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1.
Nat Commun ; 10(1): 2564, 2019 06 12.
Artículo en Inglés | MEDLINE | ID: mdl-31189878

RESUMEN

Unconventional surface states protected by non-trivial bulk orders are sources of various exotic quantum transport in topological materials. One prominent example is the unique magnetic orbit, so-called Weyl orbit, in topological semimetals where two spatially separated surface Fermi-arcs are interconnected across the bulk. The recent observation of quantum Hall states in Dirac semimetal Cd3As2 bulks have drawn attention to the novel quantization phenomena possibly evolving from the Weyl orbit. Here we report surface quantum oscillation and its evolution into quantum Hall states in Cd3As2 thin film samples, where bulk dimensionality, Fermi energy, and band topology are systematically controlled. We reveal essential involvement of bulk states in the quantized surface transport and the resultant quantum Hall degeneracy depending on the bulk occupation. Our demonstration of surface transport controlled in film samples also paves a way for engineering Fermi-arc-mediated transport in topological semimetals.

2.
Sci Rep ; 9(1): 1672, 2019 Feb 08.
Artículo en Inglés | MEDLINE | ID: mdl-30737424

RESUMEN

We investigated the fundamental physical properties in the ultra-quantum limit state of bismuth through measurements of magnetoresistance, magnetization, magnetostriction, and ultrasound attenuation in magnetic fields up to 60T. For magnetic fields applied along the bisectrix direction of a single crystal, a drastic sign reversal in magnetostriction was observed at approximately 39T, which could be ascribed to the complete valley polarization in the electron Fermi pockets. The application of magnetic fields along the binary direction presented an anomalous feature at approximately 50T only in the magnetoresistance. The emergence of a field-induced splitting of a valley was proposed as a possible origin of this anomaly.

3.
Sci Adv ; 4(6): eaat3374, 2018 06.
Artículo en Inglés | MEDLINE | ID: mdl-29942862

RESUMEN

The travel of heat in insulators is commonly pictured as a flow of phonons scattered along their individual trajectory. In rare circumstances, momentum-conserving collision events dominate, and thermal transport becomes hydrodynamic. One of these cases, dubbed the Poiseuille flow of phonons, can occur in a temperature window just below the peak temperature of thermal conductivity. We report on a study of heat flow in bulk black phosphorus between 0.1 and 80 K. We find a thermal conductivity showing a faster than cubic temperature dependence between 5 and 12 K. Consequently, the effective phonon mean free path shows a nonmonotonic temperature dependence at the onset of the ballistic regime, with a size-dependent Knudsen minimum. These are hallmarks of Poiseuille flow previously observed in a handful of solids. Comparing the phonon dispersion in black phosphorus and silicon, we show that the phase space for normal scattering events in black phosphorus is much larger. Our results imply that the most important requirement for the emergence of Poiseuille flow is the facility of momentum exchange between acoustic phonon branches. Proximity to a structural transition can be beneficial for the emergence of this behavior in clean systems, even when they do not exceed silicon in purity.

4.
Nat Commun ; 8(1): 2274, 2017 12 22.
Artículo en Inglés | MEDLINE | ID: mdl-29273770

RESUMEN

A well known semiconductor Cd3As2 has reentered the spotlight due to its unique electronic structure and quantum transport phenomena as a topological Dirac semimetal. For elucidating and controlling its topological quantum state, high-quality Cd3As2 thin films have been highly desired. Here we report the development of an elaborate growth technique of high-crystallinity and high-mobility Cd3As2 films with controlled thicknesses and the observation of quantum Hall effect dependent on the film thickness. With decreasing the film thickness to 10 nm, the quantum Hall states exhibit variations such as a change in the spin degeneracy reflecting the Dirac dispersion with a large Fermi velocity. Details of the electronic structure including subband splitting and gap opening are identified from the quantum transport depending on the confinement thickness, suggesting the presence of a two-dimensional topological insulating phase. The demonstration of quantum Hall states in our high-quality Cd3As2 films paves a road to study quantum transport and device application in topological Dirac semimetal and its derivative phases.

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