An interband cascade laser based heterodyne detector with integrated optical amplifier and local oscillator.

Heterodyne detection based on interband cascade lasers (ICL) has been demonstrated in a wide range of different applications. However, it is still often limited to bulky tabletop systems using individual components such as dual laser setups, beam shaping elements, and discrete detectors. In this work, a versatile integrated ICL platform is investigated for tackling this issue. A RF-optimized, two-section ICL approach is employed, consisting of a short section typically used for efficient modulation of the cavity field and a long gain section. Such a laser is operated in reversed mode, with the entire Fabry-Pérot waveguide utilized as a semiconductor optical amplifier (SOA) and the electrically separated short section as detector. Furthermore, a racetrack cavity is introduced as on-chip single-mode reference generator. The field of the racetrack cavity is coupled into the SOA waveguide via an 800 nm gap. By external injection of a single mode ICL operating at the appropriate wavelength, a heterodyne beating between the on-chip reference and the injected signal can be observed on the integrated detector section of the SOA-detector.

Mid-infrared supermirrors with finesse exceeding 400 000.

For trace gas sensing and precision spectroscopy, optical cavities incorporating low-loss mirrors are indispensable for path length and optical intensity enhancement. Optical interference coatings in the visible and near-infrared (NIR) spectral regions have achieved total optical losses below 2 parts per million (ppm), enabling a cavity finesse in excess of 1 million. However, such advancements have been lacking in the mid-infrared (MIR), despite substantial scientific interest. Here, we demonstrate a significant breakthrough in high-performance MIR mirrors, reporting substrate-transferred single-crystal interference coatings capable of cavity finesse values from 200 000 to 400 000 near 4.5 µm, with excess optical losses (scatter and absorption) below 5 ppm. In a first proof-of-concept demonstration, we achieve the lowest noise-equivalent absorption in a linear cavity ring-down spectrometer normalized by cavity length. This substantial improvement in performance will unlock a rich variety of MIR applications for atmospheric transport and environmental sciences, detection of fugitive emissions, process gas monitoring, breath-gas analysis, and verification of biogenic fuels and plastics.

Amplitude noise suppression in Yb:doped NALM oscillators utilizing saturable absorber settings.

Optical frequency combs based on fiber lasers mode-locked (ML) with a nonlinear amplifying loop mirror (NALM) have become the backbone of many cutting-edge applications, ranging from precision spectroscopy to quantum physics. Being extremely precise measurement tools, understanding their passive stability and low-noise operation regimes is vital. While several influences on the laser noise have been studied, many parameters remain poorly understood. Here, we systematically analyze under which preconditions the artificial saturable absorber settings of the laser can be modified during operation without losing mode-locking and the effects on laser noise, the spectrum and the output power. Our results show that it is possible to decrease the amplitude noise (AM noise) of the laser by more than 50 % by simply rotating a wave plate within the laser cavity. Additionally, we discuss differences to a similar effect observed in a NALM-alike laser amplifier and of changing the output coupling. These findings deepen our understanding and capabilities of optimizing the noise performance of ML fiber lasers, enable us to investigate new parameter spaces, and can be used to further optimize the noise performance of the NALM laser design, making it an ideal light source for advanced setups both in research and industry.

Simple approach for extending the ambiguity-free range of dual-comb ranging.

Dual-comb (DC) ranging is an established method for high-precision and high-accuracy distance measurements. It is, however, restricted by an inherent length ambiguity and the requirement for complex control loops for comb stabilization. Here, we present a simple approach for expanding the ambiguity-free measurement length of DC ranging by exploiting the intrinsic intensity modulation of a single-cavity dual-color DC for simultaneous time-of-flight and DC distance measurements. This measurement approach enables the measurement of distances up to several hundred kilometers with the precision and accuracy of a DC interferometric setup while providing a high data acquisition rate (≈2kHz) and requiring only the repetition rate of one of the combs to be stabilized.

Flexible all-PM NALM Yb:fiber laser design for frequency comb applications: operation regimes and their noise properties.

We present a flexible all-polarization-maintaining (PM) mode-locked ytterbium (Yb):fiber laser based on a nonlinear amplifying loop mirror (NALM). In addition to providing detailed design considerations, we discuss the different operation regimes accessible by this versatile laser architecture and experimentally analyze five representative mode-locking states. These five states were obtained in a 78-MHz configuration at different intracavity group delay dispersion (GDD) values ranging from anomalous (-0.035 ps2) to normal (+0.015 ps2). We put a particular focus on the characterization of the intensity noise as well as the free-running linewidth of the carrier-envelope-offset (CEO) frequency as a function of the different operation regimes. We observe that operation points far from the spontaneous emission peak of Yb (∼1030 nm) and close to zero intracavity dispersion can be found, where the influence of pump noise is strongly suppressed. For such an operation point, we show that a CEO linewidth of less than 10-kHz at 1 s integration can be obtained without any active stabilization.

Tunable dual-comb from an all-polarization-maintaining single-cavity dual-color Yb:fiber laser.

We demonstrate dual-comb generation from an all-polarization-maintaining dual-color ytterbium (Yb) fiber laser. Two pulse trains with center wavelengths at 1030 nm and 1060 nm respectively are generated within the same laser cavity with a repetition rate around 77 MHz. Dual-color operation is induced using a tunable mechanical spectral filter, which cuts the gain spectrum into two spectral regions that can be independently mode-locked. Spectral overlap of the two pulse trains is achieved outside the laser cavity by amplifying the 1030-nm pulses and broadening them in a nonlinear fiber. Spatially overlapping the two arms on a simple photodiode then generates a down-converted radio frequency comb. The difference in repetition rates between the two pulse trains and hence the line spacing of the down-converted comb can easily be tuned in this setup. This feature allows for a flexible adjustment of the tradeoff between non-aliasing bandwidth vs. measurement time in spectroscopy applications. Furthermore, we show that by fine-tuning the center-wavelengths of the two pulse trains, we are able to shift the down-converted frequency comb along the radio-frequency axis. The usability of this dual-comb setup is demonstrated by measuring the transmission of two different etalons while the laser is completely free-running.

Tunable dual-color operation of Yb:fiber laser via mechanical spectral subdivision.

We present a versatile method to generate a dual-color laser from a single fiber laser cavity by spectral subdivision using a tunable mechanical filter. As a proof-of-principle, we implement the concept in a nonlinear polarization evolution (NPE)-mode-locked ytterbium (Yb)-fiber laser. The division into two independent spectral regions is achieved by inserting a narrow blade-shaped beam block into the free-space grating compressor section of the cavity, where the spectrum is spatially dispersed. By mode-locking both spectral regions, two pulse trains, with different repetition rates around 23 MHz, are generated. Each pulse train has a FWHM of ~10 nm. The method presented here enables tuning of the difference in repetition rate as well as the spectral separation of the two independent pulse trains. The difference in repetition rates originates from intracavity dispersion and can be tuned over a large range (650 Hz - 3 kHz in this setup) by changing the length of the grating compressor. By changing the effective width of the beam block the spectral separation can be dynamically adjusted. This approach's simplicity holds great promises for the development of single-cavity dual-comb lasers featuring tunable sampling rates.

Phase-stabilized 100 mW frequency comb near 10 µm.

Long-wavelength mid-infrared (MIR) frequency combs with high power and flexible tunability are highly desired for molecular spectroscopy, including investigation of large molecules such as C60. We present a high power, phase-stabilized frequency comb near 10 µm, generated by a synchronously pumped, singly resonant optical parametric oscillator (OPO) based on AgGaSe2. The OPO can be continuously tuned from 8.4 to 9.5 µm, with a maximum average idler power of 100 mW at the center wavelength of 8.5 µm. Both the repetition rate (f rep) and the carrier-envelope offset frequency (f ceo) of the idler wave are phase-locked to microwave signals referenced to a Cs clock. We describe the detailed design and construction of the frequency comb, and discuss potential applications for precise and sensitive direct frequency comb spectroscopy.

Three-photon absorption in optical parametric oscillators based on OP-GaAs.

We report on, to the best of our knowledge, the first singly resonant (SR), synchronously pumped optical parametric oscillator (OPO) based on orientation-patterned gallium arsenide (OP-GaAs). Together with a doubly resonant (DR) degenerate OPO based on the same OP-GaAs material, the output spectra cover 3 to 6 µm within ∼3 dB of relative power. The DR-OPO has the highest output power reported to date from a femtosecond, synchronously pumped OPO based on OP-GaAs. We observed strong three-photon absorption with a coefficient of 0.35±0.08 cm3/GW2 for our OP-GaAs sample, which limits the output power of these OPOs as mid-IR light sources. We present a detailed study of the three-photon loss on the performance of both the SR- and DR-OPOs, and compare them to those without this loss mechanism.

Continuous probing of cold complex molecules with infrared frequency comb spectroscopy.

For more than half a century, high-resolution infrared spectroscopy has played a crucial role in probing molecular structure and dynamics. Such studies have so far been largely restricted to relatively small and simple systems, because at room temperature even molecules of modest size already occupy many millions of rotational/vibrational states, yielding highly congested spectra that are difficult to assign. Targeting more complex molecules requires methods that can record broadband infrared spectra (that is, spanning multiple vibrational bands) with both high resolution and high sensitivity. However, infrared spectroscopic techniques have hitherto been limited either by narrow bandwidth and long acquisition time, or by low sensitivity and resolution. Cavity-enhanced direct frequency comb spectroscopy (CE-DFCS) combines the inherent broad bandwidth and high resolution of an optical frequency comb with the high detection sensitivity provided by a high-finesse enhancement cavity, but it still suffers from spectral congestion. Here we show that this problem can be overcome by using buffer gas cooling to produce continuous, cold samples of molecules that are then subjected to CE-DFCS. This integration allows us to acquire a rotationally resolved direct absorption spectrum in the C-H stretching region of nitromethane, a model system that challenges our understanding of large-amplitude vibrational motion. We have also used this technique on several large organic molecules that are of fundamental spectroscopic and astrochemical relevance, including naphthalene, adamantane and hexamethylenetetramine. These findings establish the value of our approach for studying much larger and more complex molecules than have been probed so far, enabling complex molecules and their kinetics to be studied with orders-of-magnitude improvements in efficiency, spectral resolution and specificity.

Beam delivery and pulse compression to sub-50 fs of a modelocked thin-disk laser in a gas-filled Kagome-type HC-PCF fiber.

We present two experiments confirming that hypocycloid Kagome-type hollow-core photonic crystal fibers (HC-PCFs) are excellent candidates for beam delivery of MW peak powers and pulse compression down to the sub-50 fs regime. We demonstrate temporal pulse compression of a 1030-nm Yb:YAG thin disk laser providing 860 fs, 1.9 µJ pulses at 3.9 MHz. Using a single-pass grating pulse compressor, we obtained a pulse duration of 48 fs (FWHM), a spectral bandwidth of 58 nm, and an average output power of 4.2 W with an overall power efficiency into the final polarized compressed pulse of 56%. The pulse energy was 1.1 µJ. This corresponds to a peak power of more than 10 MW and a compression factor of 18 taking into account the exact temporal pulse profile measured with a SHG FROG. The compressed pulses were close to the transform limit of 44 fs. Moreover, we present transmission of up to 97 µJ pulses at 10.5 ps through 10-cm long fiber, corresponding to more than twice the critical peak power for self-focusing in silica.

275 W average output power from a femtosecond thin disk oscillator operated in a vacuum environment.

We present an ultrafast thin disk laser that generates an average output power of 275 W, which is higher than any other modelocked laser oscillator. It is based on the gain material Yb:YAG and operates at a pulse duration of 583 fs and a repetition rate of 16.3 MHz resulting in a pulse energy of 16.9 µJ and a peak power of 25.6 MW. A SESAM designed for high damage threshold initiated and stabilized soliton modelocking. We reduced the nonlinearity of the atmosphere inside the cavity by several orders of magnitude by operating the oscillator in a vacuum environment. Thus soliton modelocking was achieved at moderate amounts of self-phase modulation and negative group delay dispersion. Our approach opens a new avenue for power scaling femtosecond oscillators to the kW level.

Self-referenceable frequency comb from an ultrafast thin disk laser.

We present the first measurement of the carrier envelope offset (CEO) frequency of an ultrafast thin disk laser (TDL). The TDL used for this proof-of-principle experiment was based on the gain material Yb:Lu(2)O(3) and delivered 7 W of average power in 142-fs pulses, which is more than two times shorter than previously realized with this material. Using only 65 mW of the output of the laser, we generated a coherent octave-spanning supercontinuum (SC) in a highly nonlinear photonic crystal fiber (PCF). We detected the CEO beat signal using a standard f-to-2f interferometer, achieving a signal-to-noise ratio of >25 dB (3 kHz resolution bandwidth). The CEO frequency was tunable with the pump current with a slope of 33 kHz/mA. This result opens the door towards high-power frequency combs from unamplified oscillators. Furthermore, it confirms the suitability of these sources for future intralaser extreme nonlinear optics experiments such as high harmonic generation and VUV frequency comb generation from compact sources.

Frontiers in passively mode-locked high-power thin disk laser oscillators.

Semiconductor saturable absorber mirror (SESAM) mode-locked thin disk lasers define the state-of-the-art performance for high average power and high pulse energy femtosecond laser oscillators. To date pulse energies above 30 µJ and average powers above 140 W have been demonstrated. In this paper we review the achievements of mode-locked thin disk lasers in terms of average power and pulse energy. Stable mode locking requires single transverse mode operation even at the highest average power, which is challenging and therefore addressed in more detail. We then summarize our expectations on the main challenges and limitiations for the next generation of mode-locked thin disk laser oscillators with an average power above 500 W and pulse energies in excess of 100 µJ.

SESAMs for high-power femtosecond modelocking: power scaling of an Yb:LuScO3 thin disk laser to 23 W and 235 fs.

We report on power scaling of a modelocked thin disk laser based on the broadband mixed sesquioxide material Yb:LuScO3. One of the key elements to achieve this result was an improved SESAM design with reduced two-photon-absorption (TPA) and high damage threshold. In a first experiment, using a standard antiresonant SESAM with no topcoating, we could demonstrate record short pulse durations of 195 fs at a moderate average power of 9.5 W. Furthermore, we were able to power scale our thin disk laser while keeping the pulses short reaching 23 W at a pulse duration of 235 fs. This was made possible by designing a new SESAM with multiple quantum wells (QW) and a suitable dielectric topcoating. We will present SESAM optimization guidelines for short pulse generation from high-power modelocked oscillators.

227-fs pulses from a mode-locked Yb:LuScO3 thin disk laser.

We report on the first mode-locked thin disk laser based on Yb:LuScO(3). This new mixed gain material combines the emission peaks of two sesquioxides, leading to a gain bandwidth of more than 20 nm. We achieve 7.2 W average output power in 227-fs pulses, which is shorter than for any previous ultrafast thin disk laser. The output power was limited by a growth defect near the center of the thin disk.