RESUMEN
Ultraviolet spectroscopy provides unique insights into the structure of matter with applications ranging from fundamental tests to photochemistry in the Earth's atmosphere and astronomical observations from space telescopes1-8. At longer wavelengths, dual-comb spectroscopy, using two interfering laser frequency combs, has become a powerful technique capable of simultaneously providing a broad spectral range and very high resolution9. Here we demonstrate a photon-counting approach that can extend the unique advantages of this method into ultraviolet regions where nonlinear frequency conversion tends to be very inefficient. Our spectrometer, based on two frequency combs with slightly different repetition frequencies, provides a wide-span, high-resolution frequency calibration within the accuracy of an atomic clock, and overall consistency of the spectra. We demonstrate a signal-to-noise ratio at the quantum limit and an optimal use of the measurement time, provided by the multiplexed recording of all spectral data on a single photon-counter10. Our initial experiments are performed in the near-ultraviolet and in the visible spectral ranges with alkali-atom vapour, with a power per comb line as low as a femtowatt. This crucial step towards precision broadband spectroscopy at short wavelengths paves the way for extreme-ultraviolet dual-comb spectroscopy, and, more generally, opens up a new realm of applications for photon-level diagnostics, as encountered, for example, when driving single atoms or molecules.
RESUMEN
Analog quantum simulations with Rydberg atoms in optical tweezers routinely address strongly correlated many-body problems due to the hardware-efficient implementation of the Hamiltonian. Yet, their generality is limited, and flexible Hamiltonian-design techniques are needed to widen the scope of these simulators. Here we report on the realization of spatially tunable interactions for XYZ models implemented by two-color near-resonant coupling to Rydberg pair states. Our results demonstrate the unique opportunities of Rydberg dressing for Hamiltonian design in analog quantum simulators.
RESUMEN
Advanced machine learning models are currently impossible to run on edge devices such as smart sensors and unmanned aerial vehicles owing to constraints on power, processing, and memory. We introduce an approach to machine learning inference based on delocalized analog processing across networks. In this approach, named Netcast, cloud-based "smart transceivers" stream weight data to edge devices, enabling ultraefficient photonic inference. We demonstrate image recognition at ultralow optical energy of 40 attojoules per multiply (<1 photon per multiply) at 98.8% (93%) classification accuracy. We reproduce this performance in a Boston-area field trial over 86 kilometers of deployed optical fiber, wavelength multiplexed over 3 terahertz of optical bandwidth. Netcast allows milliwatt-class edge devices with minimal memory and processing to compute at teraFLOPS rates reserved for high-power (>100 watts) cloud computers.
RESUMEN
Dual-comb spectroscopy (DCS) normally operates with two independent, relatively low power and actively synchronized laser sources. This hinders the wide adoption for practical implementations and frequency conversion into deep UV and VUV spectral ranges. Here, we report a fully passive, high power dual-comb laser based on thin-disk technology and its application to direct frequency comb spectroscopy. The peak power (1.2 MW) and the average power (15 W) of our Yb:YAG thin-disk dual-comb system are more than one-order-of-magnitude higher than in any previous systems. The scheme allows easy adjustment of the repetition frequency difference during operation. Both combs share all cavity components which leads to an excellent mutual stability. A time-domain signal recorded over 10 ms without any active stabilization was sufficient to resolve individual comb lines after Fourier transformation.
RESUMEN
Time-resolved near-infrared absorption spectroscopy of single non-repeatable transient events is performed at high spectral resolution with a dual-comb interferometer using a continuous-wave laser followed by a single electro-optic amplitude modulator. By sharing high-speed electrical/optical components, our spectrometer greatly simplifies the implementation of dual-comb spectroscopy and offers a high mutual coherence time, measured up to 50 s, without any active stabilization system and/or data processing. The time resolution is as short as 100 µs in our experimental demonstration. For a span of 36 GHz, the mean signal-to-noise ratio of 80, at 100-MHz spectral resolution and 100-µs measurement time, enables precise determination of the parameters of rovibrational lines, including intensity or concentration.
RESUMEN
A novel strategy for large-scale synthesis of ZnO nanowire film is reported, which inherits the advantages of the solution-phase method and seeded growth process, such as low-temperature, efficient, economical, facile and flexible. It is easy to implement on various metals through room-temperature electrodeposition, followed by hydrothermal treatment at 90 °C, and suitable for industrialized production. The ZnO nanowires with an average wire diameter about 40 nm are in situ grown from and on nanocrystalline zinc coating, which forms a strong metallurgical bonding with the substrates. The p-type ZnO nanowire film has a well-preferred orientation along the (100) direction and a wurtzite structure, thereby displaying an effective photocatalytic capability for carcinogenic Cr6+ ions and CO2 greenhouse gas reduction under visible light irradiation. In addition to these features, the ZnO nanowire film is easy to recycle and, therefore, it has broad application prospects in contaminant degradation and renewable energy.
RESUMEN
Mid-infrared high-resolution spectroscopy has proven an invaluable tool for the study of the structure and dynamics of molecules in the gas phase. The advent of frequency combs advances the frontiers of precise molecular spectroscopy. Here we demonstrate, in the important 3-µm spectral region of the fundamental CH stretch in molecules, dual-comb spectroscopy with experimental coherence times between the combs that exceed half an hour. Mid-infrared Fourier transform spectroscopy using two frequency combs with self-calibration of the frequency scale, negligible contribution of the instrumental line shape to the spectral profiles, high signal-to-noise ratio, and broad spectral bandwidth opens up opportunities for precision spectroscopy of small molecules. Highly multiplexed metrology of line shapes may be envisioned.
RESUMEN
Dual-comb systems based on two optical frequency combs of slightly different line spacing emerge as powerful tools in spectroscopy and interferometry. Semiconductor lasers have a high impact in continuous-wave tunable laser spectroscopy. Here we demonstrate the first dual-comb interferometer based on a single femtosecond semiconductor laser: a dual-comb modelocked optically pumped external-cavity surface-emitting laser (MIXSEL) ideally suited for a 1 to 10 GHz comb spacing. At a center wavelength of 1.03 µm (9709 cm-1) we measured acetylene gas transmittance with a resolution of 2.7 GHz in 100 ms with residual errors of less than 3% using thousand comb lines without aliasing effects.
RESUMEN
Laser frequency combs emit a spectrum with hundreds of thousands of evenly spaced phase-coherent narrow lines. A comb-enabled instrument, the dual-comb interferometer, exploits interference between two frequency combs and attracts considerable interest in precision spectroscopy and sensing, distance metrology, tomography, telecommunications, etc. Mutual coherence between the two combs over the measurement time is a pre-requisite to interferometry, although it is instrumentally challenging. At best, the mutual coherence reaches about 1 s. Computer-based phase-correction techniques, which often lead to artifacts and worsened precision, must be implemented for longer averaging times. Here with feed-forward relative stabilization of the carrier-envelope offset frequencies, we experimentally realize a mutual coherence over times approaching 2000 s, more than three orders of magnitude longer than that of state-of-the-art dual-comb systems. An illustration is given with near-infrared Fourier transform molecular spectroscopy with two combs of slightly different repetition frequencies. Our technique without phase correction can be implemented with any frequency comb generator including microresonators or semiconductor lasers.
