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1.
Sci Rep ; 12(1): 9356, 2022 Jun 07.
Artículo en Inglés | MEDLINE | ID: mdl-35672354

RESUMEN

This paper presents the results of the development of a mathematical model and numerical simulation of the ascent in the atmosphere of a vertically directed jet fed by the heat of condensation of water vapor on a hygroscopic aerosol introduced into the jet at the start. The possibility of creating artificial convective clouds depending on jet parameters, condensation heat value and vertical profiles of wind speed, air temperature and humidity has been evaluated. Numerical experiments showed that the motion of a high-speed and high-temperature jet in the atmosphere has a complex turbulent nature. As the jet ascends, it expands, losing superheat and velocity. The temperature of the jet decreases faster than the velocity, so the jet rises slightly above the level at which its superheat disappears. The jet's ascent height increases as the humidity of the air and the vertical temperature gradient increase. Wind causes the jet to deform, bend, and decrease the height of ascent. Feed the jet with condensation heat results in a significant increase in jet lift height. This is particularly effective in the case of introducing into the jet two-layer NaCl/TiO2 nanoaerosol, which is capable of absorbing water vapor in an amount significantly greater than its mass. The simulation results are encouraging in the possibility of creating artificial updrafts that can lead to the formation of convective clouds and precipitation on days with favorable atmospheric conditions, when wind speed in the sub-cloud layer is < 6 m/s, air humidity is > 65%, and the temperature lapse rate is > 7.5 °C/km.

2.
ACS Nano ; 11(12): 12318-12325, 2017 12 26.
Artículo en Inglés | MEDLINE | ID: mdl-29149559

RESUMEN

Cloud-seeding materials as a promising water-augmentation technology have drawn more attention recently. We designed and synthesized a type of core/shell NaCl/TiO2 (CSNT) particle with controlled particle size, which successfully adsorbed more water vapor (∼295 times at low relative humidity, 20% RH) than that of pure NaCl, deliquesced at a lower environmental RH of 62-66% than the hygroscopic point (hg.p., 75% RH) of NaCl, and formed larger water droplets ∼6-10 times its original measured size area, whereas the pure NaCl still remained as a crystal at the same conditions. The enhanced performance was attributed to the synergistic effect of the hydrophilic TiO2 shell and hygroscopic NaCl core microstructure, which attracted a large amount of water vapor and turned it into a liquid faster. Moreover, the critical particle size of the CSNT particles (0.4-10 µm) as cloud-seeding materials was predicted via the classical Kelvin equation based on their surface hydrophilicity. Finally, the benefits of CSNT particles for cloud-seeding applications were determined visually through in situ observation under an environmental scanning electron microscope on the microscale and cloud chamber experiments on the macroscale, respectively. These excellent and consistent performances positively confirmed that CSNT particles could be promising cloud-seeding materials.

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