Intra-oscillator high harmonic source reaching 100-eV photon energy.

Resonant enhancement inside an optical cavity has been a wide-spread approach to increase efficiency of nonlinear optical conversion processes while reducing the demands on the driving laser power. This concept has been particularly important for high harmonic generation XUV sources, where passive femtosecond enhancement cavities allowed significant increase in repetition rates required for applications in photoelectron spectroscopy, XUV frequency comb spectroscopy, including the recent endeavor of thorium nuclear clock development. In addition to passive cavities, it has been shown that comparable driving conditions can be achieved inside mode-locked thin-disk laser oscillators, offering a simplified single-stage alternative. This approach is less sensitive to losses thanks to the presence of gain inside the cavity and should thus allow higher conversion efficiencies through tolerating higher intensity in the gas target. Here, we show that the intra-oscillator approach can indeed surpass the much more mature technology of passive enhancement cavities in terms of XUV flux, even reaching comparable values to single-pass sources based on chirped-pulse fiber amplifier lasers. Our system operates at 17 MHz repetition rate generating photon energies between 60 eV and 100 eV. Importantly, this covers the highly attractive wavelength for the silicon industry of 13.5 nm at which our source delivers 60 nW of outcoupled average power per harmonic order.

Efficient XUV-light out-coupling of intra-cavity high harmonics by a coated grazing-incidence plate.

We experimentally demonstrate an efficient and broadband extreme-ultraviolet light (XUV) out-coupling mechanism of intra-cavity generated high harmonics. The mechanism is based on a coated grazing-incidence plate (GIP), which utilizes the enhanced reflectivity of s-polarized light in comparison to p-polarized light for large angles of incidence (AoI). We design and produce a 60°-AoI coated GIP, tailored specifically for the high demands inside a sub-50-fs Kerr-lens mode-locked Yb:YAG thin-disk laser oscillator in which high harmonic generation (HHG) is driven at ∼450 MW peak power and 17 MHz repetition rate. The coated GIP features an XUV out-coupling efficiency of >25% for photon energies ranging from 10 eV to 60 eV while being anti-reflective for the driving laser field. The XUV spectra reach up to 52 eV in argon and 30 eV in xenon. In a single harmonic, we out-couple 1.3 µW of XUV average power at 37 eV in argon and 5.4 µW at 25 eV in xenon. The combination of an improved HHG driving laser performance and the out-coupling via the coated GIP enabled us to increase the out-coupled XUV average power in a single harmonic by a factor of 20 compared to previous HHG inside ultrafast laser oscillators. Our source approaches the state-of-the-art out-coupled XUV power levels per harmonic of femtosecond enhancement cavities operating at comparable photon energies.

Sub-30-fs Yb:YAG thin-disk laser oscillator operating in the strongly self-phase modulation broadened regime.

We experimentally investigate the limits of pulse duration in a Kerr-lens mode-locked Yb:YAG thin-disk laser (TDL) oscillator. Thanks to its excellent mechanical and optical properties, Yb:YAG is one of the most used gain materials for continuous-wave and pulsed TDLs. In mode-locked operation, its 8-nm wide gain bandwidth only directly supports pulses with a minimum duration of approximately 140 fs. For achieving shorter pulses, a Kerr-lens mode-locked TDL oscillator can be operated in the strongly self-phase modulation (SPM) broadened regime. Here, the spectral bandwidth of the oscillating pulse exceeds the available gain bandwidth by generating additional frequencies via SPM inside the Kerr medium. In this work, we study and compare different laser configurations in the strongly SPM-broadened regime. Starting with a configuration providing 84-fs pulses at 69 W average power at 17 MHz repetition rate, we reduce the pulse duration by optimizing various mode-locking parameters. One crucial parameter is the dispersion control which was provided by in-house-developed dispersive mirrors produced by ion-beam sputtering (IBS). We discuss trade-offs in average power, pulse duration, efficiency, and intra-cavity peak power. For the configuration operating at the highest SPM-broadening, we achieve a minimum pulse duration of 27 fs, which represents the shortest pulse duration directly generated by any ultrafast TDL oscillator. The corresponding full width at half maximum (FWHM) spectral bandwidth exceeds more than five times the FWHM gain bandwidth. The average output power of 3.3 W is moderate for ultrafast TDL oscillators, but higher than other Yb-based laser oscillators operating at this pulse duration. Additionally, the corresponding intra-cavity peak power of 0.8 GW is highly attractive for implementing intra-cavity extreme nonlinear optical interactions such as high harmonic generation.

Intra-oscillator broadband THz generation in a compact ultrafast diode-pumped solid-state laser.

We demonstrate broadband and powerful terahertz (THz) generation at megahertz repetition rate based on intra-oscillator optical rectification (OR) in gallium phosphide (GaP). By placing the nonlinear crystal directly inside the cavity of a Kerr-lens mode-locked ultrafast diode-pumped solid-state laser (DPSSL) oscillator, we demonstrate a compact and single-stage THz source. Using only 7 W of diode-pump power, we drive OR in a GaP crystal with 22 W of average power at ∼80 MHz repetition rate. In a first configuration, using a 0.3-mm-thick GaP and 105 fs driving pulses, we generate up to 150 µW of THz radiation with a spectrum extending to 5.5 THz. In a second configuration allowing for sub-50-fs pulse duration, we generate up to 7 THz inside a 0.1-mm-thick GaP crystal. This performance is well suited for THz time-domain spectroscopy and THz imaging. Intra-oscillator THz generation in sub-100-fs DPSSLs is a promising way to scale down footprint, complexity and cost of powerful broadband THz sources.

High-power dual-comb thin-disk laser oscillator for fast high-resolution spectroscopy.

Free-running dual-comb systems based on a single laser cavity are an attractive next generation technology for a wide variety of applications. The high average power achievable by dual-comb thin-disk laser (TDL) oscillators make this technology especially attractive for spectroscopy and sensing applications in the molecular fingerprint region enabled by nonlinear frequency conversion. However, the high noise levels of TDL oscillators, e.g., induced by the turbulent water-cooling of the disk, are a severe challenge for spectroscopic applications. In this contribution, we confirm for the first time the suitability of dual-comb TDLs for high-resolution spectroscopy. Based on the novel concept of polarization splitting inside a TDL, our oscillator generates two asynchronous pulse trains of 240-fs pulse duration at 6-W and 8-W average power per pulse train and ∼97-MHz repetition rate at a central wavelength of 1030 nm. In the first detailed noise investigation of such a system, we identify the repetition frequency as the dominant noise term and show that ∼85% of the frequency noise of the comb lines of both pulse trains is correlated (integrated from 200 Hz to 20 kHz). We detect the absorption spectrum of acetylene in free-running operation within a measurement time of 1 millisecond. Being highly suitable for nonlinear frequency conversion, we believe the here presented result is an important step towards simple yet powerful mid-infrared dual-comb systems for high-resolution spectroscopy.

Intra-oscillator high harmonic generation in a thin-disk laser operating in the 100-fs regime.

We demonstrate that Kerr lens modelocking is well-suited for operating an ultrafast thin-disk laser with intra-oscillator high harmonic generation (HHG) in the 100-fs pulse duration regime. Exploiting nearly the full emission bandwidth of the gain material Yb:YAG, we generate 105-fs pulses with an intracavity peak power of 365 MW and an intracavity average power of 470 W. We drive HHG in argon with a peak intensity of ∼7⋅1013 W/cm2 at a repetition rate of 11 MHz. Extreme-ultraviolet (XUV) light is generated up to the 31st harmonic order (H31) at 37 eV, with an average power of ∼0.4 µW in H25 at 30 eV. This work presents a considerable increase in performance of XUV sources based on intra-oscillator HHG and confirms that this approach is a promising technology for simple and portable XUV sources at MHz repetition rates.

Sub-100-fs Kerr lens mode-locked Yb:Lu2O3 thin-disk laser oscillator operating at 21 W average power.

We investigate power-scaling of a Kerr lens mode-locked (KLM) Yb:Lu2O3 thin-disk laser (TDL) oscillator operating in the sub-100-fs pulse duration regime. Employing a scheme with higher round-trip gain by increasing the number of passes through the thin-disk gain element, we increase the average power by a factor of two and the optical-to-optical efficiency by a factor of almost three compared to our previous sub-100-fs mode-locking results. The oscillator generates pulses with a duration of 95 fs at 21.1 W average power and 47.9 MHz repetition rate. We discuss the cavity design for continuous-wave and mode-locked operation and the estimation of the focal length of the Kerr lens. Unlike to usual KLM TDL oscillators, an operation at the edge of the stability zone in continuous-wave operation is not required. This work shows that KLM TDL oscillators based on the gain material Yb:Lu2O3 are an excellent choice for power-scaling of laser oscillators in the sub-100-fs regime, and we expect that such lasers will soon operate at power levels in excess of hundred watts.

Broadband terahertz pulse generation driven by an ultrafast thin-disk laser oscillator.

We demonstrate broadband THz generation driven by an ultrafast thin-disk laser (TDL) oscillator. By optical rectification of 50-fs pulses at 61 MHz repetition rate in a collinear geometry in crystalline GaP, THz radiation with a central frequency at around 3.4 THz and a spectrum extending from below 1 THz to nearly 7 THz are generated. We realized a spectroscopic characterization of a GaP crystal and a benchmark measurement of the water-vapor absorption spectrum in the THz range. Sub-50-GHz resolution is achieved within a 5 THz bandwidth. Our experiments show the potential of ultrafast TDL oscillators for driving MHz-repetition-rate broadband THz systems.

Laser-assisted morphing of complex three dimensional objects.

Morphing refers to the smooth transition from a specific shape into another one, in which the initial and final shapes can be significantly different. A typical illustration is to turn a cube into a sphere by continuous change of shape curvatures. Here, we demonstrate a process of laser-induced morphing, driven by surface tension and thermally-controlled viscosity. As a proof-of-concept, we turn 3D glass structures fabricated by a femtosecond laser into other shapes by locally heating up the structure with a feedback-controlled CO2 laser. We further show that this laser morphing process can be accurately modelled and predicted.