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1.
Phys Rev Lett ; 110(1): 017004, 2013 Jan 04.
Artículo en Inglés | MEDLINE | ID: mdl-23383829

RESUMEN

We have performed inelastic neutron scattering measurements on the single-layer cuprate Bi(2+x) Sr(2-x) CuO(6+y) (Bi2201) with x = 0.2, 0.3, 0.4, and 0.5, a doping range that spans the spin-glass to superconducting phase boundary. The doping evolution of low energy spin fluctuations (11

2.
Phys Rev Lett ; 107(12): 127002, 2011 Sep 16.
Artículo en Inglés | MEDLINE | ID: mdl-22026791

RESUMEN

We demonstrated experimentally a direct way to probe a hidden propensity to the formation of a spin-density wave in a nonmagnetic metal with strong Fermi surface nesting. Substituting Fe for a tiny amount of Cu (1%) induced an incommensurate magnetic order below 20 K in heavily overdoped La(2-x)Sr(x)CuO(4). Elastic neutron scattering suggested that this order cannot be ascribed to the localized spins on Cu or doped Fe. Angle-resolved photoemission revealed a strong Fermi surface nesting inherent in the pristine La(2-x)Sr(x)CuO(4) that likely drives this order. Our finding presents the first example of the long-sought "itinerant-spin extreme" of cuprates, where the spins of itinerant doped holes define the magnetic ordering ground state; it complements the current picture of cuprate spin physics that highlights the predominant role of localized spins at lower dopings.

3.
Phys Rev Lett ; 101(20): 205901, 2008 Nov 14.
Artículo en Inglés | MEDLINE | ID: mdl-19113356

RESUMEN

Giant negative thermal expansion is achieved in antiperovskite manganese nitrides when the sharp volume change associated with magnetic ordering is broadened by substitution. In this Letter, we address the unique role of the ''magic" element, Ge, for such broadening in Mn3Cu1-xGexN. We present evidence for a local lattice distortion well described by the low-temperature tetragonal (T4) structure of Mn3GeN for a range of x, where the overall structure remains cubic. This structural instability shows a strong correlation with the broadness of the growth of the ordered magnetic moment and, hence, is considered to trigger the broadening of the volume change.

4.
Nature ; 440(7088): 1170-3, 2006 Apr 27.
Artículo en Inglés | MEDLINE | ID: mdl-16641991

RESUMEN

The attempt to understand copper oxide superconductors is complicated by the presence of multiple strong interactions in these systems. Many believe that antiferromagnetism is important for superconductivity, but there has been renewed interest in the possible role of electron-lattice coupling. The conventional superconductor MgB2 has a very strong electron-lattice coupling, involving a particular vibrational mode (phonon) that was predicted by standard theory and confirmed quantitatively by experiment. Here we present inelastic scattering measurements that show a similarly strong anomaly in the Cu-O bond-stretching phonon in the copper oxide superconductors La(2-x)Sr(x)CuO4 (with x = 0.07, 0.15). Conventional theory does not predict such behaviour. The anomaly is strongest in La(1.875)Ba(0.125)CuO4 and La(1.48)Nd(0.4)Sr(0.12)CuO4, compounds that exhibit spatially modulated charge and magnetic order, often called stripe order; it occurs at a wave vector corresponding to the charge order. These results suggest that this giant electron-phonon anomaly, which is absent in undoped and over-doped non-superconductors, is associated with charge inhomogeneity. It follows that electron-phonon coupling may be important to our understanding of superconductivity, although its contribution is likely to be indirect.

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