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1.
Phys Rev B ; 99(19)2019 May.
Article in English | MEDLINE | ID: mdl-38712021

ABSTRACT

Systems with embedded magnetic ions that exhibit a competition between magnetic order and disorder down to absolute zero can display unusual low-temperature behaviors of the resistivity, susceptibility, and specific heat. Moreover, the dynamic response of such a system can display hyperscaling behavior in which the relaxation back to equilibrium when an amount of energy E is given to the system at temperature T only depends on the ratio E/T. Ce(Fe0.755Ru0.245)2Ge2 is a system that displays these behaviors. We show that these complex behaviors are rooted in a fragmentation of the magnetic lattice upon cooling caused by a distribution of local Kondo screening temperatures, and that the hyperscaling behavior can be attributed to the flipping of the total magnetic moment of magnetic clusters that spontaneously form and order upon cooling. We present our arguments based on the review of two-decades worth of neutron scattering and transport data on this system, augmented with new polarized and unpolarized neutron scattering experiments.

2.
Nat Mater ; 17(10): 875-880, 2018 10.
Article in English | MEDLINE | ID: mdl-30224782

ABSTRACT

Although signatures of superconductivity in Dirac semimetals have been reported, for instance by applying pressure or using point contacts, our understanding of the topological aspects of Dirac semimetal superconductivity is still developing. Here, we utilize nanoscale phase-sensitive junction technology to induce superconductivity in the Dirac semimetal Bi1-xSbx. Our radiofrequency irradiation experiments then reveal a significant contribution of 4π-periodic Andreev bound states to the supercurrent in Nb-Bi0.97Sb0.03-Nb Josephson junctions. The conditions for a substantial 4π contribution to the supercurrent are favourable because of the Dirac cone's very broad transmission resonances and a measurement frequency faster than the quasiparticle poisoning rate. In addition, we show that a magnetic field applied in the plane of the junction allows tuning of the Josephson junctions from 0 to π regimes. Our results open the technologically appealing avenue of employing the topological bulk properties of Dirac semimetals for topological superconductivity research and topological quantum computer development.

3.
Proc Natl Acad Sci U S A ; 113(49): 13989-13994, 2016 12 06.
Article in English | MEDLINE | ID: mdl-27872287

ABSTRACT

The second-order phase transition into a hidden order phase in URu2Si2 goes along with an order parameter that is still a mystery, despite 30 years of research. However, it is understood that the symmetry of the order parameter must be related to the symmetry of the low-lying local electronic [Formula: see text]-states. Here, we present results of a spectroscopic technique, namely core-level nonresonant inelastic X-ray scattering (NIXS). This method allows for the measurement of local high-multipole excitations and is bulk-sensitive. The observed anisotropy of the scattering function unambiguously shows that the 5[Formula: see text] ground-state wave function is composed mainly of the [Formula: see text] with majority [Formula: see text] = [Formula: see text] + [Formula: see text] and/or [Formula: see text] singlet states. The incomplete dichroism indicates the possibility that quantum states of other irreducible representation are mixed into the ground state.

4.
J Phys Condens Matter ; 28(28): 285601, 2016 07 20.
Article in English | MEDLINE | ID: mdl-27218143

ABSTRACT

We report the magnetism and transport properties of the Heusler compound Fe2+x V1-x Al at -0.10 ⩽ x ⩽ 0.20 under pressure and a magnetic field. A metal-insulator quantum phase transition occurred at x ≈ -0.05. Application of pressure or a magnetic field facilitated the emergence of finite zero-temperature conductivity σ 0 around the critical point, which scaled approximately according to the power law (P - P c ) (γ) . At x ⩽ -0.05, a localized paramagnetic spin appeared, whereas above the ferromagnetic quantum critical point at x ≈ 0.05, itinerant ferromagnetism was established. At the quantum critical points at x = -0.05 and 0.05, the resistivity and specific heat exhibited singularities characteristic of a Griffiths phase appearing as an inhomogeneous electronic state.

5.
Sci Rep ; 5: 12421, 2015 Jul 23.
Article in English | MEDLINE | ID: mdl-26201499

ABSTRACT

There are two prerequisites for understanding high-temperature (high-Tc) superconductivity: identifying the pairing interaction and obtaining a correct description of the normal state from which superconductivity emerges. The nature of the normal state of iron-pnictide superconductors, and the role played by correlations arising from partially screened interactions, are still under debate. Here we show that the normal state of carefully annealed electron-doped BaFe(2-x)Co(x)As2 at low temperatures has all the hallmark properties of a local Fermi liquid, with a more incoherent state emerging at elevated temperatures, an identification made possible using bulk-sensitive optical spectroscopy with high frequency and temperature resolution. The frequency dependent scattering rate extracted from the optical conductivity deviates from the expected scaling M2 (ω, T) ∝ (hω)(2) + (pπkBT)(2) with p ≈ 1.47 rather than p = 2, indicative of the presence of residual elastic resonant scattering. Excellent agreement between the experimental results and theoretical modeling allows us to extract the characteristic Fermi liquid scale T0 ≈ 1700 K. Our results show that the electron-doped iron-pnictides should be regarded as weakly correlated Fermi liquids with a weak mass enhancement resulting from residual electron-electron scattering from thermally excited quasi-particles.

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