ABSTRACT
This study presents the first data on levels of natural radioactive elements in sediments from coastal ecosystems of the Republic of Congo. Sediment samples from five coastal sites were collected and analyzed by high-resolution gamma spectrometry for determination of activities of long-lived gamma-emitting radionuclides (234Th, 238U, 226Ra, 210Pb, 228Th, 228Ra, and 40 K). The specific activities were of the same order of magnitude as those measured in sediments of most countries neighboring the Republic of Congo. However, variations in activities were observed from one site to another and also from one sampling point to another within the same site without exceeding the global average reference values. It can be assumed, therefore, that no significant anthropogenic impact is perceptible in the study area. The most commonly used radiological hazard parameters, based mainly on 238U, 232Th, and 40 K activities, were assessed and the ERICA tool was applied to quantify the radiation exposure burden to human and biota resulting from radionuclides in sediments. Besides being useful for future monitoring efforts, the data produced in this work could be important for the worldwide database on radioactivity in the oceans and seas (MARIS) since no data are available in the Congolese marine environment.
Subject(s)
Ecosystem , Geologic Sediments , Radiation Monitoring , Geologic Sediments/chemistry , Congo , Risk Assessment , Water Pollutants, Radioactive/analysis , Thorium/analysis , Uranium/analysis , Radium/analysis , HumansABSTRACT
This paper presents the determination method of the exact geographical coordinates of aboveground nuclear tests (NT) epicenters based on the radioecological study results the example of the Semipalatinsk Nuclear Test Site. By testing the NT Epicenter software for determining the exact geographic coordinates of the NT centers, it was established that it is indeed possible to determine the exact coordinates of most of the aboveground NTs. Their locations are currently determined by the presence are currently determined by the presence of technogenic disturbance of the soil surface in the area of the alleged epicenter (the presence of a crater), as well as by comparing maps of radioactive contamination and a space image. The accuracy of the precise coordinates of the NT is highly dependent on the density of the auxiliary grid: the smaller the pitch of the auxiliary grid, the higher the accuracy of the NT epicenter.
Subject(s)
Radiation Monitoring , Radiation Monitoring/methods , Geography , Soil Pollutants, Radioactive/analysis , SoftwareABSTRACT
The research aimed to determine the spatiotemporal distribution patterns of radon activity concentrations in tap water of Yerevan city and assess radon-associated hazards using both deterministic and probabilistic approaches. This was accomplished by integrating one-year monitoring data of radon in water with water consumption habits among adult population clusters, which were identified through food frequency questionnaire in Yerevan. The study findings indicated variations in radon activity levels across administrative districts. The highest average activity concentrations were detected in Davtashen (7.07 Bq/L), while the lowest average was observed in Kanaker-Zeytun (1.57 Bq/L). The overall pattern of spatiotemporal variation during monitoring period revealed higher prevalence of radon in water in the northern and western parts of the city compared to the east and south, indicating different sources of drinking water. The radon-associated hazard assessment from water, using a deterministic approach (e.g., inhalation, ingestion, radon dissolution in blood, total effective dose), revealed values below the individual dose criterion (IDC) of 0.1 mSv/y. Monte Carlo simulation revealed a probability of exceeding IDC in specific water consumption-based groups. Residents of Yerevan who drink more than 3 L water daily with the highest observed activity concentration of 11.4 Bq/L, have an 86.26 % chance of exceeding IDC. Residents consuming 2.1 L water daily have a 7.02 % chance of exceeding IDC. The study highlights the importance of applied principles and methodologies for radon monitoring, particularly considering actual water consumption data and different risk assessment approaches. Considering the worst-case scenario results, it is recommended to keep tap water consumption up to 3 L per day, keeping the tap open longer to reduce radon levels. It also emphasizes the need for continued monitoring, given the variations in radon activity. The study provides valuable insights into radon exposure assessment, mitigation, and action plans in terms of water safety and public health.
Subject(s)
Drinking Water , Radiation Monitoring , Radon , Water Pollutants, Radioactive , Radon/analysis , Drinking Water/chemistry , Drinking Water/analysis , Water Pollutants, Radioactive/analysis , Radiation Monitoring/methods , Humans , Risk AssessmentABSTRACT
Americium-241 whole body and internal biokinetics were experimentally investigated in the euryhaline diamond sturgeon Acipenser gueldenstaedtii during its uptake from water and food, in fresh (FW) and brackish water (BW; 9 psu). Whole-body uptake rates of 241Am from water and subsequent depuration rates were quantified over 14 and 28 days, respectively, and assimilation efficiency (AE) of 241Am from diet (chironomid) was determined over 28 days. FW reduced the biological half-life of 241Am following aqueous uptake by an order of magnitude. In contrast BW greatly reduced 241Am assimilation efficiency (AE) from diet (chironomid) by several orders of magnitude (from an AE of 8.5% (FW) down to 0.003% (BW)). Hence, salinity per se is indicated as a major environmental variable in determining the radiological exposure of A. gueldenstaedtii to 241Am. During aqueous exposure BW appreciably increased 241Am activity concentrations in most body components, but aqueous or dietary exposure pathway at either salinity did not determine marked differences in how 241Am was distributed among six body components. The highly mineralized skin of A. gueldenstaedtii recurred as a major repository of 241Am in all experimental treatments, as high as 50% among body components, due to its internal transfer from diet, surface adsorption and/or active absorption from water. The indicated prominence of the aqueous, compared to the dietary, exposure pathway for 241Am accumulation by A. gueldenstaedtii suggests its radiological exposure would be enhanced by BW as it leads to its greater long-term retention, due to a much longer biological half-life.
Subject(s)
Americium , Fishes , Water Pollutants, Radioactive , Animals , Fishes/metabolism , Water Pollutants, Radioactive/metabolism , Americium/pharmacokinetics , Radiation MonitoringABSTRACT
In August 2023, the long-planned discharging of radioactive wastewater from the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) started after the confirmation of its feasibility and safety. As this water contains elevated amounts of tritium even after being diluted, a lot of resources have been invested in the monitoring of the Fukushima coastal region where the discharge outlet is located. We compare the first 3H surface activity concentrations from these measurements (up to the end of November 2023) with the available background values to evaluate a possible impact of the long-term discharging on humans and environmental levels of the radionuclide of interest in the same or nearby area. From our results, we can conclude that the joint effect of horizontal and vertical mixing has been significant enough to reduce tritium concentrations at the monitored locations in the region close to the FDNPP port two days after the end of the respective phase of the discharging beyond the detection limit of the applied analytical methods (â¼0.3 Bq L-1) which is by five orders of magnitude lower than safety limit for drinking water set by the World Health Organization (WHO). Moreover, the distant correlation analysis showed that tritium concentrations at stations located further than 1.4 km were very close to pre-discharge levels (â¼0.4 Bq L-1). We also estimated that the 3H activity concentration in the offshore Fukushima region would be elevated by 0.01 Bq L-1 at maximum over a year of continuous discharging, which is in concordance with the already published modeling papers and much less than the impact of the FDNPP accident in 2011.
Subject(s)
Fukushima Nuclear Accident , Radiation Monitoring , Tritium , Water Pollutants, Radioactive , Radiation Monitoring/methods , Water Pollutants, Radioactive/analysis , Tritium/analysis , JapanABSTRACT
The Irish Sea and the Baltic Sea are nowadays still the two most Cs-137 contaminated Seas worldwide. However, the origins of this contaminations are completely different. While the Baltic Sea was unintentionally contaminated due to global fallout after the accident in the Chernobyl nuclear powerplant in 1986, the Irish sea was intentionally used for low level liquid radioactive waste discharges from the Sellafield nuclear reprocessing facility (called Windscale until 1981) between the 1950s and 1990s. Nowadays, more than 30 years later, it is still possible to detect these contaminations in fish, water and sediments of both seas. Since fish are an important part of the human diet, monitoring Cs-137 levels in fish is essential for assessing the potential radiation exposure to humans. In 2019 and 2020 two surveys were dedicated to study the current levels of radioactive contamination in fish species from both Seas. During both surveys, fish samples were collected and analysed by gamma spectrometry later on. The results show that the average Cs-137 activity in benthic, demersal and pelagic fish species from the Baltic Sea are 2.7, 4.6 and 4.2, respectively, times higher than the corresponding values of the Irish Sea. Based on this and two other comparisons, it is concluded that the Baltic Sea is the most contaminated with Cs-137.
Subject(s)
Cesium Radioisotopes , Fishes , Radiation Monitoring , Water Pollutants, Radioactive , Water Pollutants, Radioactive/analysis , Radiation Monitoring/methods , Cesium Radioisotopes/analysis , Animals , Oceans and SeasABSTRACT
One of the major demands in gamma spectrometry of environmental samples is the accurate determination of activity concentration of present radionuclides (naturally occurring and those of artificial origin), due to the fact they are commonly of relatively low content. Thus, all these measurements have in common that the detection limit, in the spectral region of interest should be as low as possible. For this reason, the construction of a good passive, as well as active shield requires a detailed knowledge of the origin of the background events in the absence of an environmental sample. In addition, an analysis of the impact on detection limits due to the presence of the sample itself is also important. Also, the knowledge of the statistical basics for low-level counting is helpful to enable the best choice of detector characteristics (relative efficiency, peak to Compton ratio, resolution), measuring time, and required level of precaution against the different background contributions. In this paper, the background spectra of several gamma spectroscopy systems (with passive and active veto shields) are analyzed and discussed, regarding their capabilities for measurements of environmental samples. Furthermore, various environmental samples are analyzed by low-level gamma spectrometry, including the sample measurements in the presence of an active veto shield against cosmic-ray muons. The disturbance of radioactive equilibrium between members of radioactive series in the samples is commented on, together with the possibility of use of certain gamma lines (including their interference and the corresponding intensities) for radionuclide activities determination.
Subject(s)
Gamma Rays , Radiation Monitoring , Spectrometry, Gamma , Radiation Monitoring/methods , Spectrometry, Gamma/methodsABSTRACT
In June 2020, observations of anthropogenic radionuclides in Estonia, Finland, and Sweden that were not related to any acknowledged environmental release led to a comprehensive investigation on the source and cause of the unusual emissions. Several of the observed radionuclides were on the list of Comprehensive Nuclear-Test-Ban Treaty (CTBT) relevant radionuclides as an indicator of a potential nuclear test, and warranted detailed investigation. While analysis of aerosol samples coupled with Atmospheric Transport and Dispersion Modelling (ATDM) is a standard approach for environmental particulate releases, several new techniques were employed to better characterize the samples that allowed for useful inferences to be made. These inferences were crucial in forming the ultimate hypothesis for determining the facility type and location of the release.
Subject(s)
Air Pollutants, Radioactive , Radiation Monitoring , Finland , Sweden , Radiation Monitoring/methods , Air Pollutants, Radioactive/analysis , Radioisotopes/analysis , EstoniaABSTRACT
Radioactive effluents, originating from nuclear power plants, medical-nuclear applications, and various extraction industries worldwide, present a significant and dangerous contamination challenge. The concentrations of radioactive substances in wastewater, surface water, and potable water vary widely depending on the source and location. For example, cesium-137 levels in wastewater from nuclear facilities can range from 0.1 to 10 Bq/L, while tritium concentrations in surface water near nuclear plants can reach up to 100 Bq/L. Regulatory guidelines, like the maximum contaminant level of 0.185 Bq/L for combined radium-226 and radium-228 in drinking water, are critical for ensuring safety and environmental protection. Specifically, in Fukushima, Japan, cesium-137 levels in surface water range from 0.1 to 10 Bq/L due to the nuclear accident. In contrast, regions with natural uranium deposits, like parts of the United States, have reported radium-226 concentrations in potable water up to 1 Bq/L. These variations highlight the necessity for focused monitoring and evaluation to protect water quality and community health. Among various methods, Gamma spectrometry and inductively coupled plasma mass spectrometry are precise for radionuclide quantification, scintillation detectors, and ion exchange, and adsorption techniques efficiently remove radioactive substances from water. This critical review examines the sources, adverse effects, and analysis and remediation strategies for various radioactive elements in wastewater. By thoroughly evaluating the origins and potential dangers associated with radioactive effluents, this report emphasizes the urgent need for rigorous monitoring and effective treatment practices to maintain the integrity of water resources and ecosystems. PRACTITIONER POINTS: Comprehensive analysis of the radioactive elements frequently found in wastewater and drinking water. Assess the negative effects of radioactive elements in water systems. Examine the treatment methods used to eliminate radioactive pollutants from water sources. Outline effective methods and tactics for addressing and controlling radioactive contamination occurrences. Analyze the latest advancements in technology, regulatory enhancements, and optimal methods to guarantee the safety of drinking water and the sustainable handling of radioactive substances in wastewater.
Subject(s)
Drinking Water , Wastewater , Water Pollutants, Radioactive , Water Pollutants, Radioactive/analysis , Wastewater/chemistry , Drinking Water/chemistry , Elements, Radioactive/analysis , Radiation Monitoring/methods , Water Purification/methodsABSTRACT
The Fukushima Daiichi Nuclear Power Plant accident released considerable radionuclides into the environment. Radioactive particles, composed mainly of SiO2, emerged as distinctive features, revealing insights into the accident's dynamics. While studies extensively focused on high-volatile radionuclides like Cs, investigations into low-volatile nuclides such as 90Sr and Pu remain limited. Understanding their abundance in radioactive particles is crucial for deciphering the accident's details, including reactor temperatures and injection processes. Here, we aimed to determine 90Sr and Pu amounts in radioactive particles and provide essential data for understanding the formation processes and conditions within the reactor during the accident. We employed radiochemical analysis on nine radioactive particles and determined the amounts of 90Sr and Pu in these particles. 90Sr and Pu quantification in radioactive particles showed that the 90Sr/137Cs radioactivity ratio (corrected to March 11, 2011) aligned with core temperature expectations. However, the 239+240Pu/137Cs activity ratio indicated nonvolatile Pu introduction, possibly through fuel fragments. Analyzing 90Sr and Pu enhances our understanding of the Fukushima Daiichi accident. Deviations in 239+240Pu/137Cs activity ratios underscore nonvolatile processes, emphasizing the accident's complexity. Future research should expand this data set for a more comprehensive understanding of the accident's nuances.
Subject(s)
Fukushima Nuclear Accident , Plutonium , Strontium Radioisotopes , Nuclear Power Plants , Radiation Monitoring , Japan , Cesium RadioisotopesABSTRACT
131I has been extensively utilized in nuclear medicine, resulting in its widespread detection in coastal algal samples due to its discharge. Therefore, it is essential to monitor 131I in the coastal algal samples. γ-spectrometry is an expeditious method for measuring 131I, but this method requires the pretreatment of the algal sample. The effect on 131I in the algal sample during the oven-drying treatment is unclear. In this study, the Laminaria japonica Areschoug and Sargassum vachellianum Greville were collected at two locations and analyzed for 131I using γ-spectrometry. Additionally, the content of iodine was measured using an Inductively Coupled Plasma-Mass Spectrometer (ICP-MS) to clarify the effect of 131I loss during drying treatment at different temperatures. The results demonstrated that the dried Laminaria and Sargassum samples had calculated 131I activity concentration relative standard deviations (RSDs) of 6.34 % and 16.31 %, respectively, while the fresh samples exhibited RSDs of 11.70 % and 15.57 %. Additionally, the iodine content RSDs in the dried samples were 9.19 % for Laminaria and 10.34 % for Sargassum. Significantly, discrepancies in 131I activity concentration between the fresh and dried Laminaria and Sargassum were 5.4 % and 10.3 %. These findings indicate that the temperature factor in drying has no effect on 131I loss in Laminaria and Sargassum in the range of 70 °C-110 °C.
Subject(s)
Iodine Radioisotopes , Laminaria , Spectrometry, Gamma , Water Pollutants, Radioactive , Iodine Radioisotopes/analysis , Water Pollutants, Radioactive/analysis , Laminaria/chemistry , Spectrometry, Gamma/methods , Radiation Monitoring/methods , Temperature , Sargassum/chemistryABSTRACT
The present study focused on the distribution of uranium in groundwater samples collected from various sources in the Chikkaballapur district and its associated risk in humans. Seventy-five groundwater samples were collected during pre-monsoon and post-monsoon seasons and were analysed for uranium concentration along with different water quality parameters. The uranium concentration ranged from 0.23 to 285.23 µg/L in the pre-monsoon season and from 0.02 to 107.87 µg/L in the post-monsoon season. More than 90% of samples, except a few, were under the safe limits of 60 µg/L as directed by the Department of Atomic Energy (DAE) of India's Atomic Energy Regulatory Board (AERB). The study analysed physicochemical parameters like pH, total dissolved solids (TDS), nitrate, total hardness, phosphate, sulphate and fluoride in collected water samples. Out of all samples, few samples noted higher values of TDS, nitrate and fluoride. Their correlation along with uranium is detailed in the study. Owing to its slightly elevated content, an evaluation of the radiological and chemical hazards associated with uranium consumption was analysed. When the risk resulting from chemical toxicity was evaluated, relatively few samples had a hazard quotient (HQ) score higher than 1, which suggested that the people were vulnerable to chemical danger. This study also evaluates the dangers of elevated uranium levels in groundwater samples to the general public's health. It also acknowledges the importance of routinely evaluating and treating the drinking water sources in the region.
Subject(s)
Groundwater , Uranium , Water Pollutants, Radioactive , Uranium/analysis , India , Groundwater/chemistry , Risk Assessment , Water Pollutants, Radioactive/analysis , Humans , Water Pollutants, Chemical/analysis , Environmental Monitoring , Radiation MonitoringABSTRACT
This study investigates the radon concentration in groundwater in Kupwara, the northernmost district of the Kashmir valley. It further assesses the annual effective dose experienced by the district's diverse population-infants, children, and adults-attributable to both inhalation of airborne radon released from drinking water and direct ingestion. In addition to this, the calculation of gamma dose rate is also carried out at each of the sampling site of radon. A portable radon-thoron monitor and a portable gamma radiation detector were respectively employed to estimate the activity concentration of radon in water samples and to measure the gamma dose rate. The radon concentration was found to exhibit variability from a minimum of 2.9 BqL-1 to a maximum of 197.2 BqL-1, with a mean of 26.3 BqL-1 and a standard deviation of 23.3 BqL-1. From a total of 85 samples, 10.6% of the samples had radon activity concentrations exceeding the permissible limits of 40 BqL-1 set by the United Nations Scientific Committee on Effects of Atomic Radiations as reported by UNSCEAR (Sources and effects of ionizing radiation, 2008) and only 1.2% of the samples have radon activity concentration exceeding the permissible limits of 100 BqL-1 set by the World Health Organization as reported by WHO (WHO guidelines for drinking-water quality, World Health Organization, Geneva, 2008). The mean of the annual effective dose due to inhalation for all age groups as well as the annual ingestion dose for infants and children, surpasses the World Health Organization's limit of 100 µSv y-1 as reported by WHO (WHO guidelines for drinking-water quality, World Health Organization, Geneva, 2008). The observed gamma radiation dose rate in the vicinity of groundwater radon sites ranged from a minimum of 138 nSv h-1 to a maximum of 250 nSv h-1. The data indicated no significant correlation between the dose rate of gamma radiation and the radon levels in the groundwater. Radon concentration of potable water in the study area presents a non-negligible exposure pathway for residents. Therefore, the judicious application of established radon mitigation techniques is pivotal to minimize public health vulnerabilities.
Subject(s)
Groundwater , Radiation Monitoring , Radon , Water Pollutants, Radioactive , Radon/analysis , Groundwater/chemistry , India , Water Pollutants, Radioactive/analysis , Humans , Drinking Water/chemistry , Drinking Water/analysis , Infant , Child , Radiation Dosage , Gamma Rays , Radiation Exposure/analysis , AdultABSTRACT
The invasion of Ukraine and military operations around Ukrainian nuclear power plants and other nuclear facilities have prompted us to search for radiocaesium in mosses from the Kopacki Rit Nature Park in Croatia, since mosses are known bioindicators of airborne radioactive pollution, and Kopacki Rit is a known low radiocaesium background area. Sampling was finished in August 2023, and our analysis found no elevated radiocaesium levels. Kopacki Rit therefore remains a suitable place for future detection of anthropogenic radioactive pollutants.
Subject(s)
Cesium Radioisotopes , Radiation Monitoring , Croatia , Ukraine , Cesium Radioisotopes/analysis , Radiation Monitoring/methods , Nuclear Power Plants , Air Pollutants, Radioactive/analysis , HumansABSTRACT
Surgical procedures involving the use of x-rays in the operating room (OR) have increased in recent years, thereby increasing the exposure of OR staff to ionizing radiation. An individual dosimeter makes it possible to record the radiation exposure to which these personnel are exposed, but there is a lack of compliance in the wearing of these dosimeters for several practical reasons. This makes the dose results obtained unreliable. To try to improve the rate of dosimeter wearing in the OR, the Dosibadge project studied the association of the individual dosimeter with the hospital access badge, forming the Dosibadge. Through a study performed at the Tours University Hospital in eight different ORs for two consecutive periods of 3 months. The results show a significant increase in the systematic use of the dosimeter thanks to the Dosibadge, which improves the reliability of the doses obtained on the dosimeters and the monitoring of personnel. The increase is especially marked with clinicians. Following these results and the very positive feedback to this first single-centre study, we are then planning a second multicentre study to validate our proof of concept on different sites, with the three brands of individual dosimeters used in France i.e. dosimeters supplied by Dosilab; Landauer and IRSN.
Subject(s)
Occupational Exposure , Operating Rooms , Radiation Dosage , Radiation Dosimeters , Radiation Monitoring , Occupational Exposure/analysis , Occupational Exposure/prevention & control , Humans , Radiation Monitoring/methods , X-Rays , Radiation Protection , Radiation Exposure/analysis , Equipment DesignABSTRACT
As the number of coastal nuclear facilities rapidly increases and the wastewater from the Fukushima Nuclear Plant has been discharged into the Pacific Ocean, the nuclear environmental safety of China's marginal seas is gaining increased attention along with the heightened potential risk of nuclear accidents. However, insufficient work limits our understanding of the impact of human nuclear activities on the Yellow Sea (YS) and the assessment of their environmental process. This study first reports the 129I and 127I records of posthuman nuclear activities in the two YS sediments. Source identification of anthropogenic 129I reveals that, in addition to the gaseous 129I release and re-emission of oceanic 129I discharged from the European Nuclear Fuel Reprocessing Plants (NFRPs), the Chinese nuclear weapons testing fallout along with the global fallout is an additional 129I input for the continental shelf of the YS. The 129I/127I atomic ratios in the North YS (NYS) sediment are significantly higher than those in the other adjacent coastal areas, attributed to the significant riverine input of particulate 129I by the Yellow River. Furthermore, we found a remarkable 129I latitudinal disparity in the sediments than those in the seawaters in the various China seas, revealing that sediments in China's marginal seas already received a huge anthropogenic 129I from terrigenous sources via rivers and thus became a significant sink of anthropogenic 129I. This study broadens an insight into the potential impacts of terrigenous anthropogenic pollution on the Chinese coastal marine radioactive ecosystem.
Subject(s)
Geologic Sediments , Radiation Monitoring , Rivers , Geologic Sediments/chemistry , Rivers/chemistry , China , Water Pollutants, Radioactive/analysis , Oceans and Seas , Humans , Iodine Radioisotopes/analysisABSTRACT
The present study attempts to obtain an a priori estimate of the absorbed dose received by an individual engaged in the reconnaissance survey in Uranium exploration using a predictive mathematical regression analysis. Other radiation safety parameters such as excess lifetime cancer risk are also calculated. Study reflects that the proper handling of naturally occurring radioactive materials accounts for an absorbed dose significantly less than the prescribed limit.
Subject(s)
Occupational Exposure , Radiation Monitoring , Uranium , Uranium/analysis , Humans , India , Radiation Monitoring/methods , Occupational Exposure/analysis , Radiation Dosage , Radiation Protection/methods , Risk Assessment/methods , Radiation Exposure/analysis , Neoplasms, Radiation-Induced/prevention & control , Neoplasms, Radiation-Induced/etiology , Neoplasms, Radiation-Induced/epidemiologyABSTRACT
Groundwater is in direct contact with the soil and rocks that dissolve many compounds and minerals including uranium and its daughter products. 210Po is one of the decay products of 238U series that cause internal radiation dose in humans when consumed in the form of water and food, including sea food. Therefore, activities of 210Po have been studied in ground and surface water, and in food samples that are commonly used in Chamarajanagar region of Karnataka, India. The average 210Po concentration in bore well water samples and surface water samples are 3.21 and 1.85 mBq L-1, respectively. In raw rice and wheat, the average values of 210Po are 96 and 41 mBq kg-1, respectively. In millets and pulses, the average activity of 210Po is 157 and 79 mBq kg-1, respectively. Among food items, the highest activity of 1.3 kBq kg-1 is observed in marine crabs and the lowest activity of 2.6 mBq kg-1 is found in milk samples. The average ingestion dose due to 210Po in ground and surface water are 2.8 and 1.62 µSv y-1, respectively. The ingestion dose due to various food samples to the population is also calculated. Total ingestion dose due to 210Po to pure vegetarian population and general population are 38.09 and 590.80 µSv y-1, respectively. The concentration of 210Po in water samples and food samples of this region are in a comparable range with the world and Indian average values and lies well below the recommended guideline level.
Subject(s)
Food Contamination, Radioactive , Polonium , Radiation Dosage , Radiation Monitoring , Water Pollutants, Radioactive , India , Food Contamination, Radioactive/analysis , Polonium/analysis , Radiation Monitoring/methods , Water Pollutants, Radioactive/analysis , Humans , Groundwater/analysisABSTRACT
Determination of uranium isotopes in ground water plays a key role in assessment of geochemical condition of ground water and for estimating ingestion dose received by the general public because of uranium intake through drinking water. An attempt has been made in the present study to estimate isotopic composition and activity ratios (AR) of uranium isotopes by analysing the ground water samples using alpha spectrometry. Associated age-dependent ingestion dose was also calculated for the public of different age groups. 238U, 235U and 234U activity concentration was found to vary in the ranges of 5.85 ± 1.19 to 76.67 ± 4.16, < 0.90 to 3.15 ± 0.84 and 6.52 ± 1.25 to 107.02 ± 4.92 mBq/L, respectively. 235U/238U AR varies from 0.038 to 0.068 with an average of 0.047 which is close to 0.046 implies that uranium in the ground water is from natural origin. Uranium concentration was found to vary in the range of 0.47 ± 0.10 µg/L to 6.20 ± 0.34 µg/L with a mean value of 3.01 ± 0.23 µg/L, which is much lower than national as well as international recommendation value. Annual ingestion dose to the public of all age groups for uranium intake through drinking water ranges from 0.60 ± 0.11 to 19.50 ± 1.03 µSv/y.
Subject(s)
Radiation Dosage , Radiation Monitoring , Uranium , Water Pollutants, Radioactive , Uranium/analysis , Water Pollutants, Radioactive/analysis , Humans , Radiation Monitoring/methods , Drinking Water/analysis , Groundwater/analysis , Child , Adult , Age Factors , Alpha Particles , Spectrum Analysis/methods , Adolescent , Child, Preschool , Young AdultABSTRACT
All organisms on the earth-crest are exposed to natural background radiation since the evolution of the earth, as many environmental matrices such as soil, air, water bodies, vegetation, etc., act as the sources of natural radioactivity. The present study deals with the evaluation of indoor concentration of 222Rn (radon) in different dwellings with various construction materials used for the roof and floor in the industrial sites of Kannur district, Kerala. A pinhole-based dosemeter coupled with LR-115 Solid State Nuclear Track Detector and Direct Radon Progeny Sensor (DRPS) were respectively used for the measurement of indoor radon concentration and equilibrium equivalent concentration of radon. The indoor radon concentrations were found to vary from 102.30 Bqm-3 to 184.75 Bqm-3 and the values were within the recommended limits provided by International Commission on Radiological Protection (ICRP). The annual effective doses and excess lifetime cancer risks were observed in the range of 2.58-4.66 mSvy-1 and 7.68 × 10-3-15.60 × 10-3, respectively, and both exceed the world average values recommended by United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR) 2000. The study shows that, the houses with marble floors and concrete roofs have comparatively higher values of radon concentration, which indicates the significant contribution of construction materials to the enhanced radiation levels inside the dwellings.