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1.
ACS Sustain Chem Eng ; 12(22): 8307-8312, 2024 Jun 03.
Artículo en Inglés | MEDLINE | ID: mdl-38845759

RESUMEN

The circular economy could transform how industry and society approach resources and waste, resulting in significant environmental justice (EJ) implications. However, there are few resources for analyzing the EJ impacts of new circular economy technologies before they are deployed. This work presents an EJ framework tailored for early stage circular economy technologies and showcases its capabilities through a case study on enzymatic plastic recycling. By providing concise, actionable, and accessible guidelines based on technology readiness levels and a series of 20 questions, the framework empowers both experts and nonexperts to evaluate the justice implications of circular economy solutions. Preliminary user feedback highlights the approachability of the framework and its corresponding interactive worksheet, as well as their potential to stimulate innovative thinking toward a more just and sustainable future.

2.
iScience ; 25(8): 104734, 2022 Aug 19.
Artículo en Inglés | MEDLINE | ID: mdl-35874102

RESUMEN

The growing number of end-of-life (EOL) wind blades could further strain US landfills or be a valuable composite materials source, depending on stakeholders' behaviors. Technical solutions based on circular economy (CE) principles have been proposed but are not guaranteed to solve the issue of EOL management. Transitioning to CE implies changing how business models, supply chains, and behaviors deal with products and waste. A spatially resolved agent-based modeling combined with a machine-learning metamodel shows that including behavioral factors is crucial to designing effective policies. Logistical barriers and transportation costs significantly affect the results: lowering blade shredding costs by a third before transportation makes EOL blades a source of valuable materials, decreasing the 2050 cumulative landfill rate below 50%. In another scenario, parameter settings simulating policy interventions aiming at boosting early adoption incites new social norms favorable to recycling, lowering the cumulative landfill rate below 10%.

3.
Annu Rev Chem Biomol Eng ; 13: 301-324, 2022 06 10.
Artículo en Inglés | MEDLINE | ID: mdl-35320697

RESUMEN

There is an urgent need for new technologies to enable circularity for synthetic polymers, spurred by the accumulation of waste plastics in landfills and the environment and the contributions of plastics manufacturing to climate change. Chemical recycling is a promising means to convert waste plastics into molecular intermediates that can be remanufactured into new products. Given the growing interest in the development of new chemical recycling approaches, it is critical to evaluate the economics, energy use, greenhouse gas emissions, and other life cycle inventory metrics for emerging processes,relative to the incumbent, linear manufacturing practices employed today. Here we offer specific definitions for classes of chemical recycling and upcycling and describe general process concepts for the chemical recycling of mixed plastics waste. We present a framework for techno-economic analysis and life cycle assessment for both closed- and open-loop chemical recycling. Rigorous application of these process analysis tools will be required to enable impactful solutions for the plastics waste problem.


Asunto(s)
Plásticos , Reciclaje , Plásticos/química , Polímeros
4.
Int J Life Cycle Assess ; 28: 156-171, 2022 Dec 19.
Artículo en Inglés | MEDLINE | ID: mdl-36891065

RESUMEN

Purpose: Electricity production is one of the largest sources of environmental emissions-especially greenhouse gases (GHGs)-in the USA. Emission factors (EFs) vary from region to region, which requires the use of spatially relevant EF data for electricity production while performing life cycle assessments (LCAs). Uncertainty information, which is sought by LCA practitioners, is rarely supplied with available life cycle inventories (LCIs). Methods: To address these challenges, we present a method for collecting data from different sources for electricity generation and environmental emissions; discuss the challenges involved in agglomerating such data; provide relevant suggestions and solutions to merge the information; and calculate EFs for electricity generation processes from various fuel sources for different spatial regions and spatial resolutions. The EFs from the US 2016 Electricity Life Cycle Inventory (eLCI) are analyzed and explored in this study. We also explore the method of uncertainty information derivation for the EFs. Results and discussion: We explore the EFs from different technologies across Emissions & Generation Resource Integrated Database (eGRID) regions in the USA. We find that for certain eGRID regions, the same electricity production technology may have worse emissions. This may be a result of the age of the plants in the region, the quality of fuel used, or other underlying factors. Region-wise life cycle impact assessment (LCIA) ISO 14040 impacts for total generation mix activities provide an overview of the total sustainability profile of electricity production in a particular region, rather than only global warming potential (GWP). We also find that, for different LCIA impacts, several eGRID regions are consistently worse than the US average LCIA impact for every unit of electricity generated. Conclusion: This work describes the development of an electricity production LCI at different spatial resolutions by combining and harmonizing information from several databases. The inventory consists of emissions, fuel inputs, and electricity and steam outputs from different electricity production technologies located across various regions of the USA. This LCI for electricity production in the USA will prove to be an enormous resource for all LCA researchers-considering the detailed sources of the information and the breadth of emissions covered by it.

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