RESUMEN
SignificanceWeyl semimetals are a class of three-dimensional materials, whose low-energy excitations mimic massless fermions. In consequence they exhibit various unusual transport properties related to the presence of chiral anomalies, a subtle quantum phenomenon that denotes the breaking of the classical chiral symmetry by quantum fluctuations. In this work we present a universal description of transport in weakly disordered Weyl semimetals with several scattering mechanisms taken into account. Our work predicts the existence of a new anomaly-induced transport regime in these materials and gives a crisp experimental signature of a chiral anomaly in optical conductivity measurements. Finally, by also capturing the hydrodynamic regime of quasiparticles, our construction bridges the gap between developments in electronic fluid mechanics and three-dimensional semimetals.
RESUMEN
Harmonic generation is a general characteristic of driven nonlinear systems, and serves as an efficient tool for investigating the fundamental principles that govern the ultrafast nonlinear dynamics. Here, we report on terahertz-field driven high-harmonic generation in the three-dimensional Dirac semimetal Cd3As2 at room temperature. Excited by linearly-polarized multi-cycle terahertz pulses, the third-, fifth-, and seventh-order harmonic generation is very efficient and detected via time-resolved spectroscopic techniques. The observed harmonic radiation is further studied as a function of pump-pulse fluence. Their fluence dependence is found to deviate evidently from the expected power-law dependence in the perturbative regime. The observed highly non-perturbative behavior is reproduced based on our analysis of the intraband kinetics of the terahertz-field driven nonequilibrium state using the Boltzmann transport theory. Our results indicate that the driven nonlinear kinetics of the Dirac electrons plays the central role for the observed highly nonlinear response.
