High repetition rate plasma mirror device for attosecond science.

This report describes an active solid target positioning device for driving plasma mirrors with high repetition rate ultra-high intensity lasers. The position of the solid target surface with respect to the laser focus is optically monitored and mechanically controlled on the nm scale to ensure reproducible interaction conditions for each shot at arbitrary repetition rate. We demonstrate the target capabilities by driving high-order harmonic generation from plasma mirrors produced on glass targets with a near-relativistic intensity few-cycle pulse laser system operating at 1 kHz. During experiments, residual target surface motion can be actively stabilized down to 47 nm (root mean square), which ensures sub-300-as relative temporal stability of the plasma mirror as a secondary source of coherent attosecond extreme ultraviolet radiation in pump-probe experiments.

Electron vacuum acceleration in a regime beyond Brunel absorption.

We describe a new regime of electron acceleration in laser plasmas driven by ultrafast pulses of relativistic intensity, in which space-charge separation leads to strongly enhanced laser absorption and the production of 20 MeV (p/m0c approximately = 40) electrons driven outward in vacuum. 1D PIC simulations show that intense attosecond pulses generated around critical density can sweep electrons outward over many wavelengths in distance. With increasing interaction scale length, absorption generalizes from the Brunel regime to one in which absorption is primarily into electrons of energy >>5 MeV.

Phase properties of laser high-order harmonics generated on plasma mirrors.

As a high-intensity laser-pulse reflects on a plasma mirror, high-order harmonics of the incident frequency can be generated in the reflected beam. We present a numerical study of the phase properties of these individual harmonics, and demonstrate experimentally that they can be coherently controlled through the phase of the driving laser field. The harmonic intrinsic phase, resulting from the generation process, is directly related to the coherent sub-laser-cycle dynamics of plasma electrons, and thus constitutes a new experimental probe of these dynamics.

Proton acceleration with high-intensity ultrahigh-contrast laser pulses.

We report on simultaneous measurements of backward- and forward-accelerated protons spectra when an ultrahigh intensity (approximately 5 x 10(18) W/cm(20), ultrahigh contrast (>10(10)) laser pulse interacts with foils of thickness ranging from 0.08 to 105 microm. Under such conditions, free of preplasma originating from ionization of the laser-irradiated surface, we show that the maximum proton energies are proportional to the p component of the laser electric field only and not to the ponderomotive force and that the characteristics of the proton beams originating from both target sides are almost identical. All these points have been corroborated by extensive 1D and 2D particle-in-cell simulations showing a very good agreement with the experimental data.

High dynamic range streak camera for subpicosecond time-resolved x-ray spectroscopy.

The full characterization of a time resolved x-ray spectrometer is presented. It is based on the coupling of a conical crystal with a subpicosecond x-ray streak camera. The detector is designed to operate in accumulation mode at high repetition rate (up to 1 kHz) allowing signal to noise ratio as high as 10(4):1. Optical switches have been used to limit the jitter induced in the subpicosecond range, demonstrating the very long term stability (a few hours) of the entire device. The data analysis have been developed to get the spectral and temporal resolution of an ultrashort laser-plasma-based x-ray source.

Relativistic AC gyromagnetic effects in ultraintense laser-matter interaction.

We demonstrate that in ultraintense ultrafast laser-matter interaction, the interplay of laser-induced oscillating space-charge fields with laser E and B fields can strongly affect whether the interaction is relativistic or not: stronger laser fields may not in fact produce more relativistic plasma interactions. We show that there exists a regime of interaction, in the relation of laser intensity and incident angle, for which the Brunel effect of electron acceleration is strongly suppressed by AC gyromagnetic fields, at a frequency different from the laser field. Analytically and with 1.5D particle-in-cell modeling, we show that from gyromagnetic effects, even in the absence of usual J x B second-harmonic contributions, there are strong effects on the harmonic emission and on the generation of attosecond pulses.

Coherent wake emission of high-order harmonics from overdense plasmas.

We present a new mechanism for high-order harmonic generation by reflection of a laser beam from an overdense plasma, efficient even at moderate laser intensities (down to Igamma2 approximately 4x10(15) W cm-2 microm2). In this mechanism, a transient phase matching between the electromagnetic field and plasma oscillations within a density gradient leads to the emission of harmonics up to the plasma frequency. These plasma oscillations are periodically excited in the wake of attosecond electron bunches which sweep across the density gradient. This process leads to a train of unevenly spaced chirped attosecond pulses and, hence, to broadened and chirped harmonics. This last effect is confirmed experimentally.

Picosecond time-resolved X-ray absorption spectroscopy of ultrafast aluminum plasmas.

We have used point-projection K-shell absorption spectroscopy to infer the ionization and recombination dynamics of transient aluminum plasmas. Two femtosecond beams of the 100 TW laser at the LULI facility were used to produce an aluminum plasma on a thin aluminum foil (83 or 50 nm), and a picosecond x-ray backlighter source. The short-pulse backlighter probed the aluminum plasma at different times by adjusting the delay between the two femtosecond driving beams. Absorption x-ray spectra at early times are characteristic of a dense and rather homogeneous plasma. Collisional-radiative atomic physics coupled with hydrodynamic simulations reproduce fairly well the measured average ionization as a function of time.

Complete characterization of a plasma mirror for the production of high-contrast ultraintense laser pulses.

Improving the temporal contrast of ultrashort and ultraintense laser pulses is a major technical issue for high-field experiments. This can be achieved using a so-called "plasma mirror." We present a detailed experimental and theoretical study of the plasma mirror that allows us to quantitatively assess the performances of this system. Our experimental results include time-resolved measurements of the plasma mirror reflectivity, and of the phase distortions it induces on the reflected beam. Using an antireflection coated plate as a target, an improvement of the contrast ratio by more than two orders of magnitude can be achieved with a single plasma mirror. We demonstrate that this system is very robust against changes in the pulse fluence and imperfections of the beam spatial profile, which is essential for applications.

Direct observation of the ponderomotive force effects in short-scale-length laser plasmas by frequency-domain interferometry.

We report on single-shot frequency-domain interferometric measurements showing space- and time-resolved ponderomotive electron density profile steepening of a short-scale-length ultraintense laser-produced plasma. The density gradient scale length is varied by applying a time-delayed laser prepulse. The measured absolute position of the critical density surface is found to be in agreement with one-dimensional hydrodynamic simulations for the range of scale lengths studied.

Non-thermal melting in semiconductors measured at femtosecond resolution.

Ultrafast time-resolved optical spectroscopy has revealed new classes of physical, chemical and biological reactions, in which directed, deterministic motions of atoms have a key role. This contrasts with the random, diffusive motion of atoms across activation barriers that typically determines kinetic rates on slower timescales. An example of these new processes is the ultrafast melting of semiconductors, which is believed to arise from a strong modification of the inter-atomic forces owing to laser-induced promotion of a large fraction (10% or more) of the valence electrons to the conduction band. The atoms immediately begin to move and rapidly gain sufficient kinetic energy to induce melting--much faster than the several picoseconds required to convert the electronic energy into thermal motions. Here we present measurements of the characteristic melting time of InSb with a recently developed technique of ultrafast time-resolved X-ray diffraction that, in contrast to optical spectroscopy, provides a direct probe of the changing atomic structure. The data establish unambiguously a loss of long-range order up to 900 A inside the crystal, with time constants as short as 350 femtoseconds. This ability to obtain the quantitative structural characterization of non-thermal processes should find widespread application in the study of ultrafast dynamics in other physical, chemical and biological systems.

Single-shot spectral interferometry with chirped pulses.

We present a method for obtaining time-resolved measurements of the amplitude modulation and the phase shift of a chirped probe pulse interacting with a femtosecond-laser-produced plasma. Based on spectral interferometry, the technique allows for single-shot measurements and keeps the temporal resolution associated with the full bandwidth of the probe pulse. We demonstrate the efficiency of this technique by probing femtosecond-laser breakdown of plastic targets.

Comparison of measured and calculated X-ray and hot-electron production in short-pulse laser-solid interactions at moderate intensities.

Ultrashort pulse laser-solid interaction experiments with 4x10(16) W/cm(2),120 fs, 45 degrees incidence angle, p-polarized pulses are theoretically analyzed with the help of 1(1/2)-dimensional (1(1/2) D) particle-in-cell (PIC) simulations. The laser impinges upon preformed plasmas with a precisely controlled density-gradient scale-length. PIC electron distribution functions are used as an input to 3D Monte Carlo simulations to interpret measured electron distributions and Kalpha radiation emission. Satisfactory agreement between the experimental and simulation results is obtained for the measured absorption coefficient, the energy distribution of the back-scattered hot electrons, the hot-electron temperature in the bulk of the target, and the Kalpha yield, when the preplasma scale-length is varied.

Hot-electron distribution functions in a subpicosecond laser interaction with solid targets of varying initial gradient scale lengths.

We have studied the distribution function of the hot electrons produced during the interaction of a 120-fs, 60-mJ, 800-nm wavelength and a p-polarized laser pulse with bilayered Al/Fe targets. The main pulse interacts with a preformed plasma, obtained with a controlled prepulse, whose density gradient scale length has been measured. The electron distribution function is characterized by means of the Kalpha emission of the two materials of the target as a function of the Al-layer thickness. The low-energy region (<50 keV) of the hot-electron distribution function shows no dependency in shape on the gradient scale length, but only a variation in the total number of the generated electrons. The comparison between the experimental results and the particle-in-cell and Monte Carlo calculations of the electron distribution function and the Kalpha emission is gratifying.

Frequency-domain interferometer for measuring the phase and amplitude of a femtosecond pulse probing a laser-produced plasma.

A frequency-domain interferometer for probing the variations of the dielectric constant of a plasma with sub-100- fs temporal resolution and lambda/2000 phase resolution is described. Imaging the plasma on the entrance slit of a spectrograph provides spatial resolution along a diameter of the focal spot. The technique is used to map out the expansion of the critical density surface of a femtosecond laser-produced plasma with subnanometer spatial resolution along the laser axis.