national level measures of air pollutant control. This study integrates the first Chinese survey of human activity patterns and the spatially continuous high-resolution PM2.5 concentration maps to reveal the spatial and temporal variations of China's air pollution exposure risk from 2013 to 2017. More importantly, the effects on risk reduction from multi-scale and multi-object perspectives (reductions of ambient PM2.5 concentrations by national or provincial measures and changes of individual behavior patterns by personal efforts) are deeply investigated. Results show that the reductions of PM2.5 concentration and associated reductions of exposure risk from 2013 to 2017 were 40% and 35.7%, respectively. They also showed that both the reduction of PM2.5 concentrations and change of personal behavior patterns were effective for risk reduction when China's total PM2.5 exposure risk was higher than 1.58. However, only individual behavior changes contributed to risk reduction for scenarios with state-level risk value below 1.58. For regional strategies, threshold values for PM2.5 exposure risk control differentiating national measures or personal efforts were spatially and temporally dependent. The role of personal behavior changes on PM2.5 exposure risk reduction was growing in these five years with concentration rapidly decreasing regions. The findings suggest that people-centered air pollution exposure risk prevention not only depends on government management for air pollution control, but also on individual changes of activity patterns. Efforts from the state and individuals are both essential for reducing air pollution exposure risk in China, especially growing individual efforts are needed in regions with the decreasing air pollutant concentrations in the coming future. Moreover, this study mainly discussed the PM2.5 exposure risk from the macroscopic perspective, the research at the microcosmic perspective is also needed in the further study.


Subject(s)
Air Pollutants , Air Pollution , Risk Reduction Behavior , Air Pollutants/toxicity , China , Environmental Exposure , Humans , Longitudinal Studies , Particulate Matter
20.
Sci Rep ; 10(1): 479, 2020 01 16.
Article in English | MEDLINE | ID: mdl-31949216

ABSTRACT

Air pollution is a major environmental health problem. The study of interaction between air pollution and human will benefit to the human health and well-being of community. Both a model for assessing population relative risk of air pollution exposure (MAPRRAPE) and air pollution concentration methods were applied in a case study to determine the optimal method in evaluating risk of population exposure to Sulfur Dioxide (SO2). The framework for building the MAPRRAPE was described in detail. Then, the spatial patterns of population by demographic characteristics exposed to SO2 from industrial, vehicle, and the mixture of industrial and vehicle pollution sources, as well as an in-depth quantitative investigation using correlation analysis were studied for further source appointment. The results showed that the MAPRRAPE was more reliable than air pollution concentration model in determining population exposure risks by demographic characteristics. The high risk areas of whites exposed to SO2 were larger than blacks and the other races due to a large number of whites, and other age groups exposed to SO2 were larger than children and the old people. In addition, the correlation analyses showed that the relative risks of population by demographic characteristics exposed to SO2 had a more significant correlation with vehicle pollution source than industrial pollution source. The results of source appointment thus demonstrated that vehicle pollution source was the main pollution source. This study suggests that there is a clear need for the implementation of programs and services that will reduce population exposed to air pollution with focusing on densely populated areas for an ultimate improvement of community health status and the environmental conditions.

SELECTION OF CITATIONS
SEARCH DETAIL
...