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1.
Phys Rev Lett ; 132(7): 076001, 2024 Feb 16.
Artículo en Inglés | MEDLINE | ID: mdl-38427861

RESUMEN

The shot noise in tunneling experiments reflects the Poissonian nature of the tunneling process. The shot-noise power is proportional to both the magnitude of the current and the effective charge of the carrier. Shot-noise spectroscopy thus enables us, in principle, to determine the effective charge q of the charge carriers of that tunnel. This can be used to detect electron pairing in superconductors: In the normal state, the noise corresponds to single electron tunneling (q=1e), while in the paired state, the noise corresponds to q=2e. Here, we use a newly developed amplifier to reveal that in typical mesoscopic superconducting junctions, the shot noise does not reflect the signatures of pairing and instead stays at a level corresponding to q=1e. We show that transparency can control the shot noise, and this q=1e is due to the large number of tunneling channels with each having very low transparency. Our results indicate that in typical mesoscopic superconducting junctions, one should expect q=1e noise and lead to design guidelines for junctions that allow the detection of electron pairing.

2.
Phys Chem Chem Phys ; 26(4): 3139-3151, 2024 Jan 24.
Artículo en Inglés | MEDLINE | ID: mdl-38189548

RESUMEN

The recent discovery of cable bacteria has greatly expanded the known length scale of biological electron transport, as these multi-cellular bacteria are capable of mediating electrical currents across centimeter-scale distances. To enable such long-range conduction, cable bacteria embed a network of regularly spaced, parallel protein fibers in their cell envelope. These fibers exhibit extraordinary electrical properties for a biological material, including an electrical conductivity that can exceed 100 S cm-1. Traditionally, long-range electron transport through proteins is described as a multi-step hopping process, in which the individual hopping steps are described by Marcus electron transport theory. Here, we investigate to what extent such a classical hopping model can explain the conductance data recorded for individual cable bacterium filaments. To this end, the conductive fiber network in cable bacteria is modelled as a set of parallel one-dimensional hopping chains. Comparison of model simulated and experimental current(I)/voltage(V) curves, reveals that the charge transport is field-driven rather than concentration-driven, and there is no significant injection barrier between electrodes and filaments. However, the observed high conductivity levels (>100 S cm-1) can only be reproduced, if we include much longer hopping distances (a > 10 nm) and lower reorganisation energies (λ < 0.2 eV) than conventionally used in electron relay models of protein structures. Overall, our model analysis suggests that the conduction mechanism in cable bacteria is markedly distinct from other known forms of long-range biological electron transport, such as in multi-heme cytochromes.


Asunto(s)
Bacterias , Transporte de Electrón , Bacterias/química , Conductividad Eléctrica
3.
Nat Commun ; 14(1): 8503, 2023 Dec 21.
Artículo en Inglés | MEDLINE | ID: mdl-38129381

RESUMEN

The temperature dependent order parameter provides important information on the nature of magnetism. Using traditional methods to study this parameter in two-dimensional (2D) magnets remains difficult, however, particularly for insulating antiferromagnetic (AF) compounds. Here, we show that its temperature dependence in AF MPS3 (M(II) = Fe, Co, Ni) can be probed via the anisotropy in the resonance frequency of rectangular membranes, mediated by a combination of anisotropic magnetostriction and spontaneous staggered magnetization. Density functional calculations followed by a derived orbital-resolved magnetic exchange analysis confirm and unravel the microscopic origin of this magnetization-induced anisotropic strain. We further show that the temperature and thickness dependent order parameter allows to deduce the material's critical exponents characterising magnetic order. Nanomechanical sensing of magnetic order thus provides a future platform to investigate 2D magnetism down to the single-layer limit.

4.
Nano Lett ; 23(15): 6973-6978, 2023 Aug 09.
Artículo en Inglés | MEDLINE | ID: mdl-37466285

RESUMEN

Magnetostrictive coupling has recently attracted interest as a sensitive method for studying magnetism in two-dimensional (2D) materials by mechanical means. However, its application in high-frequency magnetic actuators and transducers requires rapid modulation of the magnetic order, which is difficult to achieve with external magnets, especially when dealing with antiferromagnets. Here, we optothermally modulate the magnetization in antiferromagnetic 2D material membranes of metal phosphor trisulfides (MPS3), to induce a large high-frequency magnetostrictive driving force. From the analysis of the temperature-dependent resonance amplitude, we provide evidence that the force is due to a thermo-magnetostrictive effect, which significantly increases near the Neél temperature, due to the strong temperature dependence of the magnetization. By studying its angle dependence, we find the effect is observed to follow anisotropic magnetostriction of the crystal lattice. The results show that the thermo-magnetostrictive effect results in a strongly enhanced thermal expansion force near the critical temperature of magnetostrictive 2D materials, which can enable more efficient actuation of nano-magnetomechanical devices and can also provide a route for studying the high-frequency coupling among magnetic, mechanical, and thermodynamic degrees of freedom down to the 2D limit.

5.
Nat Commun ; 14(1): 490, 2023 Jan 30.
Artículo en Inglés | MEDLINE | ID: mdl-36717574

RESUMEN

Quantum sensing has developed into a main branch of quantum science and technology. It aims at measuring physical quantities with high resolution, sensitivity, and dynamic range. Electron spins in diamond are powerful magnetic field sensors, but their sensitivity in the microwave regime is limited to a narrow band around their resonance frequency. Here, we realize broadband microwave detection using spins in diamond interfaced with a thin-film magnet. A pump field locally converts target microwave signals to the sensor-spin frequency via the non-linear spin-wave dynamics of the magnet. Two complementary conversion protocols enable sensing and high-fidelity spin control over a gigahertz bandwidth, allowing characterization of the spin-wave band at multiple gigahertz above the sensor-spin frequency. The pump-tunable, hybrid diamond-magnet sensor chip opens the way for spin-based gigahertz material characterizations at small magnetic bias fields.

6.
Phys Rev Lett ; 129(3): 037205, 2022 Jul 15.
Artículo en Inglés | MEDLINE | ID: mdl-35905351

RESUMEN

We propose to directly and quantum-coherently couple a superconducting transmon qubit to magnons-the quanta of the collective spin excitations, in a nearby magnetic particle. The magnet's stray field couples to the qubit via a superconducting quantum interference device. We predict a resonant magnon-qubit exchange and a nonlinear radiation-pressure interaction that are both stronger than dissipation rates and tunable by an external flux bias. We additionally demonstrate a quantum control scheme that generates magnon-qubit entanglement and magnonic Schrödinger cat states with high fidelity.

7.
ACS Nano ; 16(7): 11251-11258, 2022 Jul 26.
Artículo en Inglés | MEDLINE | ID: mdl-35816615

RESUMEN

Atomically engineered artificial lattices are a useful tool for simulating complex quantum phenomena, but have so far been limited to the study of Hamiltonians where electron-electron interactions do not play a role. However, it is precisely the regime in which these interactions do matter where computational times lend simulations a critical advantage over numerical methods. Here, we propose a platform for constructing artificial matter that relies on the confinement of field-emission resonances, a class of vacuum-localized discretized electronic states. We use atom manipulation of surface vacancies in a chlorine-terminated Cu(100) surface to reveal square patches of the underlying metal, thereby creating atomically precise potential wells that host particle-in-a-box modes. By adjusting the dimensions of the confining potential, we can access states with different quantum numbers, making these patches attractive candidates as quantum dots or artificial atoms. We demonstrate that the lifetime of electrons in these engineered states can be extended and tuned through modification of the confining potential, either via atomic assembly or by changing the tip-sample distance. We also demonstrate control over a finite range of state filling, a parameter which plays a key role in the evolution of quantum many-body states. We model the transport through the localized state to disentangle and quantify the lifetime-limiting processes, illustrating the critical dependence of the electron lifetime on the properties of the underlying bulk band structure. The interplay with the bulk bands gives rise to negative differential resistance, leading to possible applications in engineering custom atomic-scale resonant tunnelling diodes, which exhibit similar current-voltage characteristics.

8.
Sci Adv ; 6(46)2020 Nov.
Artículo en Inglés | MEDLINE | ID: mdl-33177096

RESUMEN

Spin waves-the elementary excitations of magnetic materials-are prime candidate signal carriers for low-dissipation information processing. Being able to image coherent spin-wave transport is crucial for developing interference-based spin-wave devices. We introduce magnetic resonance imaging of the microwave magnetic stray fields that are generated by spin waves as a new approach for imaging coherent spin-wave transport. We realize this approach using a dense layer of electronic sensor spins in a diamond chip, which combines the ability to detect small magnetic fields with a sensitivity to their polarization. Focusing on a thin-film magnetic insulator, we quantify spin-wave amplitudes, visualize spin-wave dispersion and interference, and demonstrate time-domain measurements of spin-wave packets. We theoretically explain the observed anisotropic spin-wave patterns in terms of chiral spin-wave excitation and stray-field coupling to the sensor spins. Our results pave the way for probing spin waves in atomically thin magnets, even when embedded between opaque materials.

9.
Nat Commun ; 11(1): 2698, 2020 Jun 01.
Artículo en Inglés | MEDLINE | ID: mdl-32483113

RESUMEN

The reduced dimensionality of two-dimensional (2D) materials results in characteristic types of magnetically and electronically ordered phases. However, only few methods are available to study this order, in particular in ultrathin insulating antiferromagnets that couple weakly to magnetic and electronic probes. Here, we demonstrate that phase transitions in thin membranes of 2D antiferromagnetic FePS3, MnPS3 and NiPS3 can be probed mechanically via the temperature-dependent resonance frequency and quality factor. The observed relation between mechanical motion and antiferromagnetic order is shown to be mediated by the specific heat and reveals a strong dependence of the Néel temperature of FePS3 on electrostatically induced strain. The methodology is not restricted to magnetic order, as we demonstrate by probing an electronic charge-density-wave phase in 2H-TaS2. It thus offers the potential to characterize phase transitions in a wide variety of materials, including those that are antiferromagnetic, insulating or so thin that conventional bulk characterization methods become unsuitable.

10.
Phys Rev Lett ; 124(10): 107202, 2020 Mar 13.
Artículo en Inglés | MEDLINE | ID: mdl-32216419

RESUMEN

We report strong chiral coupling between magnons and photons in microwave waveguides that contain chains of small magnets on special lines. Large magnon accumulations at one edge of the chain emerge when exciting the magnets by a phased antenna array. This mechanism holds the promise of new functionalities in nonlinear and quantum magnonics.

11.
Nanotechnology ; 30(33): 335702, 2019 Aug 16.
Artículo en Inglés | MEDLINE | ID: mdl-31022709

RESUMEN

We report on the fabrication and performance of a new kind of tip for scanning tunneling microscopy. By fully incorporating a metallic tip on a silicon chip using modern micromachining and nanofabrication techniques, we realize so-called smart tips and show the possibility of device-based STM tips. Contrary to conventional etched metal wire tips, these can be integrated into lithographically defined electrical circuits. We describe a new fabrication method to create a defined apex on a silicon chip and experimentally demonstrate the high performance of the smart tips, both in stability and resolution. In situ tip preparation methods are possible and we verify that they can resolve the herringbone reconstruction and Friedel oscillations on Au(111) surfaces. We further present an overview of possible applications.

12.
Phys Rev Lett ; 123(24): 247202, 2019 Dec 13.
Artículo en Inglés | MEDLINE | ID: mdl-31922821

RESUMEN

We report a theory for the coherent and incoherent chiral pumping of spin waves into thin magnetic films through the dipolar coupling with a local magnetic transducer, such as a nanowire. The ferromagnetic resonance of the nanowire is broadened by the injection of unidirectional spin waves that generates a nonequilibrium magnetization in only half of the film. A temperature gradient between the local magnet and film leads to a unidirectional flow of incoherent magnons, i.e., a chiral spin Seebeck effect.

13.
Phys Rev Lett ; 121(8): 087205, 2018 Aug 24.
Artículo en Inglés | MEDLINE | ID: mdl-30192616

RESUMEN

Inelastic scattering of light by spin waves generates an energy flow between the light and magnetization fields, a process that can be enhanced and controlled by concentrating the light in magneto-optical resonators. Here, we model the cooling of a sphere made of a magnetic insulator, such as yttrium iron garnet, using a monochromatic laser source. When the magnon lifetimes are much larger than the optical ones, we can treat the latter as a Markovian bath for magnons. The steady-state magnons are canonically distributed with a temperature that is controlled by the light intensity. We predict that such a cooling process can significantly reduce the temperature of the magnetic order within current technology.

14.
Nat Commun ; 6: 8491, 2015 Oct 09.
Artículo en Inglés | MEDLINE | ID: mdl-26450772

RESUMEN

In cavity optomechanics, light is used to control mechanical motion. A central goal of the field is achieving single-photon strong coupling, which would enable the creation of quantum superposition states of motion. Reaching this limit requires significant improvements in optomechanical coupling and cavity coherence. Here we introduce an optomechanical architecture consisting of a silicon nitride membrane coupled to a three-dimensional superconducting microwave cavity. Exploiting their large quality factors, we achieve an optomechanical cooperativity of 146,000 and perform sideband cooling of the kilohertz-frequency membrane motion to 34±5 µK, the lowest mechanical mode temperature reported to date. The achieved cooling is limited only by classical noise of the signal generator, and should extend deep into the ground state with superconducting filters. Our results suggest that this realization of optomechanics has the potential to reach the regimes of ultra-large cooperativity and single-photon strong coupling, opening up a new generation of experiments.

15.
Phys Rev Lett ; 100(5): 056801, 2008 Feb 08.
Artículo en Inglés | MEDLINE | ID: mdl-18352406

RESUMEN

We propose a protocol for a controlled experiment to measure a weak value of the electron's spin in a solid state device. The weak value is obtained by a two step procedure--weak measurement followed by a strong one (postselection), where the outcome of the first measurement is kept provided a second postselected outcome occurs. The setup consists of a double quantum dot and a weakly coupled quantum point contact to be used as a detector. Anomalously large values of the spin of a two electron system are predicted, as well as negative values of the total spin. We also show how to incorporate the adverse effect of decoherence into this procedure.

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