Standardization of Rn-222 concentration using the multi-electrode proportional counter.

Standardization of the concentration of gaseous 222Rn based on a multi-electrode proportional counter (MEPC) is under development as a primary standard in Japan. In this study, the concept and evaluation of its performance are reported. The latter consists of a preliminary result for the uncertainty budget associated with the measurement of the MEPC and compensation of the electric field distortion in the MEPC. Moreover, an ionization-chamber-based gas circulation system was added for the calibration of radon monitors in the air.

Machine learning in environmental radon science.

Temporal dynamic as well as spatial variability of environmental radon are controlled by factors such as meteorology, lithology, soil properties, hydrogeology, tectonics, and seismicity. In addition, indoor radon concentration is subject to anthropogenic factors, such as physical characteristics of a building and usage pattern. New tools for spatial and time series analysis and prediction belong to what is commonly called machine learning (ML). The ML algorithms presented here build models based on sample and predictor data to extract information and to make predictions. We give a short overview on ML methods and discuss their respective merits, their application, and ways of validating results. We show examples of 1) geogenic radon mapping in Germany involving a number of predictors, and of 2) time series analysis of a long-term experiment being carried out in Chiba, Japan, involving indoor radon concentrations and meteorological predictors. Finally, we identified the main weakness of the techniques, and we suggest actions to overcome their limitations.

Radon Exposure in the Underground Tourist Route-Historic Silver Mine in Tarnowskie Góry, Poland.

An assessment of the exposure of workers and tourists to radon in the underground tourist route of the Historic Silver Mine in Tarnowskie Góry was carried out. The study was conducted over a one-year period to capture seasonal variations in radon concentrations. CR-39 track detectors were used to measure radon concentrations, which were exposed in the mine during the following periods: 9 February 2021-19 May 2021, 19 May 2021-26 August 2021, 26 August 2021-25 November 2021 and 25 November 2021-3 March 2022. The annual average radon concentration along the tourist route was 1021 Bq m-3. The highest measured concentration was 2280 Bq m-3 and the lowest concentration was 80 Bq m-3. Based on the measured concentrations, effective doses were calculated, assuming that employees spend 1350 h a year in underground areas and that the time of visiting the mine by tourists is ca. 1 h. The average annual effective dose a worker would receive is approximately 2.5 mSv, and a tourist below 2 µSv. The dose limit expressed as the annual effective dose is 1 mSv for members of the general public and 20 mSv for occupational exposure.

Environmental Radioactivity Monitoring and Measurements: Radon and Thoron.

We "bathe" in radiation, which is an integral part of our environment [...].

Status of radon exposure in Bangladeshi locations and dwellings.

Potentially higher cancer risk due to exposure from natural background radiation was indicated for the Bangladeshi population by estimations based on the countrywide study. Several regions with elevated natural background exhibited higher soil radium and thorium contents than the world average. Being the decay products of these radioactive elements, natural radon isotopes could constitute environmental risk factors for internal radiation exposure to the lungs of people living in these areas. Although lung cancer is one of the most prevalent types of cancer in Bangladesh, its status and features are still unclear. To clarify the present status of one of the potential risk factors for lung cancer in the country, this review intends to ascertain the countrywide radon exposure, and its pathways by types of local dwelling and by regions, which would provide an indication of the internal exposures in areas of elevated natural background radiation and radionuclides of soil as well as an understanding of the preliminary contribution of environmental radon on the country's lung cancer prevalence. In this review, countrywide monitored air radon exposures for Bangladeshi dwellings and workplaces are organized from peer-reviewed published papers. Radon has been identified as one of influential sources of radiation dose in Bangladesh with its higher radon exhalation and emanation rate from soil. A novel nationwide depiction of the overall assessed indoor and soil radon levels for Bangladesh has been made through radiation maps. This would be helpful for designing future systematic radon/radiological monitoring and research on the country's lung cancer prevalence.

Effects of Storage Time and Pre-Etching Treatment of CR-39 Detectors on Their Response to Alpha Radiation Exposure.

Radon passive monitors based on solid state nuclear track detectors (SSNTD), especially CR-39, are widely used in radon and thoron studies. They may be subjected to the influence of external factors, like changing of temperature, humidity, and pressure, both before and during the measurement. Evaluation of the exposed detectors involves chemical processing, whose conditions also influence the measurement results. The aim of this study was to check several factors, as to whether they may modify the response of CR-39 detector: concerning the phase before evaluation, storage time, and temperature during storage; and concerning the evaluation procedure, etching time, and pre-etching treatment using hot water and carbon dioxide atmosphere. Two experiments were conducted by irradiation of CR-39 detectors using alpha particles emitted from a mono-energetic 241Am source and exposed in radon atmosphere. Track density dependence of the age of production was found to be statistically not significant. On the other hand, pre-etching treatment using hot water and carbon dioxide with different etching times showed statistically significant effects on track area, track sensitivity, and roundness. It was concluded that there are simple methods to increase performance of nuclear track detectors, and that storage time is not a factor of concern.

Passive-Type Radon Monitor Constructed Using a Small Container for Personal Dosimetry.

The International Commission on Radiological Protection (ICRP) recently recommended a new dose conversion factor for radon based on the latest epidemiological studies and dosimetric model. It is important to evaluate an inhalation dose from radon and its progeny. In the present study, a passive radon personal monitor was designed using a small container for storing contact lenses and its performance was evaluated. The conversion factor for radon (222Rn), the effect of thoron (220Rn) concentration and the air exchange rate were evaluated using the calibration chamber at Hirosaki University. The minimum and maximum detectable radon concentrations were calculated. The conversion factor was evaluated as 2.0 ± 0.3 tracks cm-2 per kBq h m-3; statistical analyses of results showed no significant effect from thoron concentration. The minimum and maximum detectable radon concentrations were 92 Bq m-3 and 231 kBq m-3 for a measurement period of three months, respectively. The air exchange rate was estimated to be 0.26 ± 0.16 h-1, whose effect on the measured time-integrated radon concentration was small. These results indicate that the monitor could be used as a wearable monitor for radon measurements, especially in places where radon concentrations may be relatively high, such as mines and caves.

Variable Strength in Thoron Interference for a Diffusion-Type Radon Monitor Depending on Ventilation of the Outer Air.

Thoron interference in radon measurements using passive diffusion radon detectors/monitors is a crucial problem when it comes to assessing the internal exposure to radon precisely. The present study reported, as one of the potential factors, the effects of air flow conditions on changes in thoron interference. Rates of thoron infiltration (as thoron interference) into the diffusion chamber of the monitor were evaluated. The temporal variation was obtained based on measurements of the underfloor space of a Japanese wooden dwelling using a diffusion-type radon monitor, a reference radon monitor which was not affected by thoron interference, and a thoron monitor. The thoron infiltration rate for the diffusion-type monitor varied from 0% to 20%. In particular, it appeared to increase when ventilation of the underfloor space air was forced. The variable thoron infiltration rate, with respect to ventilation strength, implied that not only a diffusive process, but also an advective process, played a major role in air exchange between the diffusion chamber of the monitor and the outer air. When an exposure room is characterized by the frequent variation in air ventilation, a variable thoron response is considered to occur in radon-thoron discriminative detectors, in which only diffusive entry is employed as a mechanism for the discrimination of radon and thoron.

Comparison of Radon and Thoron Concentration Measuring Systems Among Asian Countries.

Comparison is an important role in the quality control and quality assurance for any measuring system. Due to the future legal regulations regarding radon levels in the air, maintaining the system quality and harmonization of results as well as validation of radon and thoron measuring systems is important. The aim of this work is to validate the degrees of equivalence and measurement precisions of the existing five radon and four thoron measuring systems located in four Asian countries (China, India, Japan and Thailand) through comparison experiment. In this project, comparison experiment was performed in order to derive the ratio between assigned value obtained from one transfer measurement device for radon and one transfer measurement device for thoron belongs to National Institutes for Quantum and Radiological Science and Technology and participants' value from their measuring instrument. As a result, the ratio value associated with measurement uncertainty was derived for each activity concentration. Finally, measurement bias and degrees of equivalence between the assigned values and values of measurement quantity from participants' measuring instruments were statistically analysed and presented.

EVALUATION OF A RADON AIR MONITOR IN THE MEASUREMENT OF RADON CONCENTRATION IN WATER IN COMPARISON WITH A LIQUID SCINTILLATION COUNTER.

The World Health Organisation (WHO) recommends that the concentration of radon in water should be no more than 100 kBq m-3 (100 BqL-1) and the Codex Alimentarius Commission states that the limit of quantification (LOQ) of a method should be no more than one-fifth of this value. In this study, a degassing method with an RAD7 device was used to measure radon concentrations in water, compared to a liquid scintillation counter (LSC) method used as the reference, to investigate whether the numerical value of the LOQ of this method was more than 1/5 (20 kBq m-3) of 100 kBq m-3. The degassing method with leak prevention was shown to reach a target value of 20 kBq m-3 or less under a relative humidity of 6% or lower in the chamber of the RAD7 device. Accordingly, the RAD7 degassing method with leak prevention can be used to accurately measure radon concentrations in water within the guidance level set out by the WHO.

PRELIMINARY TECHNICAL DISCUSSION ON A NEW RADON AND ITS PROGENY CONTINUOUS MONITOR USING TWO-FILTER METHOD.

Focusing on the scalability of Two-Filter Method, we started to develop a monitor for the concentration of radon and its progeny. In this study, we investigated the influence of a high-humidity environment on measuring radon concentration, and the influence of the decay chamber of the monitor on the measurement. In the high-humidity test, the conversion factor of (Bqm-3)/(cpm) tends to raise with increasing humidity. On the measurement of radon progeny, existence of the decay chamber of the monitor makes measurement sensitivity lower under environments of little aerosols. Radon concentration measurement by the developed monitor could be influenced by environmental humidity, and that counting loss could occur due to deposition of radon progeny inside of the decay chamber. Correction relating these would be needed based on the data of calibration tests.

Environmentally Friendly Measurement of Airborne Radon Using a Nonvolatile Liquid Scintillation Absorbent.

The practicality of using a liquid scintillation method with a nonvolatile liquid scintillation absorbent for the measurement of airborne Rn (radon) in a residence was examined. The relationship between the radioactivity absorbed by the liquid scintillation absorbent and the radon concentration in the air was investigated in a calibrated walk-in radon chamber. The equivalent radioactivity of radon was calculated for Po radioactivity immediately after radioactive equilibrium was attained using successive decay equations via alpha-particle spectrometry based on the 1 h, indirect, selective measurement of the Po alpha-particle spectrum generated after sampling radon. We confirmed that the amounts of radon absorbed in the liquid scintillation absorbent were proportional to the radon concentration in the air. The calibration curve that exhibited reliable quantitative linearity from 500 to 8,000 Bq m in air was extrapolated to the region between 0 and 500 Bq m using the least-squares method with data from 500 to 8,000 Bq m. The validity of the extrapolated curve at less than 500 Bq m was confirmed by comparison of the measured radon concentrations in the room and atmosphere with those determined using an existing ionization chamber. Variations in the absorption of radon were observed due to changes in temperature and humidity. The health and environmental safety of nonvolatile liquid scintillation absorbent was also considered.

Optimization of the Timepix chip to measurement of radon, thoron and their progenies.

Radon and thoron as well as their short-lived progenies are decay products of the radium and thorium series decays. They are the most important radionuclide elements with respect to public exposure. To utilize the semiconductor pixel radiation Timepix chip for the measurement of active and real-time alpha particles from radon, thoron and their progenies, it is necessary to check the registration and visualization of the chip. An energy check for radon, thoron and their progenies, as well as for (241)Am and(210)Po sources, was performed using the radon and thoron chambers at NIRS (National Institute of Radiological Sciences). The check found an energy resolution of 200 keV with a 14% efficiency as well as a linear dependency between the channel number (cluster volume) and the energy. The coefficient of determination r(2) of 0.99 for the range of 5 to 9 MeV was calculated. In addition, an offset for specific Timepix configurations between pre-calibration for low energy from 6 to 60 keV, and the actual calibration for alpha particles with energies from 4000 to 9000 keV, was detected.

An intercomparison done at NIRS, Japan on continuous monitors for measuring ²²°Rn concentration.

An intercomparison for continuous monitors that measure thoron ((220)Rn) concentration was carried out using a (220)Rn chamber of National Institute of Radiological Sciences (NIRS), Japan; eleven (220)Rn monitors (four types) from nine laboratories were evaluated. The (220)Rn detection principle was the same for the eleven instruments and one reference instrument, which were commercially available silicon semiconductor detectors using an electrostatic collection method. The intercomparison results showed that there was a negative deviation of more than 30% in measured (220)Rn concentrations given by the laboratories relative to the reference values, which were obtained by making a decay-correction during the travel of (220)Rn through the sampling assembly (sample tube, filter and drying unit) and using a calibration factor. In order to elucidate the reason for this and then to investigate factors that affect the (220)Rn concentration measured with the monitors. As a result, it was necessary to make the decay-correction, in particular, when using a drying unit with a large inner volume and to use the calibration factor in order to better estimate the (220)Rn concentration. It was also found to be better to determine a calibration factor inherent to an individual monitor, because the calibration factor values ranged from 0.75 to 2.32, depending on the flow rate of the monitor pump (0.37-1.02 L min(-1)). It was concluded from this study that a periodical calibration of the monitor and a check of the monitor flow rate during measurements are necessary to maintain a consistent quality level of the (220)Rn measurement.

Radon-thoron discriminative measurements in the high natural radiation areas of southwestern Cameroon.

Although indoor radon was initially measured in the uranium regions of Poli and Lolodorf using Electret Ionization Chambers, discriminative RADUET detectors were deployed in 70 houses of the high natural radiation areas of Bikoue and Ngombas in the uranium region of Lolodorf in Southwestern Cameroon. Radon and thoron concentrations were determined using Image-J and Microscope Methods for track evaluation. Radon and thoron concentrations follow lognormal distributions and ranged respectively from 27 ± 26 to 937 ± 5 Bq m(-3) and from 48 ± 40 to 700 ± 128 Bq m(-3). The arithmetic means of radon and thoron concentrations were found to be 92 ± 3 Bq m(-3) and 260 ± 13 Bq m(-3.) Less than 2% of houses have indoor radon above the reference level of 300 Bq m(-3) and 30% of houses have thoron concentrations above 300 Bq m(-3.) Inhalation doses due to radon and thoron range respectively between 0.6-17.7 mSv yr(-1) and 0.2-3 mSv yr(-1) with the mean values of 1.4 mSv yr(-1) and 1 mSv yr(-1). The contribution of indoor thoron to the total inhalation dose ranges between 15%- 78.5% with the mean value of 47%. Thus thoron cannot be neglected when assessing radiation dose.

Novel method for estimation of the indoor-to-outdoor airborne radioactivity ratio following the Fukushima Daiichi Nuclear Power Plant accident.

The accident at the Fukushima Daiichi Nuclear Power Plant (FDNPP) in Japan resulted in significant releases of fission products. While substantial data exist concerning outdoor air radioactivity following the accident, the resulting indoor radioactivity remains pure speculation without a proper method for estimating the ratio of the indoor to outdoor airborne radioactivity, termed the airborne sheltering factor (ASF). Lacking a meaningful value of the ASF, it is difficult to assess the inhalation doses to residents and evacuees even when outdoor radionuclide concentrations are available. A simple model was developed and the key parameters needed to estimate the ASF were obtained through data fitting of selected indoor and outdoor airborne radioactivity measurement data obtained following the accident at a single location. Using the new model with values of the air exchange rate, interior air volume, and the inner surface area of the dwellings, the ASF can be estimated for a variety of dwelling types. Assessment of the inhalation dose to individuals readily follows from the value of the ASF, the person's indoor occupancy factor, and the measured outdoor radioactivity concentration.

Invited article: in situ comparison of passive radon-thoron discriminative monitors at subsurface workplaces in Hungary.

During a one-year long measurement period, radon and thoron data obtained by two different passive radon-thoron discriminative monitors were compared at subsurface workplaces in Hungary, such as mines (bauxite and manganese ore) and caves (medical and touristic). These workplaces have special environmental conditions, such as, stable and high relative humidity (100%), relatively stable temperature (12°C-21°C), low or high wind speed (max. 2.4 m s(-1)) and low or elevated aerosol concentration (130-60,000 particles m(-3)). The measured radon and thoron concentrations fluctuated in a wide range among the different workplaces. The respective annual average radon concentrations and their standard deviations (in brackets) measured by the passive radon-thoron discriminative monitor with cellulose filter (CF) and the passive radon-thoron discriminative monitor with sponge filter (SF) were: 350(321) Bq m(-3) and 550(497) Bq m(-3) in the bauxite mine; 887(604) Bq m(-3) and 1258(788) Bq m(-3) in the manganese ore mine; 2510(2341) Bq m(-3) and 3403(3075) Bq m(-3) in the medical cave (Hospital Cave of Tapolca); and 6239(2057) Bq m(-3) and 8512(1955) Bq m(-3) in the touristic cave (Lake Cave of Tapolca). The respective average thoron concentrations and their standard deviation (in brackets) measured by CF and SF monitors were: 154(210) Bq m(-3) and 161(148) Bq m(-3) in the bauxite mine; 187(191) Bq m(-3) and 117(147) Bq m(-3) in the manganese-ore mine; 360(524) Bq m(-3) and 371(789) Bq m(-3) in the medical cave (Hospital Cave of Tapolca); and 1420(1184) Bq m(-3) and 1462(3655) Bq m(-3) in the touristic cave (Lake Cave of Tapolca). Under these circumstances, comparison of the radon data for the SF and CF monitors showed the former were consistently 51% higher in the bauxite mine, 38% higher in the manganese ore mine, and 34% higher in the caves. Consequently, correction is required on previously obtained radon data acquired by CF monitors at subsurface workplaces to gain comparable data for SF monitors. In the case of thoron, the data were unreliable and no significant tendency was seen during the comparison therefore comparison of previously obtained thoron data acquired by either CF or SF is doubtful. There was probable influence by relative humidity on the detection response; however, the effects of the high wind speed and elevated aerosol concentration could not be excluded. The results of this study call attention to the importance of calibration under extreme environmental conditions and the need for using reliable radon-thoron monitors for subsurface workplaces.

Simultaneous sampling of indoor and outdoor airborne radioactivity after the Fukushima Daiichi nuclear power plant accident.

Several studies have estimated inhalation doses for the public because of the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident. Most of them were based on measurement of radioactivity in outdoor air and included the assumption that people stayed outdoors all day. Although this assumption gives a conservative estimate, it is not realistic. The "air decontamination factor" (ratio of indoor to outdoor air radionuclide concentrations) was estimated from simultaneous sampling of radioactivity in both inside and outside air of one building. The building was a workplace and located at the National Institute of Radiological Sciences (NIRS) in Chiba Prefecture, Japan. Aerosol-associated radioactive materials in air were collected onto filters, and the filters were analyzed by γ spectrometry at NIRS. The filter sampling was started on March 15, 2011 and was continued for more than 1 year. Several radionuclides, such as (131)I, (134)Cs, and (137)Cs were found by measuring the filters with a germanium detector. The air decontamination factor was around 0.64 for particulate (131)I and 0.58 for (137)Cs. These values could give implications for the ratio of indoor to outdoor radionuclide concentrations after the FDNPP accident for a similar type of building.

Comparative analysis of radon, thoron and thoron progeny concentration measurements.

This study examined correlations between radon, thoron and thoron progeny concentrations based on surveys conducted in several different countries. For this purpose, passive detectors developed or modified by the National Institute of Radiological Sciences (NIRS) were used. Radon and thoron concentrations were measured using passive discriminative radon-thoron detectors. Thoron progeny measurements were conducted using the NIRS-modified detector, originally developed by Zhuo and Iida. Weak correlations were found between radon and thoron as well as between thoron and thoron progeny. The statistical evaluation showed that attention should be paid to the thoron equilibrium factor for calculation of thoron progeny concentrations based on thoron measurements. In addition, this evaluation indicated that radon, thoron and thoron progeny were independent parameters, so it would be difficult to estimate the concentration of one from those of the others.