Engineering third-order optical nonlinearities in hybrid chalcogenide-on-silicon platform.

We demonstrated a class of highly nonlinear hybrid waveguide structures based on infiltration of As2S3 chalcogenide glass into silicon slot waveguides. The nonlinear properties of the hybrid waveguides were precisely quantified via a bidirectional top-hat D-scan method, enabling a direct comparison between properties measured using different device geometries. We experimentally demonstrate hybrid As2S3-Si slot waveguides with a two-photon absorption (TPA) figure of merit exceeding 2 at near infrared wavelengths. These waveguides largely satisfy the critical criterion for efficient nonlinear integrated photonics (FOMTPAwg>1), allowing phase shifts greater than π with minimal overall losses. These results pave the way for efficient and robust ultrafast all-optical devices and circuits in large-scale silicon photonics technology.

Nonlinear Properties of Ge-rich Si1-xGex Materials with Different Ge Concentrations.

Silicon photonics is a large volume and large scale integration platform for applications from long-haul optical telecommunications to intra-chip interconnects. Extension to the mid-IR wavelength range is now largely investigated, mainly driven by absorption spectroscopy applications. Germanium (Ge) is particularly compelling as it has a broad transparency window up to 15 µm and a much higher third-order nonlinear coefficient than silicon which is very promising for the demonstration of efficient non-linear optics based active devices. Si1-xGex alloys have been recently studied due to their ability to fine-tune the bandgap and refractive index. The material nonlinearities are very sensitive to any modification of the energy bands, so Si1-xGex alloys are particularly interesting for nonlinear device engineering. We report on the first third order nonlinear experimental characterization of Ge-rich Si1-xGex waveguides, with Ge concentrations x ranging from 0.7 to 0.9. The characterization performed at 1580 nm is compared with theoretical models and a discussion about the prediction of the nonlinear properties in the mid-IR is introduced. These results will provide helpful insights to assist the design of nonlinear integrated optical based devices in both the near- and mid-IR wavelength ranges.

Bi-directional top-hat D-Scan: single beam accurate characterization of nonlinear waveguides.

The characterization of a third-order nonlinear integrated waveguide is reported for the first time by means of a top-hat dispersive-scan (D-Scan) technique, a temporal analog of the top-hat Z-Scan. With a single laser beam, and by carrying two counterdirectional nonlinear transmissions to assess the input and output coupling efficiencies, a novel procedure is described leading to accurate measurement of the TPA figure of merit, the effective two-photon absorption (TPA), and optical Kerr (including the sign) coefficients. The technique is validated in a silicon strip waveguide for which the effective nonlinear coefficients are measured with an accuracy of ±10%.

Enhanced nonlinear interaction in a microcavity under coherent excitation.

The large field enhancement that can be achieved in high quality factor and small mode volume photonic crystal microcavities leads to strengthened nonlinear interactions. However, the frequency shift dynamics of the cavity resonance under a pulsed excitation, which is driven by nonlinear refractive index change, tends to limit the coupling efficiency between the pulse and the cavity. As a consequence, the cavity enhancement effect cannot last for the entire pulse duration, limiting the interaction between the pulse and the intra-cavity material. In order to preserve the benefit of light localization throughout the pulsed excitation, we report the first experimental demonstration of coherent excitation of a nonlinear microcavity, leading to an enhanced intra-cavity nonlinear interaction. We investigate the nonlinear behavior of a Silicon-based microcavity subject to tailored positively chirped pulses, enabling to increase the free carrier density generated by two-photon absorption by up to a factor of 2.5 compared with a Fourier-transform limited pulse excitation of equal energy. It is accompanied by an extended frequency blue-shift of the cavity resonance reaching 19 times the linear cavity bandwidth. This experimental result highlights the interest in using coherent excitation to control intra-cavity light-matter interactions and nonlinear dynamics of microcavity-based optical devices.

Nonlinear optimization of slot Si waveguides: TPA minimization with FOM(TPA) up to 4.25.

The χ(3) nonlinear properties of slotted crystalline silicon photonic waveguides filled with third-order nonlinear materials (NM) are studied by calculating the effective nonlinear susceptibilities associated to the silicon and cladding material, respectively. The adopted approach circumvents the assumptions that the introduced NM dominates the nonlinear behavior of the slotted waveguide and that strong light confinement in the slot allows neglecting the two-photon absorption (TPA) process in the silicon rails. Optimization of the geometry of silicon-slotted waveguides is performed on the basis of the nonlinear figure of merit (FOM(TPA)) of the guided mode, which is related to the balance between the Kerr and the TPA effects, allowing to reach a FOM(TPA)=4.25. The obtained results reveal the importance of properly choosing the waveguide width of the silicon rails in order to minimize the TPA effect even by tolerating a reduced overall nonlinearity.

Second order coherence of broadband down-converted light on ultrashort time scale determined by two photon absorption in semiconductor.

We study the photon correlation properties of broadband parametric down-converted light. The measurement of the photon correlation is carried out thanks to a modified Hanbury Brown-Twiss interferometer based on two photon absorption in GaAs detector. Since this method is not affected by the phase matching conditions of the detecting apparatus (so called "final state post-selection"), the detection bandwidth can be extremely large. This is illustrated by studying, with the same apparatus, the degree of second order coherence of parametric light in both degenerate and non-degenerate cases. We show that our experiment is able to determine the coherent as well as the incoherent contributions to the degree of second order coherence of parametric light with a time resolution in the fs range scale.

Light localization induced enhancement of third order nonlinearities in a GaAs photonic crystal waveguide.

Nonlinear propagation experiments in GaAs photonic crystal waveguides (PCW) were performed, which exhibit a large enhancement of third order nonlinearities, due to light propagation in a slow mode regime, such as two-photon absorption (TPA), optical Kerr effect and refractive index changes due to free-carriers generated by TPA. A theoretical model has been established that shows a very good quantitative agreement with experimental data and demonstrates the important role that the group velocity plays. These observations give a strong insight into the use of PCWs for optical switching devices.

Self-induced transverse mode selection in a photorefractive extended cavity laser diode.

Previous works on photorefractive self-organizing laser cavities were about lasers that oscillate, prior the self-organization process occurs, on a set of axial modes sharing the same transverse structure. In a well-designed broad-area laser diode extended cavity, we theoretically and experimentally demonstrate that the insertion of a photorefractive crystal can also affect the transverse modal structure to force the laser, initially oscillating on several transverse modes, to oscillate on a single transverse and axial mode. This spatial self-organization process leads to an enhancement of the single mode operating range of the laser.

Evaluation of the ordering of membranes in multilayer stacks built on an ATR-FTIR germanium crystal with atomic force microscopy: the case of the H(+),K(+)-ATPase-containing gastric tubulovesicle membranes.

Polarized attenuated total reflection Fourier transform infrared spectra were recorded on multilayer stacks of native gastric tubulovesicle membranes. The spectral intensity and linear dichroism were measured for average thicknesses ranging between 0 and 100 bilayers. Atomic force microscopy was used to investigate the orientation of the membranes at the top of the stack. Height profiles were obtained along randomly drawn lines and slopes were computed over various distances. Orientation distribution functions were obtained from the slopes and decomposed into Legendre polynomials. It was found that the second Legendre polynomials coefficient characterizing the membrane orientation was always larger than 0.9. It could therefore be concluded that the membrane tilt does not significantly contribute to the infrared dichroism, even for the largest thicknesses tested.