RESUMEN
In this study we explore optical absorptance of single-layer hafnia dielectric coatings deposited on fused silica by ion beam sputtering technique. We investigate both linear and nonlinear absorptance by varying the laser intensity of 10 ps pulses at a 1 MHz repetition rate across wavelengths of 1064 nm, 532 nm, and 355 nm. Significant differences were observed between the as-deposited and thermally treated coatings. The as-deposited sample exhibited diminishing absorptance, while the thermally treated coatings showed an increase in absorption. Furthermore, our study delves into the strong impact of the pump wavelength on the nonlinear response. These findings bear potential significance in enhancing our understanding of the long-term effects in optical coatings. This understanding could prove crucial in the context of fatigue or laser-induced damage.
RESUMEN
The effectiveness of ultrashort pulse compression depends on the coatings group delay dispersion (GDD) characteristics in chirped mirror (CM)-based optical systems. Current porous-layer-based CMs with low GDD oscillations are limited to less than half optical octave spectral bandwidth and the stability of their spectral parameters is still unknown. In order to address these limitations, a broadband CM (covering 400 nm bandwidth) with a porous top layer was deposited and spectral parameters were measured at different environmental conditions. The modeled refractive index of the porous layer varied by approximately 1% due to the changes in humidity. Deposited coatings exhibited low sensitivity of GDD oscillations to deposition errors of porous layer and humidity in the surrounding environment.
RESUMEN
The decrease of laser-induced damage threshold (LIDT) when exposed with high number of laser pulses is a well-known phenomenon in dielectrics. In the femtosecond regime this fatigue is usually attributed to the incubation of laser-induced lattice defects. In this work, a computational model is used to combine the data from time-resolved digital holographic microscopy measurements together with results of S-on-1 laser-induced damage threshold test in order to investigate fatigue of ZrO 2 single layer coating. Two distinct damage modes were identified and shown to follow different fatigue behaviors: formation of catastrophic damage is highly nonlinear in time, while incubation of color-change mode appears to be linear in time.
RESUMEN
In this paper, the relation between the laser-induced damage threshold (LIDT) and the electric field intensity (EFI) distribution inside a CM is investigated experimentally. We show that it is possible to increase the LIDT values by slightly modifying the electric field of a standing wave distribution without loss of spectral and dispersion performance. Suggested CM design improvement could increase reliability and LIDT performance of both CM elements and high-power systems they are used in.
RESUMEN
We report on the laser damage resistance of ion beam-sputtered oxide materials (Al2O3, Nb2O5, HfO2, SiO2, Ta2O5, ZrO2) and mixtures of Al2O3-SiO2, Nb2O5-SiO2, HfO2-SiO2, Ta2O5-SiO2, and ZrO2-SiO2, irradiated by single 500 fs pulses at 1030 nm. Laser-induced damage threshold (LIDT), refractive index, and bandgaps of the single-layer coatings are measured. For pure oxide materials a linear evolution of the LIDT with bandgap is observed. The results are in accordance with our simulations based on photo-ionization and avalanche-ionization. In the case of mixtures, however, deviations from the previous behaviors are evidenced. The evolution of the LIDT as a function of the refractive index is analyzed, and an empirical description of the relation between refractive index and LIDT is proposed.
RESUMEN
ZrO2-SiO2 and Nb2O5-SiO2 mixture coatings as well as those of pure zirconia (ZrO2), niobia (Nb2O5), and silica (SiO2) deposited by ion-beam sputtering were investigated. Refractive-index dispersions, bandgaps, and volumetric fractions of materials in mixed coatings were analyzed from spectrophotometric data. Optical scattering, surface roughness, nanostructure, and optical resistance were also studied. Zirconia-silica mixtures experience the transition from crystalline to amorphous phase by increasing the content of SiO2. This also results in reduced surface roughness. All niobia and silica coatings and their mixtures were amorphous. The obtained laser-induced damage thresholds in the subpicosecond range also correlates with respect to the silica content in both zirconia- and niobia-silica mixtures.
