Advanced Solid-State Lasers: feature issue introduction.

This joint issue of Optics Express and Optical Materials Express features 23 peer-reviewed articles primarily by authors who participated in the Advanced Solid State Lasers conference, which was part of the Optica Laser Congress held in Tacoma, Washington, USA on October 8-12, 2023. This review provides a brief summary of these articles covering the latest developments in laser gain materials and nonlinear crystals, mode-locked lasers, fiber lasers and amplifiers, nonlinear optical sources, and novel concepts in laser design.

Rapid calculation of the efficiency of self-terminating four-level Q-switched lasers.

We have developed a simple approach to deriving the efficiency of Q-switched four-level lasers, valid even for arbitrarily long lower laser level lifetimes. By eliminating time dependence from the calculation, numerical solutions can be obtained very rapidly. Its threshold and limiting slope efficiency values provide useful estimates for free-running pulsed four-level lasers as well as Q-switched.

Enhanced mid-infrared emission of Pr3+ ions in solids through a "3-for-1" excitation process - quantified.

Evidence is presented that a "three-for-one" process based on two cross-relaxations between Pr3+ ions efficiently populates the mid-infrared-emitting 3H5 manifold in a Pr3+-doped low-maximum-phonon-energy host. The concentration dependence of infrared fluorescence spectra and lifetimes of polycrystalline Pr:KPb2Cl5 initially excited to the 3F3,4 manifolds indicate that the 3500-5500-nm fluorescence becomes strongly favored over shorter-wavelength infrared emission bands in the higher-concentration sample. The strong concentration dependence of the 3F3 and 3H6 manifold lifetimes suggests that both of these decay by cross-relaxation processes, resulting in more than one ion excited to 3H5 for each ion initially excited to 3F3. Indeed, modeling and accounting for all possible decay paths indicate that, on average, about 2.3 ions are excited to 3H5 for each initially-excited ion. This confirms that the three-for-one excitation process must occur and contribute significantly to the total excitation efficiency. These results indicate that the two distinct cross-relaxation processes observed between Pr ions result in substantially higher excitation quantum efficiency, 230%, than any ever reported in rare-earth doped materials.

Cladding-pumped, Yb:YAG-core, fiber-like waveguide laser: modeling and experiment.

We developed a model describing the performance of the cladding-pumped, Yb:YAG-core, fiber-like waveguide laser with a large cladding-to-core area ratio. We analyzed how pump absorption and laser output efficiencies depend on the Yb-doping level as well as the waveguide parameters, such as clad-to-core area ratio and waveguide length. We also determined the conditions that maximize both pump and laser efficiency. We showed that, depending on the waveguide design, cavity parameters as well as the core temperature, this laser can operate either at 1030 or 1050 nm. We have also shown that the main factor limiting power scaling of such a waveguide laser is the core temperature. The model was validated by laser experiments with a 174 mm long, double-clad, Yb(20%):YAG-core waveguide, with the cladding-to-core area ratio of 43.4. An output power of 41.6 W and slope efficiency of 73% with respect to the absorbed pump power have been achieved with cladding pumping by a fiber-coupled laser diode module at 933 nm. Our experimental results were in a good agreement with the modeling predictions.

Pr:RbPb2Cl5: temperature dependent spectra, dynamics and three-for-one excitation: erratum.

We present an erratum regarding the contents of Table 1.

Low-loss 'crystalline-core/crystalline-clad' (C4) fibers for highly power scalable high efficiency fiber lasers.

We report the latest progress in fabrication and laser performance of the fully crystalline double-clad 'Yb:YAG-core/undoped-YAG-clad' fibers grown by the hybrid crystal growth method. The single-crystalline ytterbium (Yb) doped yttrium aluminum garnet (YAG) fiber cores were grown by the laser heated pedestal growth (LHPG) method, and the single-crystalline undoped YAG claddings were grown by the liquid phase epitaxy (LPE) technique, in which the single-crystalline Yb:YAG cores were used as the growth seeds. The key parameters of the hybrid-grown 'crystalline core/crystalline clad' (C4) fibers, including material composition, crystal structure, and fiber propagation loss, were characterized. The results confirmed that the grown C4 fibers, indeed, have both the single-crystalline fiber core and single-crystalline fiber clad. By utilizing a double-clad low-loss C4 fiber as a diode-cladding-pumped laser gain medium, we realized a fiber laser with the optical-to-optical conversion efficiency of 68.7% versus the incident pump power.

Pr:RbPb2Cl5: temperature dependent spectra, dynamics and three-for-one excitation.

The temperature dependence of the absorption, fluorescence, and fluorescence lifetimes of states relevant to short-wave-infrared and mid-infrared laser operation have been measured in Pr:RbPb2Cl5. The 3600-5500-nm fluorescence grows strongly with temperature, and at room temperature represents the large majority of the observed photon flux. Intra-ionic decay processes cannot explain this dominance, but a combination of two cross-relaxation processes provides good agreement with the data. These results indicate a three-for-one process: the excitation of nearly three ions to the 3H5 manifold of Pr3+ by each one initially excited to 3F3, with the potential for exceptionally high efficiency excitation of mid-infrared laser materials.

Nanoparticle doping for high power fiber lasers at eye-safer wavelengths.

A nanoparticle (NP) doping technique was developed for fabricating erbium (Er)- and holmium (Ho)-doped silica-based optical fibers for high energy lasers. Slope efficiencies in excess of 74% were realized for Er NP doping in a single mode fiber based master oscillator power amplifier (MOPA) and 53% with multi-Watt-level output in a resonantly cladding-pumped power oscillator laser configuration based on a double-clad fiber. Cores comprising Ho doped LaF3 and Lu2O3 nanoparticles exhibited slope efficiencies as high as 85% at 2.09 µm in a laser configuration. To the best of the authors' knowledge, this is the first report of a holmium nanoparticle doped fiber laser as well as the highest efficiency and power output reported from an erbium nanoparticle doped fiber laser.

High-efficiency, 154 W CW, diode-pumped Raman fiber laser with brightness enhancement.

We demonstrate a high-power, high-efficiency Raman fiber laser pumped directly by laser diode modules at 978 nm. 154 W of CW power were obtained at a wavelength of 1023 nm with an optical to optical efficiency of 65%. A commercial graded-index (GRIN) core fiber acts as the Raman fiber in a power oscillator configuration, which includes spectral selection to prevent generation of the second Stokes. In addition, brightness enhancement of the pump beam by a factor of 8.4 is attained due to the Raman gain distribution profile in the GRIN fiber. To the best of our knowledge this is the highest power and highest efficiency Raman fiber laser demonstrated in any configuration allowing brightness enhancement (i.e., in either cladding-pumped configuration or with GRIN fibers, excluding step-index core pumped), regardless of pumping scheme (i.e., either diode pumped or fiber laser pumped).

Scalable waveguide design for three-level operation in Neodymium doped fiber laser.

We have constructed a double clad neodymium doped fiber laser operating on the three-level 4F3/2→4I9/2 transition. The laser has produced 11.5 W at 925 nm with 55% slope efficiency when pumped at 808 nm, comparable to the best previous results for a double-clad fiber configuration on this transition. Higher power pumping with both 808 nm and 880 nm sources resulted in an output of 27 W, albeit at lower slope efficiency. In both cases, output power was limited by available pump, indicating the potential for further power scaling. To suppress the stronger four-level 4F3/2→4I11/2 transition we developed a waveguide that provides spectral filtering distributed along the length of the fiber, based on an all-solid micro-structured optical fiber design, with resonant inclusions creating a leakage path to the cladding. The waveguide supports large mode areas and provides strong suppression at selectable wavelength bands, thus easing the restrictions on core and cladding sizes that limited power scaling of previous approaches.

Thermal characterization, crystal field analysis and in-band pumped laser performance of Er doped NaY(WO(4))(2) disordered laser crystals.

Undoped and Er-doped NaY(WO4)2 disordered single crystals have been grown by the Czochralski technique. The specific heat and thermal conductivity (κ) of these crystals have been characterized from T = 4 K to 700 K and 360 K, respectively. It is shown that κ exhibits anisotropy characteristic of single crystals as well as a κ(T) behavior observed in glasses, with a saturation mean free phonon path of 3.6 Å and 4.5 Å for propagation along a and c crystal axes, respectively. The relative energy positions and irreducible representations of Stark Er(3+) levels up to (4)G(7/2) multiplet have been determined by the combination of experimental low (<10 K) temperature optical absorption and photoluminescence measurements and simulations with a single-electron Hamiltonian including both free-ion and crystal field interactions. Absorption, emission and gain cross sections of the (4)I(13/2)↔(4)I(15/2) laser related transition have been determined at 77 K. The (4)I(13/2) Er(3+) lifetime (τ) was measured in the temperature range of 77-300 K, and was found to change from τ (77K) ≈ 4.5 ms to τ (300K) ≈ 3.5 ms. Laser operation is demonstrated at 77 K and 300 K by resonantly pumping the (4)I(13/2) multiplet at λ≈1500 nm with a broadband (FWHM≈20 nm) diode laser source perfectly matching the 77 K crystal (4)I(15/2) → (4)I(13/2) absorption profile. At 77 K as much as 5.5 W of output power were obtained in π-polarized configuration with a slope efficiency versus absorbed pump power of 57%, the free running laser wavelength in air was λ≈1611 nm with the laser output bandwidth of 3.5 nm. The laser emission was tunable over 30.7 nm, from 1590.7 nm to 1621.4 nm, for the same π-polarized configuration.

Resonantly diode-pumped Ho3+:Y2O3 ceramic 2.1 µm laser.

We report what is believed to be the first laser operation based on Ho3+-doped Y2O3. The Ho3+:Y2O3 ceramic was resonantly diode-pumped at ~1.93 µm to produce up to 2.5 W of continuous wave (CW) output power at ~2.12 µm. The laser had a slope efficiency of ~35% with respect to absorbed power and a beam propagation factor of M2 ~1.1. We have measured the absorption and stimulated emission cross sections of Ho3+:Y2O3 at 77 K and 300 K and present the calculated gain cross section spectrum at 77 K for different excited state inversion levels.

Resonantly cladding-pumped Yb-free Er-doped LMA fiber laser with record high power and efficiency.

We report the results of our power scaling experiments with resonantly cladding-pumped Er-doped eye-safe large mode area (LMA) fiber laser. While using commercial off-the-shelf LMA fiber we achieved over 88 W of continuous-wave (CW) single transverse mode power at ~1590 nm while pumping at 1532.5 nm. Maximum observed optical-to-optical efficiency was 69%. This result presents, to the best of our knowledge, the highest power reported from resonantly-pumped Yb-free Er-doped LMA fiber laser, as well as the highest efficiency ever reported for any cladding-pumped Er-doped laser, either Yb-co-doped or Yb-free.

Principal modes in fiber amplifiers.

The dynamics of the state of polarization in multimode fiber amplifiers is presented. The experimental results reveal that although the state of polarizations at the output can vary over a large range when changing the temperatures of the fiber amplifiers, the variations are significantly reduced when resorting to the principal states of polarization in single-mode fiber amplifiers and principal modes in multimode fiber amplifiers.

Fiber amplification of radially and azimuthally polarized laser light.

The results of amplifying either radially or azimuthally polarized light with a fiber amplifier are presented. Experimental results reveal that more than 85% polarization purity can be retained at the output even with 40 dB amplification and that efficient conversion of the amplified light to linear polarization can be obtained.

Temperature dependence of a diode-pumped cryogenic Er:YAG laser.

We report the laser performance of resonantly diode-pumped Er:YAG from liquid nitrogen temperature to above room temperature. Relative to incident pump power, the best performance was observed at approximately 160 K. Spectroscopy and modeling show that this is due primarily to the changing efficiency of diode pump absorption as the absorption lines broaden with temperature. However, the physics of the Er:YAG system indicates that even with arbitrarily narrow pump linewidth the most efficient laser performance should occur at a temperature somewhat above 77 K. The causes of the temperature dependence are at least qualitatively understood.

Ultralow quantum-defect eye-safe Er:Sc2O3 laser.

Resonantly pumped Er(3+):Sc(2)O(3) laser operation is achieved with a quantum defect (QD) of 1.5% at liquid nitrogen temperature. The laser, in-line pumped at 1535 nm, operated at 1558 nm with a slope efficiency of over 45%. This is believed to be the lowest QD eye-safe laser ever reported. CW output of over 3.3 W was obtained in this first experiment.

Concentration quenching in fine-grained ceramic Nd:YAG.

We have studied the concentration dependent fluorescence decay kinetics of ceramic Nd:YAG, to resolve inconsistencies in the previous literature. Our data indicate that earlier reports of single exponential lifetimes even at Nd concentrations of a few percent were due to the effects of long-pulse excitation. Under short-pulse excitation the fluorescence decay is nonexponential for concentrations greater than about 1% atomic. Energy migration to sinks consisting of cross-relaxing Nd ions dominates at long times, whereas single-step energy transfer to randomly distributed quenching sites dominates at earlier times. The concentration dependence of this single-step transfer indicates direct cross-relaxation between individual ions at concentrations below 4% atomic, but resonant transfer to quenching sites consisting of Nd pairs at higher concentrations.

Ultrahigh-gain bulk solid-state stimulated Brillouin scattering phase-conjugation material.

We report what is believed to be the first observation of phase conjugation by stimulated Brillouin scattering (SBS) in TeO2 single crystal. The observed very low threshold for phase-conjugate mirror (PCM) formation, high PCM reflectivities in this initial experiment, and commercial availability of material hold promise for a host of practical applications in the near future. The resultant steady-state gain parameter, approximately 100 cm/GW, is to our knowledge the largest ever reported for any SBS material.